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1.
Sci Rep ; 12(1): 16596, 2022 Oct 05.
Artigo em Inglês | MEDLINE | ID: mdl-36198688

RESUMO

Multiple objectives optimization of frequency selective surface (FSS) structures is challenging in electromagnetic wave filter design. For example, one of the sub-objectives, the sidelobe level (SLL), is critical to directional anti-interference, which is complicated and becomes the bottleneck for radar design. Here, we established a dynamic algorithm for fitness function to automatically adjust the weights of multiple objectives in the optimization process of FSS structures. The dynamic algorithm could efficiently evaluate the achieving probability of sub-objectives according to the statistical analysis of the latest individual distribution so that the fitness function could automatically adjusted to focus on the sub-objective difficult to optimize, such as SLL. Computational results from the dynamic algorithm showed that the efficiency of multi-objective optimization was greatly improved by 213%, as compared to the fixed-weighted algorithm of the fitness function. Specifically for SLL, the efficiency rate increased even better, up to 315%. More interestingly, the FSS structures were most improved while picking median value or golden section value as the reference value. Taken together, the current study indicated that the dynamic algorithm with fitness function might be a better choice for FSS structural optimization with SLL suppression and potentially for the better design of lower SLL radar.

2.
Front Chem ; 8: 630687, 2020.
Artigo em Inglês | MEDLINE | ID: mdl-33791274

RESUMO

To meet the requirement of indoor R/G/B monochrome illumination a simplified OLEDs structure and fabrication process must occur. Herein, a design philosophy of low efficiency roll-off and simple-structure OLEDs incorporating R/G/B phosphorescent ultrathin non-doped emissive layers (EMLs) within non-exciplex forming interfaces a luminescent system by a direct charge trapping mechanism has been reported, which uses bis(2-methyldibenzo[f,h]-quinoxaline)(acetylacetonate)iridium(III) (MDQ)2Ir(acac), bis(3-phenylpyridin-e)iridium(III) (Ir(ppy)3), and bis(3,5-difluoro-2 -(2-pyridyl)phenyl-(2-carboxypyridyl) iridiumII) (Firpic) as R/G/B luminescent dyes, respectively. Although the recombination zone is narrow in the designed OLEDs, the efficiency roll-off of the designed OLEDs are unexpectedly slow, due to stable charge trapping of the emitters and are refrained from concentration quenching in relatively low current density, but the luminance meets the requirement of indoor lighting. With a low threshold voltage of 2.9/2.9/3.5 V, the designed R/G/B phosphorescent OLEDs show an efficiency roll-off as low as 7.6/3.2/4.3% for indoor luminance from 10 cd/m2 to 1,000 cd/m2, respectively. The perspective of R/G/B luminescent dyes on luminous efficiency, chromaticity coordinate drifts, efficiency roll-off, and direct charge trapping has been thoroughly studied. Therefore, our research may help to further develop ideal indoor lighting using a simplified undoped R/G/B OLEDs structure with simultaneous ultraslow efficiency roll-off, low threshold voltage, simplified fabrication process, low reagent consumption, and cost.

3.
ACS Appl Mater Interfaces ; 10(34): 28256-28261, 2018 Aug 29.
Artigo em Inglês | MEDLINE | ID: mdl-30117726

RESUMO

The dilute donor-fullerene bulk heterojunction (BHJ) has been proven to be an efficient architecture of organic solar cells. However, the hole-extraction pathway and the origin of the high open-circuit voltage ( VOC) in this peculiar architecture remains elusive. Direct evidence is provided here that the photogenerated holes can be extracted via the acceptor phase even under the operating conditions. Meanwhile VOC is found to be closely correlated with the surface composition at the MoO3/BHJ interface. Extending these findings into device optimization, more than 37% enhancement is achieved in a prototype BHJ device. These results evoke renewed insight into the underlying physics in organic solar cells.

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