Compact Metasurface-Based Optical Pulse-Shaping Device.

Dispersion is present in every optical setup and is often an undesired effect, especially in nonlinear-optical experiments where ultrashort laser pulses are needed. Typically, bulky pulse compressors consisting of gratings or prisms are used to address this issue by precompensating the dispersion of the optical components. However, these devices are only able to compensate for a part of the dispersion (second-order dispersion). Here, we present a compact pulse-shaping device that uses plasmonic metasurfaces to apply an arbitrarily designed spectral phase delay allowing for a full dispersion control. Furthermore, with specific phase encodings, this device can be used to temporally reshape the incident laser pulses into more complex pulse forms such as a double pulse. We verify the performance of our device by using an SHG-FROG measurement setup together with a retrieval algorithm to extract the dispersion that our device applies to an incident laser pulse.

Broadband optical Ta2O5 antennas for directional emission of light.

Highly directive antennas with the ability of shaping radiation patterns in desired directions are essential for efficient on-chip optical communication with reduced cross talk. In this paper, we design and optimize three distinct broadband traveling-wave tantalum pentoxide antennas exhibiting highly directional characteristics. Our antennas contain a director and reflector deposited on a glass substrate, which are excited by a dipole emitter placed in the feed gap between the two elements. Full-wave simulations in conjunction with global optimization provide structures with an enhanced linear directivity as high as 119 radiating in the substrate. The high directivity is a result of the interplay between two dominant TE modes and the leaky modes present in the antenna director. Furthermore, these low-loss dielectric antennas exhibit a near-unity radiation efficiency at the operational wavelength of 780 nm and maintain a broad bandwidth. Our numerical results are in good agreement with experimental measurements from the optimized antennas fabricated using a two-step electron-beam lithography, revealing the highly directive nature of our structures. We envision that our antenna designs can be conveniently adapted to other dielectric materials and prove instrumental for inter-chip optical communications and other on-chip applications.

Nonlinear Imaging of Nanoscale Topological Corner States.

Topological states of light represent counterintuitive optical modes localized at boundaries of finite-size optical structures that originate from the properties of the bulk. Being defined by bulk properties, such boundary states are insensitive to certain types of perturbations, thus naturally enhancing robustness of photonic circuitries. Conventionally, the N-dimensional bulk modes correspond to (N - 1)-dimensional boundary states. The higher-order bulk-boundary correspondence relates N-dimensional bulk to boundary states with dimensionality reduced by more than 1. A special interest lies in miniaturization of such higher-order topological states to the nanoscale. Here, we realize nanoscale topological corner states in metasurfaces with C6-symmetric honeycomb lattices. We directly observe nanoscale topology-empowered edge and corner localizations of light and enhancement of light-matter interactions via a nonlinear imaging technique. Control of light at the nanoscale empowered by topology may facilitate miniaturization and on-chip integration of classical and quantum photonic devices.

Nonlinear Imaging with All-Dielectric Metasurfaces.

Nonlinear metasurfaces incorporate many of the functionalities of their linear counterparts such as wavefront shaping, but simultaneously they perform nonlinear optical transformations. This dual functionality leads to a rather unintuitive physical behavior which is still widely unexplored for many photonic applications. The nonlinear processes render some basic principles governing the functionality of linear metasurfaces. Exemplarily, the superposition principle and the geometric optics approximation become not directly applicable to nonlinear metasurfaces. On the other hand, nonlinear metasurfaces facilitate new phenomena that are not possible in the linear regime. Here, we study the imaging of objects through a dielectric nonlinear metalens. We illuminate objects by infrared light and record their generated images at the visible third-harmonic wavelengths. We revisit the classical lens theory and suggest a generalized Gaussian lens equation for nonlinear imaging, verified both experimentally and analytically. We also demonstrate experimentally higher-order spatial correlations facilitated by the nonlinear metalens, resulting in additional image features.

All-optical switching of a dye-doped liquid crystal plasmonic metasurface.

