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1.
Environ Res ; 251(Pt 2): 118735, 2024 Jun 15.
Artigo em Inglês | MEDLINE | ID: mdl-38518905

RESUMO

Inert construction and demolition waste from Hong Kong (HK public fills) has been used for marine trial reclamation in the Guanghai Bay (GHWT) of the Chinese Mainland. However, an environmental assessment of HK public fills is necessary due to higher radioactivity in HK soils than typical global levels. Here, radiation dose rate, gamma radionuclides and gross beta of HK public fills were analyzed. The origin information was explored using natural primordial radionuclides as fingerprints. Our data show that radiation dose rate of HK public fills before disposal was 0.14-0.54 (0.33 ± 0.03) µSv/h (n = 16,722 data with 2787 ships) in 2014, which is less than the GHWT background. Monthly detection of 238U, 226Ra, 210Pb, 232Th, 228Th, 40K, and gross beta in HK public fills was conducted on three random ships. Their specific activities were <6.27-155.5, 58.7-98.7, <7.83-238.2,97.9-168.6, 87.1-136.0, 463.1-1,018, and 1047-1658 Bq/kgDW, respectively. These results suggest that the radioactivity levels of HK public fills are essentially the same as the GHWT background. The study assessed potential risks using various indices icluding Raeq (Radium equivalent activity), Hex (External radiation hazard index), Hin (Internal radiation hazard index), Iγ (Gamma index), AUI (Activity utilization index), AUI (Activity utilization index), E (Annual effective dose), AGDE (Annual gonadal dose equivalent), RLI (Representative level index), Din (Indoor air absorbed dose rate), Dout (Outdoor air absorbed dose rate), and ELCR (Excess lifetime cancer risk). The study suggests that HK public fills should be used for the trial reclamation rather than building-house materials. This provides valuable insights for the resource utilization and minimizing environmental pollution of HK public fills. The aim is to offer fundamental technical assistance for future waste resource utilization, ecological protection, and restoration in the Guangdong-Hong Kong-Macao Greater Bay Area.


Assuntos
Baías , Hong Kong , Monitoramento de Radiação/métodos , Materiais de Construção/análise
2.
Environ Res ; 250: 118467, 2024 Jun 01.
Artigo em Inglês | MEDLINE | ID: mdl-38354887

RESUMO

In the aftermath of the Fukushima Daiichi Nuclear Power Plant accident, a pioneering large-scale decontamination project was initiated, aiming to enable the return of evacuees. This project, the first of its kind in human history, involved the transportation of soils collected during decontamination to interim storage facilities. Before recycling or disposal, these soils undergo processes like volume reduction. However, there's a need for innovative methods to reduce volume effectively and treat secondary wastes more efficiently. The current study explores the impact of a dispersant, sodium hexametaphosphate (SHMP), on the behavior of radiocesium (r-Cs: 137Cs) dynamics in different size fractions of radioactively contaminated soils from Fukushima. The solid-phase speciation analysis of Fukushima soils validated that at least 50% of the 137Cs or other minerals are associated with difficult-to-extract soil phases. Nonetheless, the low 137Cs/133Cs ratio in corresponding soil phases implies a slower r-Cs fixation mechanism. The wet-sieving of r-Cs contaminated soil fraction, < 2 mm, with SHMP, resulted in different soil subfractions (2000-212, 212-53, and < 53 µm). Following SHMP treatment, dispersion of > 92% of 137Cs associated with < 212 µm soil size fractions was observed. The migration of 137Cs towards smaller soil size fractions can be attributed to either SHMP-induced cation exchange or the formation of polyvalent complexes involving SHMP and soil minerals. The condensation of 137Cs in < 212 µm, as induced by SHMP, enabled the subsequent reuse of the larger soil fraction (> 212 µm), which was less contaminated. This study provides a new perspective on the effects of dispersants and contributes to a better understanding of the complex interactions among organic carbon, 137Cs, monovalent and polyvalent cations, and soil functional groups concerning the volume reduction of soils contaminated with r-Cs.


