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1.
Nat Mater ; 23(3): 377-382, 2024 Mar.
Artigo em Inglês | MEDLINE | ID: mdl-38195865

RESUMO

Topological insulators are a concept that originally stems from condensed matter physics. As a corollary to their hallmark protected edge transport, the conventional understanding of such systems holds that they are intrinsically closed, that is, that they are assumed to be entirely isolated from the surrounding world. Here, by demonstrating a parity-time-symmetric topological insulator, we show that topological transport exists beyond these constraints. Implemented on a photonic platform, our non-Hermitian topological system harnesses the complex interplay between a discrete coupling protocol and judiciously placed losses and, as such, inherently constitutes an open system. Nevertheless, even though energy conservation is violated, our system exhibits an entirely real eigenvalue spectrum as well as chiral edge transport. Along these lines, this work enables the study of the dynamical properties of topological matter in open systems without the instability arising from complex spectra. Thus, it may inspire the development of compact active devices that harness topological features on-demand.

2.
Rep Prog Phys ; 87(3)2024 Feb 15.
Artigo em Inglês | MEDLINE | ID: mdl-38241725

RESUMO

For decades, frustrated quantum magnets have been a seed for scientific progress and innovation in condensed matter. As much as the numerical tools for low-dimensional quantum magnetism have thrived and improved in recent years due to breakthroughs inspired by quantum information and quantum computation, higher-dimensional quantum magnetism can be considered as the final frontier, where strong quantum entanglement, multiple ordering channels, and manifold ways of paramagnetism culminate. At the same time, efforts in crystal synthesis have induced a significant increase in the number of tangible frustrated magnets which are generically three-dimensional in nature, creating an urgent need for quantitative theoretical modeling. We review the pseudo-fermion (PF) and pseudo-Majorana (PM) functional renormalization group (FRG) and their specific ability to address higher-dimensional frustrated quantum magnetism. First developed more than a decade ago, the PFFRG interprets a Heisenberg model Hamiltonian in terms of Abrikosov pseudofermions, which is then treated in a diagrammatic resummation scheme formulated as a renormalization group flow ofm-particle pseudofermion vertices. The article reviews the state of the art of PFFRG and PMFRG and discusses their application to exemplary domains of frustrated magnetism, but most importantly, it makes the algorithmic and implementation details of these methods accessible to everyone. By thus lowering the entry barrier to their application, we hope that this review will contribute towards establishing PFFRG and PMFRG as the numerical methods for addressing frustrated quantum magnetism in higher spatial dimensions.

3.
Proc Natl Acad Sci U S A ; 118(32)2021 08 10.
Artigo em Inglês | MEDLINE | ID: mdl-34349024

RESUMO

The transfer of topological concepts from the quantum world to classical mechanical and electronic systems has opened fundamentally different approaches to protected information transmission and wave guidance. A particularly promising emergent technology is based on recently discovered topolectrical circuits that achieve robust electric signal transduction by mimicking edge currents in quantum Hall systems. In parallel, modern active matter research has shown how autonomous units driven by internal energy reservoirs can spontaneously self-organize into collective coherent dynamics. Here, we unify key ideas from these two previously disparate fields to develop design principles for active topolectrical circuits (ATCs) that can self-excite topologically protected global signal patterns. Realizing autonomous active units through nonlinear Chua diode circuits, we theoretically predict and experimentally confirm the emergence of self-organized protected edge oscillations in one- and two-dimensional ATCs. The close agreement between theory, simulations, and experiments implies that nonlinear ATCs provide a robust and versatile platform for developing high-dimensional autonomous electrical circuits with topologically protected functionalities.

4.
Nano Lett ; 23(7): 2476-2482, 2023 Apr 12.
Artigo em Inglês | MEDLINE | ID: mdl-36972710

RESUMO

Step edges of topological crystalline insulators can be viewed as predecessors of higher-order topology, as they embody one-dimensional edge channels embedded in an effective three-dimensional electronic vacuum emanating from the topological crystalline insulator. Using scanning tunneling microscopy and spectroscopy, we investigate the behavior of such edge channels in Pb1-xSnxSe under doping. Once the energy position of the step edge is brought close to the Fermi level, we observe the opening of a correlation gap. The experimental results are rationalized in terms of interaction effects which are enhanced since the electronic density is collapsed to a one-dimensional channel. This constitutes a unique system to study how topology and many-body electronic effects intertwine, which we model theoretically through a Hartree-Fock analysis.