A switchable metasurface composed of plasmonic split ring resonators and a dye-doped liquid crystal is developed. The transmission of the metasurface in the infrared spectral range can be changed by illuminating the dye-doped liquid crystal with light in the visible spectral range. The effect is particularly efficient in the case of hybrid alignment of the liquid crystal, i. e. alignment of the director perpendicular to the surface on one substrate and parallel alignment on the counter substrate. This all-optical switching effect can be attributed to the behavior described in earlier works as colossal optical nonlinearity or surface-induced nonlinear optical effect.

Strong Nonlinear Optical Activity Induced by Lattice Surface Modes on Plasmonic Metasurface.

Optical metasurfaces, consisting of spatially variant meta-atoms, represent a new kind of optical platform for controlling the wavefront of light, with which many interesting applications, such as metalens and optical holography, have been successfully demonstrated. Further extension of the optical functionalities of metasurfaces into the nonlinear optical regime has led to unprecedented control over the local optical nonlinear generation processes. It has been shown that the nonlinear optical metasurface with achiral geometries could exhibit intrinsic optical activity in second- and third- harmonic generations. In this work, we propose an alternative approach for achieving strong nonlinear optical activity in achiral plasmonic metasurfaces by exploiting the lattice surface modes of plasmonic metasurfaces. Specifically, we theoretically and experimentally demonstrate the strong circular dichroism for second harmonic generation (SHG) on plasmonic metasurfaces consisting of split-ring resonator meta-atoms. The strong nonlinear circular dichroism is attributed to the contribution from lattice surface modes at fundamental wavelengths. Our findings may open new routes to design novel nonlinear optical devices with strong optical activity.

Nonreciprocal Asymmetric Polarization Encryption by Layered Plasmonic Metasurfaces.

As flexible optical devices that can manipulate the phase and amplitude of light, metasurfaces would clearly benefit from directional optical properties. However, single layer metasurface systems consisting of two-dimensional nanoparticle arrays exhibit only a weak spatial asymmetry perpendicular to the surface and therefore have mostly symmetric transmission features. Here, we present a metasurface design principle for nonreciprocal polarization encryption of holographic images. Our approach is based on a two-layer plasmonic metasurface design that introduces a local asymmetry and generates a bidirectional functionality with full phase and amplitude control of the transmitted light. The encoded hologram is designed to appear in a particular linear cross-polarization channel, while it is disappearing in the reverse propagation direction. Hence, layered metasurface systems can feature asymmetric transmission with full phase and amplitude control and therefore expand the design freedom in nanoscale optical devices toward asymmetric information processing and security features for anticounterfeiting applications.

Simultaneous Spectral and Spatial Modulation for Color Printing and Holography Using All-Dielectric Metasurfaces.

Metasurfaces possess the outstanding ability to tailor phase, amplitude, and even spectral responses of light with an unprecedented ultrahigh resolution and thus have attracted significant interest. Here, we propose and experimentally demonstrate a novel meta-device that integrates color printing and computer-generated holograms within a single-layer dielectric metasurface by modulating spectral and spatial responses at subwavelength scale, simultaneously. In our design, such metasurface appears as a microscopic color image under white light illumination, while encrypting two different holographic images that can be projected at the far-field when illuminated with red and green laser beams. We choose amorphous silicon dimers and nanofins as building components and use a modified parallel Gerchberg-Saxton algorithm to obtain multiple subholograms with arbitrary spatial shapes for image-indexed arrangements while avoiding the loss of phase information. Such a method can further extend the design freedom of metasurfaces. By exploiting spectral and spatial control at the level of individual pixels, multiple sets of independent information can be introduced into a single-layer device; the additional complexity and enlarged information capacity are promising for novel applications such as information security and anticounterfeiting.

Silicon Metasurfaces for Third Harmonic Geometric Phase Manipulation and Multiplexed Holography.