Assuntos
Radioisótopos de Césio , Acidente Nuclear de Fukushima , Poluentes Radioativos do Solo , Radioisótopos de Césio/análise , Poluentes Radioativos do Solo/análise , Solo/química , Monitoramento de Radiação/métodos , Descontaminação/métodos , Japão
3.
Environ Res ; 260: 119524, 2024 Nov 01.
Artigo em Inglês | MEDLINE | ID: mdl-38972338

RESUMO

This review offers a detailed examination of the current landscape of radio frequency (RF) electromagnetic field (EMF) assessment tools, ranging from spectrum analyzers and broadband field meters to area monitors and custom-built devices. The discussion encompasses both standardized and non-standardized measurement protocols, shedding light on the various methods employed in this domain. Furthermore, the review highlights the prevalent use of mobile apps for characterizing 5G NR radio network data. A growing need for low-cost measurement devices is observed, commonly referred to as "sensors" or "sensor nodes", that are capable of enduring diverse environmental conditions. These sensors play a crucial role in both microenvironmental surveys and individual exposures, enabling stationary, mobile, and personal exposure assessments based on body-worn sensors, across wider geographical areas. This review revealed a notable need for cost-effective and long-lasting sensors, whether for individual exposure assessments, mobile (vehicle-integrated) measurements, or incorporation into distributed sensor networks. However, there is a lack of comprehensive information on existing custom-developed RF-EMF measurement tools, especially in terms of measuring uncertainty. Additionally, there is a need for real-time, fast-sampling solutions to understand the highly irregular temporal variations EMF distribution in next-generation networks. Given the diversity of tools and methods, a comprehensive comparison is crucial to determine the necessary statistical tools for aggregating the available measurement data.


Assuntos
Campos Eletromagnéticos , Exposição Ambiental , Ondas de Rádio , Campos Eletromagnéticos/efeitos adversos , Exposição Ambiental/análise , Humanos , Monitoramento de Radiação/métodos , Monitoramento de Radiação/instrumentação
4.
Environ Res ; 257: 119278, 2024 Sep 15.
Artigo em Inglês | MEDLINE | ID: mdl-38821459

RESUMO

This study estimated the accumulation potential of tritium, a major radionuclide released from the Fukushima Daiichi Nuclear Power Station (FDNPS), into the olive flounder as organically bound tritium (OBT) using a computer simulation model. In this estimation, two transfer pathways into the OBT were assumed: formation from tritiated water (HTO) in the tricarboxylic acid (TCA) cycle, and ingestion of OBT through the food chain (from phytoplankton, small fish, to the flounder). The food chain structure was reconstructed based on fish growth model. The OBT concentration in the flounder was estimated on three scenarios: Tritium was supplied to the flounder as only HTO in seawater (Scenario 1), as HTO in seawater and OBT formed from HTO in the small fish (Scenario 2), and as HTO in seawater and OBT accumulated in the small fish through the formation and ingestion of OBT in phytoplankton (Scenario 3). The estimated OBT concentrations in the flounder were in the following order: Scenario 3 > 2 > 1. The ratio of the estimated concentration in Scenario 1 to that in Scenario 3 reached a certain value (66 % after a year from the start of HTO exposure), indicating that the tritium transfer from the seawater into the flounder more significantly contributed to this concentration than ingestions of the small fish and the phytoplankton. Additionally, the difference between the estimations of Scenarios 1 and 2 is significantly larger than that between Scenarios 2 and 3. This suggests that phytoplankton contributed weakly to the OBT concentration in the flounder compared to the small fish.


Assuntos
Linguado , Cadeia Alimentar , Acidente Nuclear de Fukushima , Água do Mar , Trítio , Poluentes Radioativos da Água , Animais , Trítio/análise , Água do Mar/química , Poluentes Radioativos da Água/análise , Linguado/metabolismo , Japão , Monitoramento de Radiação/métodos , Fitoplâncton , Simulação por Computador
5.
J Water Health ; 22(8): 1372-1386, 2024 Aug.
Artigo em Inglês | MEDLINE | ID: mdl-39212276

RESUMO

The neutron activation of stable isotopes in environmental matrices, such as soil and groundwater, is a critical aspect of assessing the impact of radionuclide production facilities on the surrounding ecosystem. The envisioned Low-Energy Radioactive Ion Beams (LERIB) facility at the iThemba LABS, South Africa is anticipated to generate significant sources of ionising radiation. The study investigated the possible repercussions of neutron irradiation stemming from the facility, focusing on the activation of stable isotopic compositions in the environment. The investigation employed a combination of experimental and analytical techniques to characterize the neutron activation products in soil and groundwater samples collected from the vicinity. Samples were collected from designated areas for background radiological measurements and were irradiated with neutrons for a period of 1 h. The induced radioactivity measured by the High Purity Germanium detector included 24Na, 22Na, 54Mn, 52Mn, and 46Sc. The application of Darcy's law for groundwater velocity suggests that radionuclides in groundwater will migrate at an average flow velocity of 0.8 m/day. The isotopes with longer half-lives have count rates at background concentrations; therefore, environmental impacts on the site and surrounding communities might be minimal.