5.
Angew Chem Int Ed Engl ; 63(15): e202400313, 2024 Apr 08.
Artigo em Inglês | MEDLINE | ID: mdl-38316614

RESUMO

Replacement of sp2-hybridized carbon in polycyclic aromatic hydrocarbons (PAHs) by boron affords electron-deficient π-scaffolds due to the vacant pz-orbital of three-coordinate boron with the potential for pronounced electronic interactions with electron-rich metal surfaces. Using a diboraperylene diborinic acid derivative as precursor and a controlled on-surface non-covalent synthesis approach, we report on a self-assembled chiral supramolecular kagome network on an Ag(111) surface stabilized by intermolecular hydrogen-bonding interactions at low temperature. Scanning tunneling microscopy (STM) and spectroscopy (STS) reveal a flat band at ca. 0.33 eV above the Fermi level which is localized at the molecule center, in good agreement with tight-binding model calculations of flat bands characteristic for kagome lattices.

6.
Phys Rev Lett ; 130(25): 256001, 2023 Jun 23.
Artigo em Inglês | MEDLINE | ID: mdl-37418713

RESUMO

We study the quasiparticle interference (QPI) pattern emanating from a pair of adjacent impurities on the surface of a gapped superconductor (SC). We find that hyperbolic fringes (HFs) in the QPI signal can appear due to the loop contribution of the two-impurity scattering, where the locations of the two impurities are the hyperbolic focus points. For a single pocket Fermiology, a HF pattern signals chiral SC order for nonmagnetic impurities and requires magnetic impurities for a nonchiral SC. For a multipocket scenario, a sign-changing order parameter such as an s_{±} wave likewise yields a HF signature. We discuss twin impurity QPI as a new tool to complement the analysis of superconducting order from local spectroscopy.

7.
Phys Rev Lett ; 131(1): 016901, 2023 Jul 07.
Artigo em Inglês | MEDLINE | ID: mdl-37478434

RESUMO

We report high resolution polar Kerr effect measurements on CsV_{3}Sb_{5} single crystals in search of signatures of spontaneous time-reversal symmetry breaking below the charge-order transition at T^{*}≈94 K. Utilizing two different versions of zero-area loop Sagnac interferometers operating at 1550 nm wavelength, each with the fundamental attribute that without a time-reversal symmetry breaking sample at its path, the interferometer is perfectly reciprocal, we find no observable Kerr effect to within the noise floor limit of the apparatus at 30 nanoradians. Simultaneous coherent reflection ratio measurements confirm the sharpness of the charge-order transition in the same optical volume as the Kerr measurements. At finite magnetic field we observe a sharp onset of a diamagnetic shift in the Kerr signal at T^{*}, which persists down to the lowest temperature without change in trend. Since 1550 nm is an energy that was shown to capture all features of the optical properties of the material that interact with the charge-order transition, we are led to conclude that it is highly unlikely that time-reversal symmetry is broken in the charge ordered state in CsV_{3}Sb_{5}.

8.
Nat Mater ; 20(10): 1353-1357, 2021 Oct.
Artigo em Inglês | MEDLINE | ID: mdl-34112979

RESUMO

Intertwining quantum order and non-trivial topology is at the frontier of condensed matter physics1-4. A charge-density-wave-like order with orbital currents has been proposed for achieving the quantum anomalous Hall effect5,6 in topological materials and for the hidden phase in cuprate high-temperature superconductors7,8. However, the experimental realization of such an order is challenging. Here we use high-resolution scanning tunnelling microscopy to discover an unconventional chiral charge order in a kagome material, KV3Sb5, with both a topological band structure and a superconducting ground state. Through both topography and spectroscopic imaging, we observe a robust 2 × 2 superlattice. Spectroscopically, an energy gap opens at the Fermi level, across which the 2 × 2 charge modulation exhibits an intensity reversal in real space, signalling charge ordering. At the impurity-pinning-free region, the strength of intrinsic charge modulations further exhibits chiral anisotropy with unusual magnetic field response. Theoretical analysis of our experiments suggests a tantalizing unconventional chiral charge density wave in the frustrated kagome lattice, which can not only lead to a large anomalous Hall effect with orbital magnetism, but also be a precursor of unconventional superconductivity.

9.
Phys Rev Lett ; 128(9): 099901, 2022 Mar 04.
Artigo em Inglês | MEDLINE | ID: mdl-35302838

RESUMO

This corrects the article DOI: 10.1103/PhysRevLett.127.217601.