Nonlinear wavefront control is a crucial requirement in realizing nonlinear optical applications with metasurfaces. Numerous aspects of nonlinear frequency conversion and wavefront control have been demonstrated for plasmonic metasurfaces. However, several disadvantages limit their applicability in nonlinear nanophotonics, including high dissipative loss and low optical damage threshold. In contrast, it has been shown that metasurfaces made of high-index dielectrics can provide strong nonlinear responses. Regardless of the recent progress in nonlinear optical processes using all-dielectric nanostructures and metasurfaces, much less advancement has been made in realizing a full wavefront control directly with the generation process. Here, we demonstrate the nonlinear wavefront control for the third-harmonic generation with a silicon metasurface. We use a Pancharatnam-Berry phase approach to encode phase gradients and holographic images on nanostructured silicon metasurfaces. We experimentally demonstrate the polarization-dependent wavefront control and the reconstruction of an encoded hologram at the third-harmonic wavelength with high fidelity. Further, we show that holographic multiplexing is possible by utilizing the polarization states of the third harmonic generation. Our approach eases design and fabrication processes and paves the way to an easy to use toolbox for nonlinear optical wavefront control with all-dielectric metasurfaces.

Reconfigurable metasurface hologram by utilizing addressable dynamic pixels.

The flatness, compactness and high-capacity data storage capability make metasurfaces well-suited for holographic information recording and generation. However, most of the metasurface holograms are static, not allowing a dynamic modification of the phase profile after fabrication. Here, we propose and demonstrate a dynamic metasurface hologram by utilizing hierarchical reaction kinetics of magnesium upon a hydrogenation/dehydrogenation process. The metasurface is composed of composite gold/magnesium V-shaped nanoantennas as building blocks, leading to a reconfigurable phase profile in a hydrogen/oxygen environment. We have developed an iterative hologram algorithm based on the Fidoc method to build up a quantified phase relation, which allows the reconfigurable phase profile to reshape the reconstructed image. Such a strategy introduces actively controllable dynamic pixels through a hydrogen-regulated chemical process, showing unprecedented potentials for optical encryption, information processing and dynamic holographic image alteration.

Dynamic control of mode modulation and spatial multiplexing using hybrid metasurfaces.

Designing reconfigurable metasurfaces that can dynamically control scattered electromagnetic waves and work in the near-infrared (NIR) and optical regimes remains a challenging task, which is hindered by the static material property and fixed structures. Phase change materials (PCMs) can provide high contrast optical refractive indexes at high frequencies between amorphous and crystal states, therefore are promising as feasible materials for reconfigurable metasurfaces. Here, we propose a hybrid metasurface that can arbitrarily modulate the complex amplitude of incident light with uniform amplitude and full 2π phase coverage by utilizing composite concentric rings (CCRs) with different ratios of gold and PCMs. Our designed metasurface possesses a bi-functionality that is capable of splitting beams or generating vortex beams by thermal switching between metal and semiconductor states of vanadium oxide (VO2), respectively. It can be easily integrated into low loss photonic circuits with an ultra-small footprint. Our metadevice serves as a novel paradigm for active control of beams, which may open new opportunities for signal processing, memory storage, holography, and anti-counterfeiting.

Ultrathin Nonlinear Metasurface for Optical Image Encoding.

Security of optical information is of great importance in modern society. Many cryptography techniques based on classical and quantum optics have been widely explored in the linear optical regime. Nonlinear optical encryption in which encoding and decoding involve nonlinear frequency conversions represents a new strategy for securing optical information. Here, we demonstrate that an ultrathin nonlinear photonic metasurface, consisting of meta-atoms with 3-fold rotational symmetry, can be used to hide optical images under illumination with a fundamental wave. However, the hidden image can be read out from second harmonic generation (SHG) waves. This is achieved by controlling the destructive and constructive interferences of SHG waves from two neighboring meta-atoms. In addition, we apply this concept to obtain gray scale SHG imaging. Nonlinear metasurfaces based on space variant optical interference open new avenues for multilevel image encryption, anticounterfeiting, and background free image reconstruction.

Directional Emission from Dielectric Leaky-Wave Nanoantennas.