Assuntos
Água Subterrânea , Monitoramento de Radiação , Poluentes Radioativos da Água , Água Subterrânea/química , Água Subterrânea/análise , África do Sul , Poluentes Radioativos da Água/análise , Monitoramento de Radiação/métodos , Solo/química , Poluentes Radioativos do Solo/análise , Radioisótopos/análise , Análise de Ativação de Nêutrons , Nêutrons , Isótopos/análise
6.
Bioelectromagnetics ; 45(4): 193-199, 2024 May.
Artigo em Inglês | MEDLINE | ID: mdl-38444067

RESUMO

In Greece, 5G New Radio (NR) has started launching in the end of 2020, at the 3400-3800 MHz (FR1) frequency band. Focusing on 117 Base Stations (BSs) which were already equipped with 5G NR antennas, in situ broadband and frequency selective measurements have been conducted at minimum three points of interest, at adjacent rooftops (when accessible). The points have been selected according to the sweeping method and the electric field strength (E) value has been stored on the selected worst-case scenario point. Spectrum analysis was conducted in the FR1, for the allocated spectrum that corresponds to each mobile communication provider, in order to get preliminary results concerning the contribution of the 5G NR emissions in the general public exposure levels. The vast majority of the in situ measurements has been conducted in urban environments from the beginning of 2021 until the mid of 2022, since in Greece 5G NR services launching started from the big cities. Additionally, a 5G NR BS, installed in a suburban environment (in the city of Kalamata) is thoroughly investigated during its pilot and regular operation, based on broadband and frequency selective measurements data derived by the National Observatory of Electromagnetic Fields (NOEF) monitoring sensor network. In situ measurement data within the 5G NR frequency range are verified via the NOEF's output. The 5G NR contribution to the total E-field levels is assessed in time, from pilot to regular operation of the BS. In all cases, compliance with the reference levels for general public exposure is affirmed.


Assuntos
Campos Eletromagnéticos , Monitoramento de Radiação , Exposição Ambiental/análise , Grécia , Monitoramento de Radiação/métodos , Ondas de Rádio
7.
Bioelectromagnetics ; 45(6): 281-292, 2024 Sep.
Artigo em Inglês | MEDLINE | ID: mdl-38778514

RESUMO

Fifth generation (5G) wireless communication is being rolled out around the world. In this work, the latest radio frequency electromagnetic field (EMF) exposure measurement results on commercial 28-GHz band 5G base stations (BSs) deployed in the urban area of Tokyo, Japan, are presented. The measurements were conducted under realistic traffic conditions with a 5G smartphone and using both omnidirectional and horn antennas. First and foremost, in all cases, the electric-field (E-field) intensity is much lower (<-38 dB) than the exposure limits. The E-field intensities for traffic-off cases do not show any significant difference between the two antennas with the maximum being 3.6 dB. For traffic-on cases, the omnidirectional antenna can undesirably capture the radio wave from the smartphone in some cases, resulting in a 7-13 dB higher E-field intensity than that using the horn antenna. We also present comparative results between 4G long term evolution BSs and sub-6-GHz band and 28-GHz band 5G BSs and provide recommendations on acquiring meaningful EMF exposure data. This work is a further step toward the standardization of the measurement method regarding quasi-millimeter/millimeter wave 5G BSs.


Assuntos
Campos Eletromagnéticos , Campos Eletromagnéticos/efeitos adversos , Tóquio , Tecnologia sem Fio , Monitoramento de Radiação/métodos , Monitoramento de Radiação/instrumentação , Ondas de Rádio/efeitos adversos , Exposição Ambiental/análise , Smartphone , Humanos , Japão
8.
Radiat Environ Biophys ; 63(2): 271-281, 2024 05.
Artigo em Inglês | MEDLINE | ID: mdl-38668871

RESUMO

The most significant source of human exposure to ionizing radiation is the radioactive gas radon (basically 222Rn) and its daughter decay products, creating more than half of the effective dose from all natural sources. Radon enters buildings mainly from dense rocks, which are below building foundations at depths of 1 m and more. In this paper long-term measurements of radon flux density are analyzed, with radon exhalation from the surface of the most common rocks-loams, sandy loams, clays, clay shales, several types of sandy-gravel-pebble deposits, clay and rocky limestone. The influence of geophysical properties of rocks on radon flux density due to exhalation from surfaces of those rocks was studied. Based on the results obtained, a method of local assessment of the hazard from radon and its progeny in buildings is proposed, which is based on the geophysical properties of rocks below the foundations of those buildings.