10.
Phys Rev Lett ; 128(16): 166402, 2022 Apr 22.
Artigo em Inglês | MEDLINE | ID: mdl-35522481

RESUMO

Motivated by recent realizations of hyperbolic lattices in superconducting waveguides and electric circuits, we compute the Hofstadter butterfly on regular hyperbolic tilings. Utilizing large hyperbolic lattices with periodic boundary conditions, we obtain the true bulk spectrum unaffected by boundary states. The butterfly spectrum with large extended gapped regions prevails, and its shape is universally determined by the fundamental tile, while the fractal structure is lost. We explain how these features originate from Landau levels in hyperbolic space and can be verified experimentally.

11.
Phys Rev Lett ; 128(16): 167002, 2022 Apr 22.
Artigo em Inglês | MEDLINE | ID: mdl-35522509

RESUMO

Atomic layers deposited on semiconductor substrates introduce a platform for the realization of the extended electronic Hubbard model, where the consideration of electronic repulsion beyond the on-site term is paramount. Recently, the onset of superconductivity at 4.7 K has been reported in the hole-doped triangular lattice of tin atoms on a silicon substrate. Through renormalization group methods designed for weak and intermediate coupling, we investigate the nature of the superconducting instability in hole-doped Sn/Si(111). We find that the extended Hubbard nature of interactions is crucial to yield triplet pairing, which is f-wave (p-wave) for moderate (higher) hole doping. In light of persisting challenges to tailor triplet pairing in an electronic material, our finding promises to pave unprecedented ways for engineering unconventional triplet superconductivity.

12.
Phys Rev Lett ; 129(24): 246402, 2022 Dec 09.
Artigo em Inglês | MEDLINE | ID: mdl-36563257

RESUMO

Recently, hyperbolic lattices that tile the negatively curved hyperbolic plane emerged as a new paradigm of synthetic matter, and their energy levels were characterized by a band structure in a four- (or higher-) dimensional momentum space. To explore the uncharted topological aspects arising in hyperbolic band theory, we here introduce elementary models of hyperbolic topological band insulators: the hyperbolic Haldane model and the hyperbolic Kane-Mele model; both obtained by replacing the hexagonal cells of their Euclidean counterparts by octagons. Their nontrivial topology is revealed by computing topological invariants in both position and momentum space. The bulk-boundary correspondence is evidenced by comparing bulk and boundary density of states, by modeling propagation of edge excitations, and by their robustness against disorder.

13.
Nano Lett ; 21(15): 6398-6405, 2021 08 11.
Artigo em Inglês | MEDLINE | ID: mdl-34328737

RESUMO

Interacting bosonic particles in artificial lattices have proven to be a powerful tool for the investigation of exotic phases of matter as well as phenomena resulting from nontrivial topology. Exciton-polaritons, bosonic quasi-particles of light and matter, have been shown to combine the on-chip benefits of optical systems with strong interactions, inherited from their matter character. Technologically significant semiconductor platforms strictly require cryogenic temperatures. In this communication, we demonstrate exciton-polariton lasing for topological defects emerging from the imprinted lattice structure at room temperature. We utilize red fluorescent protein derived from DsRed of Discosoma sea anemones, hosting highly stable Frenkel excitons. Using a patterned mirror cavity, we tune the lattice potential landscape of a linear Su-Schrieffer-Heeger chain to design topological defects at domain boundaries and at the edge. We unequivocally demonstrate polariton lasing from these topological defects. This progress has paved the road to interacting boson many-body physics under ambient conditions.


Assuntos
Lasers , Fótons , Semicondutores , Temperatura
14.
Phys Rev Lett ; 127(21): 217601, 2021 Nov 19.
Artigo em Inglês | MEDLINE | ID: mdl-34860107

RESUMO

Motivated by the recent discovery of unconventional charge order, we develop a theory of electronically mediated charge density wave formation in the family of kagome metals AV_{3}Sb_{5} (A=K,Rb,Cs). The intertwining of van Hove filling and sublattice interference suggests a three-fold charge density wave instability at T_{CDW}. From there, the charge order forming below T_{CDW} can unfold into a variety of phases capable of exhibiting orbital currents and nematicity. We develop a Ginzburg Landau formalism to stake out the parameter space of kagome charge order. We find a nematic chiral charge order to be energetically preferred, which shows tentative agreement with experimental evidence.