An important source of innovation in nanophotonics is the idea to scale down known radio wave technologies to the optical regime. One thoroughly investigated example of this approach are metallic nanoantennas which employ plasmonic resonances to couple localized emitters to selected far-field modes. While metals can be treated as perfect conductors in the microwave regime, their response becomes Drude-like at optical frequencies. Thus, plasmonic nanoantennas are inherently lossy. Moreover, their resonant nature requires precise control of the antenna geometry. A promising way to circumvent these problems is the use of broadband nanoantennas made from low-loss dielectric materials. Here, we report on highly directional emission from hybrid dielectric leaky-wave nanoantennas made of Hafnium dioxide nanostructures deposited on a glass substrate. Colloidal semiconductor quantum dots deposited in the nanoantenna feed gap serve as a local light source. The emission patterns of hybrid nanoantennas with different sizes are measured by Fourier imaging. We find for all antenna sizes a highly directional emission, underlining the broadband operation of our design.

Nonlinear Metasurface for Simultaneous Control of Spin and Orbital Angular Momentum in Second Harmonic Generation.

The spin and orbital angular momentum (SAM and OAM) of light is providing a new gateway toward high capacity and robust optical communications. While the generation of light with angular momentum is well studied in linear optics, its further integration into nonlinear optical devices will open new avenues for increasing the capacity of optical communications through additional information channels at new frequencies. However, it has been challenging to manipulate the both SAM and OAM of nonlinear signals in harmonic generation processes with conventional nonlinear materials. Here, we report the generation of spin-controlled OAM of light in harmonic generations by using ultrathin photonic metasurfaces. The spin manipulation of OAM mode of harmonic waves is experimentally verified by using second harmonic generation (SHG) from gold meta-atom with 3-fold rotational symmetry. By introducing nonlinear phase singularity into the metasurface devices, we successfully generate and measure the topological charges of spin-controlled OAM mode of SHG through an on-chip metasurface interferometer. The nonlinear photonic metasurface proposed in this work not only opens new avenues for manipulating the OAM of nonlinear optical signals but also benefits the understanding of the nonlinear spin-orbit interaction of light in nanoscale devices.

Tunable wave plate based on active plasmonic metasurfaces.

Polarization conversion is highly desired for numerous valuable applications such as remote detection and high-precision measurement. It is conventionally achieved through utilizing bulky birefringent crystals or by delicate tailored anisotropy materials. However, such schemes are not compatible with both dynamic and compact on-chip applications. We propose an active metasurface that can generate tunable ellipticity for arbitrary incident polarization with a non-volatile and reversible modulation method. The metasurface consists of V-shape plasmonic antenna arrays and an interval modulation layer made of the phase change material GST for active phase control. Our approach allows the generation of high-quality arbitrary elliptical polarization states in an ultrathin, non-mechanical, and flexible fashion, representing a significant advance compared with its conventional counterparts.

Manipulation of vector beam polarization with geometric metasurfaces.

Describing a class of beams with space-variant polarization, vector beams find many applications in both classical and quantum optics. However, simultaneous manipulation of its space-dependent polarization states is still a challenge with a single optical element. Here we demonstrate polarization modulation of a vector field by employing a plasmonic metasurface exhibiting strong and controllable optical activity. By changing the lateral phase shift between two reflective metasurface supercells, the rotation angle of a linear polarized light can be continuously tuned from zero to π with a high efficiency. As the optical activity of our metasurface devices only depends on geometrical phase, the metasurfaces can simultaneously modulate the rotation angle of a vector beam regardless of its space-variant polarization distribution. Our work provides a high efficient method in manipulating the polarization state of vector beams, especially with metasurface in a compact space, which presents great potential in research fields involving vector beams.

A graphene-based broadband optical modulator.

