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1.
Nano Lett ; 23(10): 4152-4159, 2023 May 24.
Artigo em Inglês | MEDLINE | ID: mdl-37130341

RESUMO

Friedrich-Wintgen (FW) interference is an atypical coupling mechanism that grants loss exchange between leaky resonances in non-Hermitian classical and quantum systems. Intriguingly, such a mechanism makes destructive interference possible for scenarios in which a radiating wave becomes a bound state in the continuum (BIC) by giving away all of its losses. Here we propose and demonstrate experimentally an original concept to tailor FW-BICs with polarization singularity at on-demand wavevectors in an optical metasurface. As a proof-of-concept, using hybrid organic-inorganic halide perovskite as an active material, we empower this novel polarization singularity to obtain lasing emission, exhibiting both highly directional emission at oblique angles and a polarization vortex in momentum space. Our results pave the way to steerable coherent emission with a tailored polarization pattern for applications in optical communication/manipulation in free space, high-resolution imaging/focusing, and data storage.

2.
Appl Opt ; 59(19): 5697-5701, 2020 Jul 01.
Artigo em Inglês | MEDLINE | ID: mdl-32609692

RESUMO

We propose a method to pattern organic optically active materials based on local photobleaching for creating a wavelength-selective grating. Usually, photobleaching is considered a limitation for an organic emitter. Here, this property is exploited to locally suppress dye emission and absorption at the microscale with an abrupt interface and no changes in layer thickness. Periodic patterns were fabricated and exhibit diffraction only at a 590 nm wavelength with a spectral selectivity of 11 nm. Based on laser writer flexibility and efficiency, this study shows the potential of local photobleaching for applications such as wavelength-selective grating fabrication.

3.
J Opt Soc Am A Opt Image Sci Vis ; 31(5): 1067-73, 2014 May 01.
Artigo em Inglês | MEDLINE | ID: mdl-24979639

RESUMO

We report the experimental combination of leakage radiation microscopy with a Young slit experiment to address the spatial coherence properties of surface waves. We applied this method to measurements of surface plasmon polaritons (SPPs). The relationship between the spatial decay and interference contrast allows us to extract the degree of coherence. In a second step, we investigate the coherence properties of the plasmon in the weak coupling regime between fluorophores and metallic surfaces. Finally, a method is proposed to extract the propagation length of SPPs in a large variety of systems.

4.
Talanta ; 250: 123731, 2022 Dec 01.
Artigo em Inglês | MEDLINE | ID: mdl-35841661

RESUMO

Layer-by-layer self-assembly (L-b-L assembly) makes possible to obtain polyelectrolyte multilayers (PEMs) and one of the polyelectrolytes could be replaced by a dye molecule to obtain multilayers which may exhibit optical properties of great interest. On the other hand, µCp has become a routine technique for the preparation of micro- and nanostructured surfaces. In our development in progress of a surface engineering strategy to transfer J-Agg cyanine dyes onto surfaces by integrating L-b-L process and µCp, this contribution highlights how surface analysis imaging techniques can bring valuable information for the development of the process involving a double Multilayers Transfer Printing (MTP) with a Moiré effect. Key parameters sustaining image interpretation are difference in deposit thickness (optical microscopy, atomic force microscopy, scanning electron microscopy), in roughness (atomic force microscopy and scanning electron microscopy), in charge effect (scanning electron microscopy) and the chemical contrast between unprinted and printed areas (time-of-flight secondary ion mass spectrometry).


Assuntos
Corantes , Microscopia de Força Atômica , Microscopia Eletrônica de Varredura , Polieletrólitos , Propriedades de Superfície
5.
Proc Natl Acad Sci U S A ; 104(39): 15328-33, 2007 Sep 25.
Artigo em Inglês | MEDLINE | ID: mdl-17878301

RESUMO

We observe the myosin V stepping mechanism by traveling wave tracking. This technique, associated with optical tweezers, allows one to follow a scattering particle in a two-dimensional plane, with nanometer accuracy and a temporal resolution in the microsecond range. We have observed that, at the millisecond time scale, the myosin V combines longitudinal and vertical motions during the step. Because at this time scale the steps appear heterogeneous, we deduce their general features by aligning and averaging a large number of them. Our data show that the 36-nm step occurs in three main stages. First, the myosin center of mass moves forward 5 nm; the duration of this short prestep depends on the ATP concentration. Second, the motor performs a fast motion over 23 nm; this motion is associated to a vertical movement of the myosin center of mass, whose distance from the actin filament increases by 6 nm. Third, the myosin head freely diffuses toward the next binding site and the vertical position is recovered. We propose a simple model to describe the step mechanism of the dimeric myosin V.


Assuntos
Miosina Tipo V/química , Actinas/química , Actinas/metabolismo , Animais , Galinhas , Dimerização , Cinesinas/química , Modelos Moleculares , Modelos Estatísticos , Músculo Esquelético/metabolismo , Miosinas/química , Poliestirenos/química , Coelhos , Espectroscopia de Infravermelho com Transformada de Fourier , Termodinâmica
6.
Appl Opt ; 42(33): 6678-81, 2003 Nov 20.
Artigo em Inglês | MEDLINE | ID: mdl-14658472

RESUMO

Continuous-wave operation, to as high as 7 degrees C, of 1.5-microm optically pumped vertical-external-cavity surface-emitting lasers is reported. The epitaxial structure, monolithically grown on InP by metal-organic chemical vapor deposition, consists of an InAlAs/GaInAlAs Bragg reflector, an InGaAs/InGaAsP active region, and an InP capping layer. The threshold incident pump intensity is <9 kW/cm2.

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