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1.
J Am Chem Soc ; 133(10): 3252-5, 2011 Mar 16.
Artigo em Inglês | MEDLINE | ID: mdl-21341739

RESUMO

The effect of chemical and hydrostatic pressure has been studied systematically in a selected system belonging to the 1111 family of iron pnictide high-temperature superconductors. The results show a surprising similarity between the trend of critical temperature vs hydrostatic pressure for isoelectronic samples with different rare earths (RE) on the RE site and samples of the SmFeAsO(1-x)F(x) series with different doping levels. These results open new questions about the underlying mechanism for superconductivity in iron pnictides.

2.
Rev Sci Instrum ; 78(1): 013903, 2007 Jan.
Artigo em Inglês | MEDLINE | ID: mdl-17503929

RESUMO

Torque magnetometry is a powerful method to determine a sample's magnetic properties. In a torque magnetometer, the sample under interest is mounted on a suitable sensor, the core part of the instrument. Piezoresistive atomic force microscope tips are proven to be very useful torque sensors and have already been optimized for the specific needs of torque magnetometry. However, this type of sensor did not offer the possibility of measuring torque along two perpendicular directions simultaneously without sacrificing sensitivity. In this article we demonstrate a fundamentally new sensor design based on the piezoresistive readout technique, which offers a large variability of measurement modes. With a symmetric arrangement of the sensor legs, concurrent two-axis measurements are easily possible with two separate readout circuits. Furthermore, the variability can be exploited by fabricating a thermometer on the sample platform to directly measure the sample temperature. Test measurements are in good agreement with elasticity calculations.


Assuntos
Magnetismo , Microscopia de Força Atômica , Microscopia de Força Atômica/instrumentação , Microscopia de Força Atômica/métodos
3.
Sci Rep ; 5: 12528, 2015 Jul 30.
Artigo em Inglês | MEDLINE | ID: mdl-26224422

RESUMO

In the generic phase diagram of heavy fermion systems, tuning an external parameter such as hydrostatic or chemical pressure modifies the superconducting transition temperature. The superconducting phase forms a dome in the temperature-tuning parameter phase diagram, which is associated with a maximum of the superconducting pairing interaction. Proximity to antiferromagnetism suggests a relation between the disappearance of antiferromagnetic order and superconductivity. We combine muon spin rotation, neutron scattering, and x-ray absorption spectroscopy techniques to gain access to the magnetic and electronic structure of CeCo(In(1-x)Cdx)5 at different time scales. Different magnetic structures are obtained that indicate a magnetic order of itinerant character, coexisting with bulk superconductivity. The suppression of the antiferromagnetic order appears to be driven by a modification of the bandwidth/carrier concentration, implying that the electronic structure and consequently the interplay of superconductivity and magnetism is strongly affected by hydrostatic and chemical pressure.

4.
J Phys Condens Matter ; 27(26): 262201, 2015 Jul 08.
Artigo em Inglês | MEDLINE | ID: mdl-26053273

RESUMO

EuTiO3 exhibits strong magneto-electric coupling at the onset of antiferromagnetic order below TN = 5.7 K. The dielectric permittivity drops at TN by 7% and recovers to normal values with increasing magnetic field. This effect is shown to stem from tiny lattice effects as seen in magnetostriction data which directly affect the soft optic mode and its polarizability coordinate. By combining experimental results with theory we show that marginal changes in the lattice parameter of the order of 0.01% have a more than 1000% effect on the transverse optic soft mode of ETO and thus easily induce a ferroelectric instability.

5.
J Phys Condens Matter ; 24(23): 233201, 2012 Jun 13.
Artigo em Inglês | MEDLINE | ID: mdl-22551702

RESUMO

In this review we consider three classes of superconductors, namely cuprate superconductors, MgB(2) and the new Fe based superconductors. All of these three systems are layered materials and multiband compounds. Their pairing mechanisms are under discussion with the exception of MgB(2), which is widely accepted to be a 'conventional' electron-phonon interaction mediated superconductor, but extending the Bardeen-Cooper-Schrieffer (BCS) theory to account for multiband effects. Cuprates and Fe based superconductors have higher superconducting transition temperatures and more complex structures. Superconductivity is doping dependent in these material classes unlike in MgB(2) which, as a pure compound, has the highest values of T(c) and a rapid suppression of superconductivity with doping takes place. In all three material classes isotope effects have been observed, including exotic ones in the cuprates, and controversial ones in the Fe based materials. Before the area of high-temperature superconductivity, isotope effects on T(c) were the signature for phonon mediated superconductivity-even when deviations from the BCS value to smaller values were observed. Since the discovery of high T(c) materials this is no longer evident since competing mechanisms might exist and other mediating pairing interactions are discussed which are of purely electronic origin. In this work we will compare the three different material classes and especially discuss the experimentally observed isotope effects of all three systems and present a rather general analysis of them. Furthermore, we will concentrate on multiband signatures which are not generally accepted in cuprates even though they are manifest in various experiments, the evidence for those in MgB(2), and indications for them in the Fe based compounds. Mostly we will consider experimental data, but when possible also discuss theoretical models which are suited to explain the data.

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