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1.
Appl Opt ; 59(31): 9896-9904, 2020 Nov 01.
Artigo em Inglês | MEDLINE | ID: mdl-33175827

RESUMO

The total ozone column amount (TOCA) values from the Ozone Monitoring Instrument (OMI) derived from OMI/Aura ozone (O3) differential optical absorption spectroscopy (DOAS) V003 (OMDOAO3) have been validated against the ground-based TOCA values derived from Dobson and the Norwegian Institute for Air Research UV measurements in Kampala (0.31º N, 32.58º E, 1200 m), Uganda, for the period between 2005 and 2018. Under all-sky conditions, the OMI retrieval algorithm was found to underestimate the TOCA values with mean bias (MnB), root mean square error (RMSE), and correlation coefficient (r) values ranging from about -3.4% to -1.7%, 2.4% to 4.9%, and 0.73 to 0.90, respectively. When only days with a radiation modification factor greater than or equal to 65% were considered, the MnB, RMSE, and r values between TOCA values derived from ground-based and OMI measurements improved, and they ranged from -2.5% to -1.3%, 1.4% to 3.8%, and 0.8 to 0.91, respectively. A good agreement was found between TOCA values derived from Dobson measurements and those derived from OMI satellite measurements with MnB, RMSE, and r values of about -1.8%, 1.4%, and 0.91, respectively. This was due to the fact that Dobson measurements were taken only when the sky was perceived clear. The underestimation of TOCA values by the OMI retrieval algorithm was found to be due mainly to clouds and aerosols.

2.
Appl Opt ; 54(6): 1505-14, 2015 Feb 20.
Artigo em Inglês | MEDLINE | ID: mdl-25968219

RESUMO

Between February 2012 and April 2014, we measured and analyzed direct solar radiances at a ground-based station in Bergen, Norway. We discovered that the spectral aerosol optical thickness (AOT) and precipitable water vapor column (PWVC) retrieved from these measurements have a seasonal variation with highest values in summer and lowest values in winter. The highest value of the monthly median AOT at 440 nm of about 0.16 was measured in July and the lowest of about 0.04 was measured in December. The highest value of the monthly median PWVC of about 2.0 cm was measured in July and the lowest of about 0.4 cm was measured in December. We derived Ångström exponents that were used to deduce aerosol particle size distributions. We found that coarse-mode aerosol particles dominated most of the time during the measurement period, but fine-mode aerosol particles dominated during the winter seasons. The derived Ångström exponent values suggested that aerosols containing sea salt could have been dominating at this station during the measurement period.

3.
Appl Opt ; 54(28): 8537-45, 2015 Oct 01.
Artigo em Inglês | MEDLINE | ID: mdl-26479632

RESUMO

The Ozone Monitoring Instrument (OMI) overpass solar ultraviolet (UV) indices have been validated against the ground-based UV indices derived from Norwegian Institute for Air Research UV measurements in Kampala (0.31° N, 32.58° E, 1200 m), Uganda for the period between 2005 and 2014. An excessive use of old cars, which would imply a high loading of absorbing aerosols, could cause the OMI retrieval algorithm to overestimate the surface UV irradiances. The UV index values were found to follow a seasonal pattern with maximum values in March and October. Under all-sky conditions, the OMI retrieval algorithm was found to overestimate the UV index values with a mean bias of about 28%. When only days with radiation modification factor greater than or equal to 65%, 70%, 75%, and 80% were considered, the mean bias between ground-based and OMI overpass UV index values was reduced to 8%, 5%, 3%, and 1%, respectively. The overestimation of the UV index by the OMI retrieval algorithm was found to be mainly due to clouds and aerosols.


Assuntos
Poluentes Atmosféricos/análise , Monitoramento Ambiental/métodos , Ozônio/análise , Raios Ultravioleta , Aerossóis , Algoritmos , Automóveis , Calibragem , Simulação por Computador , Reprodutibilidade dos Testes , Estações do Ano , Astronave , Espectrofotometria Ultravioleta , Luz Solar , Uganda
4.
Appl Opt ; 53(14): 2964-73, 2014 May 10.
Artigo em Inglês | MEDLINE | ID: mdl-24922014

RESUMO

Aerosols affect the climate directly through absorption and reflection of sunlight back to space and indirectly by acting as cloud condensation nuclei. This paper is based on more than three decades of satellite data (1979-1994 and 1996-2012) from total ozone mapping spectrometer (TOMS) and ozone monitoring instrument (OMI), which have provided measurements of backscattered radiances in the wavelength range from 331 to 380 nm. These data have been used to determine the aerosol climatology and to investigate the influence of the aerosol index (AI) on the ultraviolet index (UVI) in coastal land areas in Serrekunda (13.28°N, 16.34°W), The Gambia, and Dar-es-Salaam (6.8°S, 39.26°E), Tanzania, as well as in inland areas in Kampala (0.19°N, 32.34°E), Uganda. Heavy aerosol loadings were found to occur in the dry seasons at all three locations. To reduce the influence of clouds, we disregarded TOMS and OMI data for days during which the UV reflectivity was larger than 9% and investigated the correlation of the AI with the UVI for the remaining days at the three locations. We found a high correlation coefficient of 0.82 for Serrekunda, but poor correlation for Kampala and Dar-es-Salaam. The average AI for Serrekunda was found to be about three times higher than that for Kampala or Dar-es-Salaam, and a positive trend was found for the AI in Kampala and Dar-es-Salaam, whereas a negative trend was found for the AI in Serrekunda.


Assuntos
Aerossóis/análise , Poluentes Atmosféricos/análise , Atmosfera/química , Monitoramento Ambiental/métodos , Ozônio/análise , Refratometria/métodos , Análise Espectral/métodos , África , Atmosfera/análise , Fotometria/métodos
5.
Appl Opt ; 46(36): 8553-61, 2007 Dec 20.
Artigo em Inglês | MEDLINE | ID: mdl-18091964

RESUMO

Lake Victoria, Africa's largest freshwater lake, suffers greatly from negative changes in biomass of species of fish and also from severe eutrophication. The continuing deterioration of Lake Victoria's ecological functions has great long-term consequences for the ecosystem benefits it provides to the countries bordering its shores. However, knowledge about temporal and spatial variations of optical properties and how they relate to lake constituents is important for a number of reasons such as remote sensing, modeling of underwater light fields, and long-term monitoring of lake waters. Based on statistical analysis of data from optical measurements taken during half a year of weekly cruises in Murchison Bay, Lake Victoria, we present a three-component model for the absorption and a two-component model for the scattering of light in the UV and the visible regions of the solar spectrum along with tests of their ranges of validity. The three-component input to the model for absorption is the chlorophyll-a (Chl-a), total suspended materials concentrations, and yellow substance absorption, while the two-component input to the model for scattering is the Chl-a concentration and total suspended materials.


Assuntos
Clorofila/análise , Água Doce/análise , Água Doce/química , Modelos Químicos , Nefelometria e Turbidimetria/métodos , Fotometria/métodos , Poluentes Químicos da Água/análise , África , Clorofila A , Simulação por Computador
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