Assuntos
Radônio , Radônio/análise , Monitoramento de Radiação/métodos , Fenômenos Geológicos
9.
Radiat Environ Biophys ; 63(3): 371-383, 2024 Aug.
Artigo em Inglês | MEDLINE | ID: mdl-38980362

RESUMO

Routine monitoring of internal exposures requires the detection of effective doses of at most 1 mSv per calendar year. For some radionuclides, this requirement cannot be satisfied by a conventional evaluation of the spectra that are gained in alpha or gamma spectrometry. However, since several measurements are conducted per calendar year on a regular basis, a combined evaluation of measurements, i.e. the evaluation of sum spectra, is possible. Additionally, radionuclides that feature several emissions of alpha or gamma radiation allow a combined evaluation of their emissions. Both methods can lead to significantly smaller detection limits as compared to a separate evaluation of spectra in many cases. However, the variation of parameters that influence the evaluation such as the measurement efficiency, abundance and chemical yield requires specific calculations and treatments of the spectra as well as a manipulation of the channel contents: In a combination of emissions, energy regions are summed and evaluated with a combined efficiency that is weighted by the abundances. In a combination of spectra, the channel contents must be scaled by the ratio of the calibration factors before the summation of the spectra. In the routine monitoring of short-lived radionuclides that feature a variety of emissions such as 225Ac, these combinations are particularly effective in reducing the detectable annual effective dose. For alpha spectrometry of 225Ac, both methods applied together can lead to a detectable effective dose of about 1 mSv per year as compared to a dose of about 90 mSv with a conventional separate evaluation.


Assuntos
Limite de Detecção , Monitoramento de Radiação , Monitoramento de Radiação/métodos , Humanos , Radioisótopos/análise , Exposição à Radiação/análise
10.
Radiat Environ Biophys ; 63(3): 357-369, 2024 Aug.
Artigo em Inglês | MEDLINE | ID: mdl-39033202

RESUMO

To assess public exposure to radon, thoron, and their progeny, measurements were conducted in 50 dwellings within the bauxite-rich area of Fongo-Tongo in western Cameroon. Passive integrating radon-thoron discriminative detectors (specifically RADUET) were employed for radon and thoron measurements. Additionally, concentrations of short-lived radon and thoron progeny were estimated using Direct Radon Progeny Sensors (DRPSs) and Direct Thoron Progeny Sensors (DTPSs) based on LR-115 detectors. The findings revealed indoor radon concentrations ranging from 31 to 123 Bq m-3 with a geometric mean (GM) of 62 Bq m-3, and indoor thoron concentrations ranging from 36 to 688 Bq m-3 with a GM of 242 Bq m-3. The Equilibrium Equivalent Radon Concentration (EERC) ranged from 3 to 86 Bq m-3 with a GM of 25 Bq m-3, while the Equilibrium Equivalent Thoron Concentration (EETC) ranged from 1.2 to 12.5 Bq m-3 with a GM of 7.6 Bq m-3. Notably, all dwellings recorded radon concentrations below 100 Bq m-3. Arithmetic means of radon and thoron equilibrium factors were calculated as 0.47 and 0.04, respectively. To assess annual effective doses from radon and thoron inhalation, equilibrium factors were used along with direct measurements of EERC and EETC. The differences observed in annual effective doses were 4.5% for radon and 42.5% for thoron. Furthermore, the contribution of thoron and its decay products to the annual effective dose from radon, thoron, and their progeny ranged from 12 to 94%, with an average contribution of 58%. Thus, this study found that the effective dose due to thoron inhalation in the study area exceeded that due to radon inhalation. It is concluded that, when evaluating radiation doses and health risks, it is crucial to consider both thoron and its progeny alongside radon and its progeny. This underscores the importance of considering direct measurements for accurately estimating radiation doses.


