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1.
Nano Lett ; 18(3): 1724-1732, 2018 03 14.
Artigo em Inglês | MEDLINE | ID: mdl-29433320

RESUMO

We report an experimental observation and direct control of quantum transport in artificial two-dimensional Au lattices. Combining the advanced techniques of low-temperature deposition and newly developed double-probe scanning tunneling spectroscopy, we display a two-dimensional carrier transport and demonstrate a strong in-plane transport modulation in the two-dimensional Au lattices. In well-ordered Au lattices, we observe the carrier transport behavior manifesting as a band-like feature with an energy gap. Furthermore, controlled structural modification performed by constructing coupled "stadiums" enables a transition of system dynamics in the lattices, which in turn establishes tunable resonant transport throughout a wide energy range. Our findings open the possibility of the construction and transport engineering of artificial lattices by the geometrical arrangement of scatterers and quantum chaotic dynamics.

2.
Sci Adv ; 8(16): eabm9896, 2022 Apr 22.
Artigo em Inglês | MEDLINE | ID: mdl-35452283

RESUMO

We study a Cooper pair transistor realized by two Josephson weak links that enclose a superconducting island in an InSb-Al hybrid nanowire. When the nanowire is subject to a magnetic field, isolated subgap levels arise in the superconducting island and, because of the Coulomb blockade, mediate a supercurrent by coherent cotunneling of Cooper pairs. We show that the supercurrent resulting from such cotunneling events exhibits, for low to moderate magnetic fields, a phase offset that discriminates even and odd charge ground states on the superconducting island. Notably, this phase offset persists when a subgap state approaches zero energy and, based on theoretical considerations, permits parity measurements of subgap states by supercurrent interferometry. Such supercurrent parity measurements could, in a series of experiments, provide an alternative approach for manipulating and protecting quantum information stored in the isolated subgap levels of superconducting islands.

3.
Nat Commun ; 12(1): 4914, 2021 Aug 13.
Artigo em Inglês | MEDLINE | ID: mdl-34389705

RESUMO

The realization of hybrid superconductor-semiconductor quantum devices, in particular a topological qubit, calls for advanced techniques to readily and reproducibly engineer induced superconductivity in semiconductor nanowires. Here, we introduce an on-chip fabrication paradigm based on shadow walls that offers substantial advances in device quality and reproducibility. It allows for the implementation of hybrid quantum devices and ultimately topological qubits while eliminating fabrication steps such as lithography and etching. This is critical to preserve the integrity and homogeneity of the fragile hybrid interfaces. The approach simplifies the reproducible fabrication of devices with a hard induced superconducting gap and ballistic normal-/superconductor junctions. Large gate-tunable supercurrents and high-order multiple Andreev reflections manifest the exceptional coherence of the resulting nanowire Josephson junctions. Our approach enables the realization of 3-terminal devices, where zero-bias conductance peaks emerge in a magnetic field concurrently at both boundaries of the one-dimensional hybrids.

4.
ACS Appl Mater Interfaces ; 6(16): 13823-32, 2014 Aug 27.
Artigo em Inglês | MEDLINE | ID: mdl-25055030

RESUMO

We investigated the interface between hexagonal ZnO films and cubic MgO (001) substrates, fabricated via molecular beam epitaxy. X-ray diffraction and (scanning) transmission electron microscopy revealed that growth follows the single [0001] direction when the temperature of the substrate is above 200 °C, while when the substrate temperature is below 150 °C, growth initially is along [0001] and then mainly changes to [0-332] variants beyond a thickness of ∼10 nm. Interestingly, a double-domain feature with a rotational angle of 30° appears during growth along [0001] regardless of the temperature, experimentally demonstrating the theoretical predictions for the occurrence of double rotational domains in such a heteroepitaxy [Grundmann et al., Phys. Rev. Lett. 105, 146102 (2010)]. We also found that the optical properties of the ZnO film are influenced greatly by the mutation of growth directions, stimulated by the bond-length modulations, as we determined from X-ray absorption spectra at Zn K edge. These results also showed the evolution of the 4p(xy) and 4p(z) states in the conduction band with the rise in the temperature for growth. We consider that our findings may well promote the applications of ZnO in advanced optoelectronics for which its integration with other materials of different phases is desirable.

5.
Nanoscale ; 5(2): 574-80, 2013 Jan 21.
Artigo em Inglês | MEDLINE | ID: mdl-23196786

RESUMO

Periodic Ag nanoball (NB) arrays on ZnO hollow nanosphere (HNS) supporting structures were fabricated in a large area by a laser irradiation method. The optimized laser power and spherical supporting structure of ZnO with a certain size and separation were employed to aggregate a sputtering-deposited Ag nano-film into an ordered, large-area, and two dimensional Ag NB array. A significant band edge (BE) emission enhancement of ZnO HNSs was achieved on this Ag NB/ZnO HNS hybrid structure and the mechanism was revealed by further experimental and theoretical analyses. With successfully fabricating the direct-contact structure of a Ag NB on the top of each ZnO HNS, the highly localized quadrupole mode surface plasmon resonance (SPR), realized on the metal NBs in the ultraviolet region, can effectively improve the BE emission of ZnO through strong coupling with the excitons of ZnO. Compared with the dipole mode SPR, the quadrupole mode SPR is insensitive to the metal nanoparticle's size and has a resonance frequency in the BE region of the wide band gap materials, hence, it can be potentially applied in related optoelectronic devices.


Assuntos
Nanotecnologia/métodos , Prata/química , Ressonância de Plasmônio de Superfície/métodos , Óxido de Zinco/química , Eletrônica , Lasers , Nanopartículas Metálicas/química , Microscopia Eletrônica de Varredura/métodos , Microscopia Eletrônica de Transmissão/métodos , Conformação Molecular , Óptica e Fotônica , Oxigênio/química , Fótons , Poliestirenos/química , Semicondutores , Espectrofotometria Ultravioleta/métodos , Temperatura , Fatores de Tempo , Difração de Raios X
6.
Sci Rep ; 3: 3551, 2013 Dec 19.
Artigo em Inglês | MEDLINE | ID: mdl-24352032

RESUMO

The vacuum Rabi splitting of exciton-polariton emission is observed in cathodoluminescence (CL) and photoluminescence spectra of an AlN epitaxial film. Atomic force microscopy and CL measurements show that the film has an atomically flat surface, high purity, and high crystal quality. By changing the temperature, anticrossing behavior between the upper and lower polariton branch can be obtained in low temperature with a Rabi splitting of 44 meV, in agreement with the calculation. This large energy splitting is caused by strong oscillator strength, intrinsically pure polarization in wurtzite AlN semiconductor, and high fraction of free exciton in the sample. These properties indicate that AlN can be a potential semiconductor for the further development of polariton physics and polariton-based novel devices.

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