RESUMO
Circular dichroism (CD) is highly required in the applications of biological detection and analytical chemistry. In this paper, we achieved a giant, broadband, and strength-switchable CD effect in a quadruple z-shaped G e 2 S b 2 T e 5 (GST) metasurface. At the amorphous state of GST (a-GST), the giant CD reaches 0.92 and the width of the absorption >0.80 is about 100 nm. The giant and broadband CD originates from polarization selective excitations of Mie resonances and the coupling between subunit resonators. With the transition from a-GST to crystalline GST, CD could be dynamically switched from 0.92 to 0.05. The GST-based metasurfaces with giant and wide-range switching CD will promote the development of active chiral devices.
RESUMO
A multifunctional metasurface capable of dynamic control for polarization selectivity and absorption is proposed by controlling the phase of Ge2Sb2Te5 (GST) in the near-infrared region. At amorphous state of GST (a-GST), the proposed GST strip array realized polarization selectivity in transmission-reflection integrated modes. The high-efficiency asymmetric transmission (AT = 0.92) and asymmetric reflection (AR = -0.82) are both obtained by selectively exciting Mie multipole resonances. With the transition from a-GST to crystalline (c-GST) state, the giant polarization selectivity almost disappeared, and the absorptions climb from < 0.1 to > 0.9. The maximum modulation depth reaches 94%. The mechanism of the dynamic switching between polarization selectivity and absorption is quantitively analyzed via multipole expansion. The GST based metasurfaces simultaneously possess excellent switchable capability for AT, AR, and absorption without refabricating structures, which is promising to the applications for next generation optical devices.
RESUMO
Circular dichroism (CD) is originally obtained from three-dimensional spiral structures by simultaneously exciting electric and magnetic resonances. To simplify construction, multilayer stacked asymmetric structures and the symmetric structures relying on oblique incidence are proposed for enhancing CD. Herein, we achieved the enhancement of dual-waveband CD by adding a Ge2Sb2Te5 (GST) layer on the top of a Z-shape gold array in a normally incident system. Benefited from the polarization selective excitations of electric and magnetic dipole resonances, the CD in a simple planar structure is immensely enhanced from near zero to 0.73 at 1.58 µm. Furthermore, the CD strengths is dynamically tuned by controlling the phase of GST. With the GST phase transition from amorphous (a-GST) to crystalline state (c-GST), CD magnitudes are switched by about 0.73 and 0.27 at dual wavebands respectively. The enhancement of CD by adding a layer on a simple planar array offers a new method for designing planar metasurfaces with strong chirality.
RESUMO
Circular dichroism (CD) is required in the applications of biological detection, analytical chemistry, etc. Here, we numerically demonstrated large-range switchable CD by controlling the phase change of Ge2Sb2Te5 (GST) in a zigzag array. At the amorphous state of GST (a-GST), the strong and dual-waveband CD effects are realized via the selective excitations of electric, magnetic, and toroidal resonances. With the transition from a-GST to crystalline state GST, CD strengths are tailored dynamically in large ranges. In detail, the CD magnitudes change by about 0.93 and the modulation depths exceed 94% at dual wavebands. The strong CD effects and large-range switch capability in the GST-based metasurfaces will boost the development of active chiroptical devices.