Enhancing the magneto-optical Kerr effect through the use of a plasmonic antenna.

We employ an extended finite-element model as a design tool capable of incorporating the interaction between plasmonic antennas and magneto-optical effects, specifically the magneto-optical Kerr effect (MOKE). We first test our model in the absence of an antenna and show that for a semi-infinite thin-film, good agreement is obtained between our finite-element model and analytical calculations. The addition of a plasmonic antenna is shown to yield a wavelength dependent enhancement of the MOKE. The antenna geometry and its separation from the magnetic material are found to impact the strength of the observed MOKE signal, as well as the antenna's resonance wavelength. Through optimization of these parameters we achieved a MOKE enhancement of more than 100 when compared to a magnetic film alone. These initial results show that our modeling methodology offers a tool to guide the future fabrication of hybrid plasmonic magneto-optical devices and plasmonic antennas for magneto-optical sensing.

Direct Detection of Pure ac Spin Current by X-Ray Pump-Probe Measurements.

Despite recent progress in spin-current research, the detection of spin current has mostly remained indirect. By synchronizing a microwave waveform with synchrotron x-ray pulses, we use the ferromagnetic resonance of the Py (Ni_{81}Fe_{19}) layer in a Py/Cu/Cu_{75}Mn_{25}/Cu/Co multilayer to pump a pure ac spin current into the Cu_{75}Mn_{25} and Co layers, and then directly probe the spin current within the Cu_{75}Mn_{25} layer and the spin dynamics of the Co layer by x-ray magnetic circular dichroism. This element-resolved pump-probe measurement unambiguously identifies the ac spin current in the Cu_{75}Mn_{25} layer.

Ultrafast optical parametric pumping of magnetization reorientation and precessional dynamics in DyFe2/YFe2 exchange springs.

The magnetization dynamics of a wound [DyFe(2)(20 Å)/YFe(2)(80 Å)](×40) exchange spring multilayer have been explored in optical pump probe experiments. Ultrafast optical heating was used to modify the magnetic parameters of the multilayer, while the time resolved magneto-optical Kerr effect was used to probe its response. Although the probe signal is dominated by precession and winding of the exchange spring within the soft YFe(2) layer, reorientation of the DyFe(2) hard-layer magnetization is detected on time scales less than 100 ps. Micromagnetic simulations reproduce the main features of the experimental data and indicate a dramatic optically induced reduction of the hard-layer anisotropy. The results establish the feasibility of switching a spring system by means of parametric excitation.

Isolating the dynamic dipolar interaction between a pair of nanoscale ferromagnetic disks.

Dynamic dipolar interactions between spin wave eigenmodes of closely spaced nanomagnets determine the collective behavior of magnonic and spintronic metamaterials and devices. However, dynamic dipolar interactions are difficult to quantify since their effects must be disentangled from those of static dipolar interactions and variations in the shape, size, and magnetic properties of the nanomagnets. It is shown that when two imperfect nanoscale magnetic disks with similar but nonidentical modes are brought into close proximity, the effect of the dynamic dipolar interaction can be detected by considering the difference of the phase of precession within the two disks. Measurements show that the interaction is stronger than expected from micromagnetic simulations, highlighting both the need for characterization and control of magnetic properties at the deep nanoscale, and also the potential for improved control of collective magnetic phenomena. Our approach is equally applicable to other physical systems in which dynamic interactions are obscured by inhomogeneous broadening and static interactions.

Imaging collective magnonic modes in 2D arrays of magnetic nanoelements.

We have used time resolved scanning Kerr microscopy to image collective spin wave modes within a 2D array of magnetic nanoelements. Long wavelength spin waves are confined within the array as if it was a continuous element of the same size but with effective material properties determined by the structure of the array and its constituent nanoelements. The array is an example of a magnonic metamaterial, the demonstration of which provides new opportunities within the emerging field of magnonics.

Coherent ac spin current transmission across an antiferromagnetic CoO insulator.

The recent discovery of spin current transmission through antiferromagnetic insulating materials opens up vast opportunities for fundamental physics and spintronics applications. The question currently surrounding this topic is: whether and how could THz antiferromagnetic magnons mediate a GHz spin current? This mismatch of frequencies becomes particularly critical for the case of coherent ac spin current, raising the fundamental question of whether a GHz ac spin current can ever keep its coherence inside an antiferromagnetic insulator and so drive the spin precession of another ferromagnet layer coherently? Utilizing element- and time-resolved x-ray pump-probe measurements on Py/Ag/CoO/Ag/Fe75Co25/MgO(001) heterostructures, here we demonstrate that a coherent GHz ac spin current pumped by the Py ferromagnetic resonance can transmit coherently across an antiferromagnetic CoO insulating layer to drive a coherent spin precession of the Fe75Co25 layer. Further measurement results favor thermal magnons rather than evanescent spin waves as the mediator of the coherent ac spin current in CoO.

Investigation of magnetic droplet solitons using x-ray holography with extended references.

