Strong Light-Matter Interactions in Single Open Plasmonic Nanocavities at the Quantum Optics Limit.

Reaching the quantum optics limit of strong light-matter interactions between a single exciton and a plasmon mode is highly desirable, because it opens up possibilities to explore room-temperature quantum devices operating at the single-photon level. However, two challenges severely hinder the realization of this limit: the integration of single-exciton emitters with plasmonic nanostructures and making the coupling strength at the single-exciton level overcome the large damping of the plasmon mode. Here, we demonstrate that these two hindrances can be overcome by attaching individual J aggregates to single cuboid Au@Ag nanorods. In such hybrid nanosystems, both the ultrasmall mode volume of ∼71 nm^{3} and the ultrashort interaction distance of less than 0.9 nm make the coupling coefficient between a single J-aggregate exciton and the cuboid nanorod as high as ∼41.6 meV, enabling strong light-matter interactions to be achieved at the quantum optics limit in single open plasmonic nanocavities.

Vacuum Rabi splitting in a coupled system of single quantum dot and photonic crystal cavity: effect of local and propagation Green's functions.

We investigate the light emission characteristics for single two level quantum dot (QD) in a realistic photonic crystal (PC) L3 cavity based upon the local coupling strength between the QD and cavity together with the Green's function in which the propagation function related to the position of the detector is taken into account. We find for a PC cavity that the line shape of the propagation function in frequency domain is identical to that of the cavity and independent on the detector's position. We confirm that this identity is not influenced by the horizontal decay of the cavity. Furthermore, it is revealed that the vacuum fluorescence spectrum of the coupled system never give the triplet in strong coupling regime. Our work demonstrates that the experimental spectral-triplet in coupled system of single QD and PC cavity cannot be individually understood by vacuum Rabi splitting without including other physics mechanism.

Exact mobility edges in quasiperiodic systems without self-duality.

Mobility edge (ME), a critical energy separating localized and extended states in spectrum, is a central concept in understanding localization physics. However, there are few models with exact MEs, and their presences are fragile against perturbations. In the paper, we generalize the Aubry-André-Harper model proposed in (Ganeshanet al2015Phys. Rev. Lett.114146601) and recently realized in (Anet al2021Phys. Rev. Lett.126040603), by introducing a relative phase in the quasiperiodic potential. Applying Avila's global theory, we analytically compute localization lengths of all single-particle states and determine the exact expression of ME, which both significantly depend on the relative phase. They are verified by numerical simulations, and physical perception of the exact expression is also provided. We show that old exact MEs, guaranteed by the delicate self-duality which is broken by the relative phase, are special ones in a series controlled by the phase. Furthermore, we demonstrate that out of expectation, exact MEs are invariant against a shift in the quasiperiodic potential, although the shift changes the spectrum and localization properties. Finally, we show that the exact ME is related to the one in the dual model which has long-range hoppings.

Entanglement entropy of non-Hermitian free fermions.

We study the entanglement properties of non-Hermitian free fermionic models with translation symmetry using the correlation matrix technique. Our results show that the entanglement entropy has a logarithmic correction to the area law in both one-dimensional and two-dimensional systems. For any one-dimensional one-band system, we prove that each Fermi point of the system contributes exactly 1/2 to the coefficientcof the logarithmic correction. Moreover, this relation betweencand Fermi point is verified for more general one-dimensional and two-dimensional cases by numerical calculations and finite-size scaling analysis. In addition, we also study the single-particle and density-density correlation functions.

Strong anisotropic lifetime orientation distributions of a two-level quantum emitter around a plasmonic nanorod.

Spontaneous emission lifetime orientation distributions of a two-level quantum emitter in metallic nanorod structures are theoretically investigated by the rigorous electromagnetic Green function method. It was found that spontaneous emission lifetime strongly depended on the transition dipole orientation and the position of the emitter. The anisotropic factor defined as the ratio between the maximum and minimum values of the lifetimes along different dipole orientations can reach up to 10(3). It is much larger than those in dielectric structures which are only several times usually. Our results show that the localized plasmonic resonance effect provides a new degree of freedom to effectively control spontaneous emission by the dipole orientation of the quantum emitters.

Plasmon-mediated resonance energy transfer by metallic nanorods.

We investigate the enhancement of the resonance energy transfer rate between donor and acceptor associated by the surface plasmons of the Ag nanorods on a SiO2 substrate. Our results for a single nanorod with different cross sections reveal that the cylinder nanorod has the strongest ability to enhance the resonance energy transfer rate. Moreover, for donor and acceptor with nonparallel polarization directions, we propose simple V-shaped nanorod structures which lead to the remarkable resonance energy transfer enhancement that is ten times larger than that by the single nanorod structure. We demonstrate that these structures have good robustness and controllability. Our work provides a way to improve the resonance energy transfer efficiency in integrated photonic devices. PACS: 78.67.Qa, 73.20.Mf, 42.50.Ex.

Slab thickness tuning approach for solid-state strong coupling between photonic crystal slab nanocavity and a quantum dot.

The quality factor and mode volume of a nanocavity play pivotal roles in realizing the strong coupling interaction between the nanocavity mode and a quantum dot. We present an extremely simple method to obtain the mode volume and investigate the effect of the slab thickness on the quality factor and mode volume of photonic crystal slab nanocavities. We reveal that the mode volume is approximatively proportional to the slab thickness. As compared with the previous structure finely optimized by introducing displacement of the air holes, via tuning the slab thickness, the quality factor can be enhanced by about 22%, and the ratio between the coupling coefficient and the nanocavity decay rate can be enhanced by about 13%. This can remarkably enhance the capability of the photonic crystal slab nanocavity for realizing the strong coupling interaction. The slab thickness tuning approach is feasible and significant for the experimental fabrication of the solid-state nanocavities.