Integrated optical modulators with high modulation speed, small footprint and large optical bandwidth are poised to be the enabling devices for on-chip optical interconnects. Semiconductor modulators have therefore been heavily researched over the past few years. However, the device footprint of silicon-based modulators is of the order of millimetres, owing to its weak electro-optical properties. Germanium and compound semiconductors, on the other hand, face the major challenge of integration with existing silicon electronics and photonics platforms. Integrating silicon modulators with high-quality-factor optical resonators increases the modulation strength, but these devices suffer from intrinsic narrow bandwidth and require sophisticated optical design; they also have stringent fabrication requirements and limited temperature tolerances. Finding a complementary metal-oxide-semiconductor (CMOS)-compatible material with adequate modulation speed and strength has therefore become a task of not only scientific interest, but also industrial importance. Here we experimentally demonstrate a broadband, high-speed, waveguide-integrated electroabsorption modulator based on monolayer graphene. By electrically tuning the Fermi level of the graphene sheet, we demonstrate modulation of the guided light at frequencies over 1 GHz, together with a broad operation spectrum that ranges from 1.35 to 1.6 µm under ambient conditions. The high modulation efficiency of graphene results in an active device area of merely 25 µm(2), which is among the smallest to date. This graphene-based optical modulation mechanism, with combined advantages of compact footprint, low operation voltage and ultrafast modulation speed across a broad range of wavelengths, can enable novel architectures for on-chip optical communications.

Continuous control of the nonlinearity phase for harmonic generations.

The capability of locally engineering the nonlinear optical properties of media is crucial in nonlinear optics. Although poling is the most widely employed technique for achieving locally controlled nonlinearity, it leads only to a binary nonlinear state, which is equivalent to a discrete phase change of π in the nonlinear polarizability. Here, inspired by the concept of spin-rotation coupling, we experimentally demonstrate nonlinear metasurfaces with homogeneous linear optical properties but spatially varying effective nonlinear polarizability with continuously controllable phase. The continuous phase control over the local nonlinearity is demonstrated for second and third harmonic generation by using nonlinear metasurfaces consisting of nanoantennas of C3 and C4 rotational symmetries, respectively. The continuous phase engineering of the effective nonlinear polarizability enables complete control over the propagation of harmonic generation signals. Therefore, this method seamlessly combines the generation and manipulation of harmonic waves, paving the way for highly compact nonlinear nanophotonic devices.

Coupling Mediated Coherent Control of Localized Surface Plasmon Polaritons.

We investigate the phase-dependent excitation of localized surface plasmon polaritons in coupled nanorods by using nonlinear spectroscopy. Our design of a coupled three-nanorod structure allows independent excitation with cross-polarized light. Here, we show that the excitation of a particular plasmon mode can be coherently controlled by changing the relative phase of two orthogonally polarized light fields. Furthermore, we observe a phase relation for the excitation that is dominantly caused by damping effects.

Plasmon lasers at deep subwavelength scale.

Laser science has been successful in producing increasingly high-powered, faster and smaller coherent light sources. Examples of recent advances are microscopic lasers that can reach the diffraction limit, based on photonic crystals, metal-clad cavities and nanowires. However, such lasers are restricted, both in optical mode size and physical device dimension, to being larger than half the wavelength of the optical field, and it remains a key fundamental challenge to realize ultracompact lasers that can directly generate coherent optical fields at the nanometre scale, far beyond the diffraction limit. A way of addressing this issue is to make use of surface plasmons, which are capable of tightly localizing light, but so far ohmic losses at optical frequencies have inhibited the realization of truly nanometre-scale lasers based on such approaches. A recent theoretical work predicted that such losses could be significantly reduced while maintaining ultrasmall modes in a hybrid plasmonic waveguide. Here we report the experimental demonstration of nanometre-scale plasmonic lasers, generating optical modes a hundred times smaller than the diffraction limit. We realize such lasers using a hybrid plasmonic waveguide consisting of a high-gain cadmium sulphide semiconductor nanowire, separated from a silver surface by a 5-nm-thick insulating gap. Direct measurements of the emission lifetime reveal a broad-band enhancement of the nanowire's exciton spontaneous emission rate by up to six times owing to the strong mode confinement and the signature of apparently threshold-less lasing. Because plasmonic modes have no cutoff, we are able to demonstrate downscaling of the lateral dimensions of both the device and the optical mode. Plasmonic lasers thus offer the possibility of exploring extreme interactions between light and matter, opening up new avenues in the fields of active photonic circuits, bio-sensing and quantum information technology.