A dissipative magnetic soliton, or magnetic droplet, is a structure that has been predicted to exist within a thin magnetic layer when non-linearity is balanced by dispersion, and a driving force counteracts the inherent damping of the spin precession. Such a soliton can be formed beneath a nano-contact (NC) that delivers a large spin-polarized current density into a magnetic layer with perpendicular magnetic anisotropy. Although the existence of droplets has been confirmed from electrical measurements and by micromagnetic simulations, only a few attempts have been made to directly observe the magnetic landscape that sustains these structures, and then only for a restricted set of experimental parameter values. In this work we use and x-ray holography technique HERALDO, to image the magnetic structure of the [Co/Ni]x4 multilayer within a NC orthogonal pseudo spin-valve, for different range of magnetic fields and injected electric currents. The magnetic configuration imaged at -33 mA and 0.3 T for devices with 90 nm NC diameter reveals a structure that is within the range of current where the droplet soliton exist based on our electrical measurements and have it is consistent with the expected size of the droplet (∼100 nm diameter) and its spatial position within the sample. We also report the magnetisation configurations observed at lower DC currents in the presence of fields (0-50 mT), where it is expected to observe regimes of the unstable droplet formation.

Time-resolved imaging of magnetic vortex dynamics using holography with extended reference autocorrelation by linear differential operator.

The magnetisation dynamics of the vortex core and Landau pattern of magnetic thin-film elements has been studied using holography with extended reference autocorrelation by linear differential operator (HERALDO). Here we present the first time-resolved x-ray measurements using this technique and investigate the structure and dynamics of the domain walls after excitation with nanosecond pulsed magnetic fields. It is shown that the average magnetisation of the domain walls has a perpendicular component that can change dynamically depending on the parameters of the pulsed excitation. In particular, we demonstrate the formation of wave bullet-like excitations, which are generated in the domain walls and can propagate inside them during the cyclic motion of the vortex core. Based on numerical simulations we also show that, besides the core, there are four singularities formed at the corners of the pattern. The polarisation of these singularities has a direct relation to the vortex core, and can be switched dynamically by the wave bullets excited with a magnetic pulse of specific parameters. The subsequent dynamics of the Landau pattern is dependent on the particular configuration of the polarisations of the core and the singularities.

Observation of T2-like coherent optical phonons in epitaxial Ge2Sb2Te5/GaSb(001) films.

The phonon spectrum of Ge2Sb2Te5 is a signature of its crystallographic structure and underlies the phase transition process used in memory applications. Epitaxial materials allow coherent optical phonons to be studied in femtosecond anisotropic reflectance measurements. A dominant phonon mode with frequency of 3.4 THz has been observed in epitaxial Ge2Sb2Te5 grown on GaSb(001). The dependence of signal strength upon pump and probe polarization is described by a theory of transient stimulated Raman scattering that accounts for the symmetry of the crystallographic structure through use of the Raman tensor. The 3.4 THz mode has the character of the 3 dimensional T2 mode expected for the O(h) point group, confirming that the underlying crystallographic structure is cubic. New modes are observed in both Ge2Sb2Te5 and GaSb after application of large pump fluences, and are interpreted as 1 and 2 dimensional modes associated with segregation of Sb.

Ultrafast magnetization dynamics of spintronic nanostructures.

The ultrafast (sub-nanosecond) magnetization dynamics of ferromagnetic thin films and elements that find application in spintronic devices is reviewed. The major advances in the understanding of magnetization dynamics in the two decades since the discovery of giant magnetoresistance and the prediction of spin-transfer torque are discussed, along with the plethora of new experimental techniques developed to make measurements on shorter length and time scales. Particular consideration is given to time-resolved measurements of the magneto-optical Kerr effect, and it is shown how a succession of studies performed with this technique has led to an improved understanding of the dynamics of nanoscale magnets. The dynamics can be surprisingly rich and complicated, with the latest studies of individual nanoscale elements showing that the dependence of the resonant mode spectrum upon the physical structure is still not well understood. Finally, the article surveys the prospects for development of high-frequency spintronic devices and highlights areas in which further study of fundamental properties will be required within the coming decade.

Ultrafast nanomagnets: seeing data storage in a new light.

Magnetic materials provide the most important form of erasable data storage for information technology today. The demand for increased storage capacity has caused bit sizes and features of the read-write transducers to be reduced to the nanoscale. However, increased storage capacity is only useful if there is a commensurate reduction in the time taken to read and write the data. In this article, the basic principles that determine the behaviour of nanomagnetic materials are introduced and their use in data-storage systems is described. Particular attention is paid to processes that limit the speed of operation of the data-storage system. It is shown that optical pump-probe experiments may be used to characterize dynamic magnetic processes with femtosecond temporal resolution. The macroscopic magnetization of a ferromagnet can be made to precess in response to an optically triggered magnetic field pulse, leading to reduced switching times. Alternatively, an ultrashort laser pulse may be used to manipulate the magnitude of the magnetization on femtosecond time-scales, leading to an ultrafast demagnetization in certain ferromagnets, and providing new insight into magnetotransport phenomena. Finally, the outlook for increased record and replay rates is assessed and the prospect of further use of optical techniques within magnetic data-storage technology is discussed.