15.
Phys Rev Lett ; 127(17): 177001, 2021 Oct 22.
Artigo em Inglês | MEDLINE | ID: mdl-34739258

RESUMO

The recent discovery of AV_{3}Sb_{5} (A=K,Rb,Cs) has uncovered an intriguing arena for exotic Fermi surface instabilities in a kagome metal. Among them, superconductivity is found in the vicinity of multiple van Hove singularities, exhibiting indications of unconventional pairing. We show that the sublattice interference mechanism is central to understanding the formation of superconductivity in a kagome metal. Starting from an appropriately chosen minimal tight-binding model with multiple van Hove singularities close to the Fermi level for AV_{3}Sb_{5}, we provide a random phase approximation analysis of superconducting instabilities. Nonlocal Coulomb repulsion, the sublattice profile of the van Hove bands, and the interaction strength turn out to be the crucial parameters to determine the preferred pairing symmetry. Implications for potentially topological surface states are discussed, along with a proposal for additional measurements to pin down the nature of superconductivity in AV_{3}Sb_{5}.

16.
Phys Rev Lett ; 126(21): 215302, 2021 May 28.
Artigo em Inglês | MEDLINE | ID: mdl-34114871

RESUMO

We employ electric circuit networks to study topological states of matter in non-Hermitian systems enriched by parity-time symmetry PT and chiral symmetry anti-PT (APT). The topological structure manifests itself in the complex admittance bands which yields excellent measurability and signal to noise ratio. We analyze the impact of PT-symmetric gain and loss on localized edge and defect states in a non-Hermitian Su-Schrieffer-Heeger (SSH) circuit. We realize all three symmetry phases of the system, including the APT-symmetric regime that occurs at large gain and loss. We measure the admittance spectrum and eigenstates for arbitrary boundary conditions, which allows us to resolve not only topological edge states, but also a novel PT-symmetric Z_{2} invariant of the bulk. We discover the distinct properties of topological edge states and defect states in the phase diagram. In the regime that is not PT symmetric, the topological defect state disappears and only reemerges when APT symmetry is reached, while the topological edge states always prevail and only experience a shift in eigenvalue. Our findings unveil a future route for topological defect engineering and tuning in non-Hermitian systems of arbitrary dimension.

17.
Nature ; 583(7816): 364-365, 2020 07.
Artigo em Inglês | MEDLINE | ID: mdl-32669691
18.
Proc Natl Acad Sci U S A ; 115(33): 8311-8315, 2018 08 14.
Artigo em Inglês | MEDLINE | ID: mdl-30061416

RESUMO

Anomalous surface states with Fermi arcs are commonly considered to be a fingerprint of Dirac semimetals (DSMs). In contrast to Weyl semimetals, however, Fermi arcs of DSMs are not topologically protected. Using first-principles calculations, we predict that ß-cuprous iodide (ß-CuI) is a peculiar DSM whose surface states form closed Fermi pockets instead of Fermi arcs. In such a fermiological Dirac semimetal, the deformation mechanism from Fermi arcs to Fermi pockets stems from a large cubic term preserving all crystal symmetries and from the small energy difference between the surface and bulk Dirac points. The cubic term in ß-CuI, usually negligible in prototypical DSMs, becomes relevant because of the particular crystal structure. As such, we establish a concrete material example manifesting the lack of topological protection for surface Fermi arcs in DSMs.

19.
Phys Rev Lett ; 122(24): 247702, 2019 Jun 21.
Artigo em Inglês | MEDLINE | ID: mdl-31322409

RESUMO

We propose an electric circuit array with topologically protected unidirectional voltage modes at its boundary. Instead of external bias fields or Floquet engineering, we employ negative impedance converters with current inversion (INICs) to accomplish a nonreciprocal, time-reversal symmetry-broken electronic network we call a topolectrical Chern circuit (TCC). The TCC features an admittance bulk gap fully tunable via the resistors used in the INICs, along with a chiral voltage boundary mode reminiscent of the Berry flux monopole present in the admittance band structure. The active circuit elements in the TCC can be calibrated to compensate for dissipative loss.

20.
Phys Rev Lett ; 122(11): 116402, 2019 Mar 22.
Artigo em Inglês | MEDLINE | ID: mdl-30951331

RESUMO

The monopnictides TaAs and TaP are well-established Weyl semimetals. Yet, a precise assignment of Fermi arcs, accommodating the predicted chiral charge of the bulk Weyl points, has been difficult in these systems, and the topological character of different surface features in the Fermi surface is not fully understood. Here, employing a joint analysis from linear dichroism in angle-resolved photoemission and first-principles calculations, we unveil the orbital texture on the full Fermi surface of TaP(001). We observe pronounced switches in the orbital texture at the projected Weyl nodes, and show how they facilitate a topological classification of the surface band structure. Our findings establish a critical role of the orbital degrees of freedom in mediating the surface-bulk connectivity in Weyl semimetals.

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