Assuntos
Poluentes Radioativos do Ar , Poluição do Ar em Ambientes Fechados , Doses de Radiação , Monitoramento de Radiação , Produtos de Decaimento de Radônio , Radônio , Radônio/análise , Camarões , Poluentes Radioativos do Ar/análise , Poluição do Ar em Ambientes Fechados/análise , Produtos de Decaimento de Radônio/análise , Monitoramento de Radiação/métodos , Humanos , Habitação
11.
Radiat Environ Biophys ; 63(3): 385-394, 2024 Aug.
Artigo em Inglês | MEDLINE | ID: mdl-39031187

RESUMO

Monitoring of internal exposure to short-lived alpha-emitting radionuclides such as actinium-225 (225Ac), which are becoming increasingly important in nuclear medicine, plays an important role in the radiation protection of occupationally exposed persons. After having tested gamma spectrometry, liquid scintillation counting and alpha spectrometry for monitoring of internal exposure, the focus of the present study was on solid phase extraction of 225Ac from urine in combination with alpha spectrometry. The development of the method was based on recent findings from the literature on this topic. The method was used in a pilot phase to monitor internal exposure of four workers who were directly or indirectly involved in the manufacture and/or use of 225Ac. The monitoring protocol allowed a relatively short 24-hour urine sample analysis with excellent recovery of the internal standard, but it did not allow for a detection limit of less than 1 mBq nor a sufficient yield of 225Ac. Based on these results it is concluded that an in vitro excretion analysis alone is not appropriate for monitoring internal exposure to 225Ac. Instead, different radiation monitoring techniques have to be combined to ensure the radiation protection of employees.


Assuntos
Actínio , Partículas alfa , Exposição Ocupacional , Monitoramento de Radiação , Exposição Ocupacional/análise , Humanos , Monitoramento de Radiação/métodos , Medicina Nuclear , Radioisótopos/urina , Masculino , Extração em Fase Sólida , Proteção Radiológica , Exposição à Radiação , Doses de Radiação , Adulto
12.
Sensors (Basel) ; 24(10)2024 May 07.
Artigo em Inglês | MEDLINE | ID: mdl-38793821

RESUMO

Radon is a naturally occurring noble radioactive gas that poses significant health risks, particularly lung cancer, due to its colorless, odorless, and tasteless nature, which makes detection challenging without formal testing. It is found in soil, rock, and water, and it infiltrates indoor environments, necessitating regulatory standards and guidelines from organizations such as the Environmental Protection Agency, the World Health Organization, and the Occupational Health and Safety Agency to mitigate exposure. In this paper, we present various methods and instruments for radon assessment in occupational and environmental settings. Discussion on long- and short-term monitoring, including grab sampling, radon dosimetry, and continuous real-time monitoring, is provided. The comparative analysis of detection techniques-active versus passive-is highlighted from real-time data and long-term exposure assessment, including advances in sensor technology, data processing, and public awareness, to improve radon exposure evaluation techniques.


Assuntos
Exposição Ocupacional , Radônio , Radônio/análise , Humanos , Exposição Ocupacional/análise , Exposição Ocupacional/prevenção & controle , Monitoramento de Radiação/métodos , Monitoramento de Radiação/instrumentação , Poluição do Ar em Ambientes Fechados/análise , Poluentes Radioativos do Ar/análise , Exposição Ambiental/análise
13.
Environ Geochem Health ; 46(8): 297, 2024 Jul 09.
Artigo em Inglês | MEDLINE | ID: mdl-38980451

RESUMO

The radiological characterization of soil contaminated with natural radionuclides enables the classification of the area under investigation, the optimization of laboratory measurements, and informed decision-making on potential site remediation. Neural networks (NN) are emerging as a new candidate for performing these tasks as an alternative to conventional geostatistical tools such as Co-Kriging. This study demonstrates the implementation of a NN for estimating radiological values such as ambient dose equivalent (H*(10)), surface activity and activity concentrations of natural radionuclides present in a waste dump of a Cu mine with a high level of natural radionuclides. The results obtained using a NN were compared with those estimated by Co-Kriging. Both models reproduced field measurements equivalently as a function of spatial coordinates. Similarly, the deviations from the reference concentration values obtained in the output layer of the NN were smaller than the deviations obtained from the multiple regression analysis (MRA), as indicated by the results of the root mean square error. Finally, the method validation showed that the estimation of radiological parameters based on their spatial coordinates faithfully reproduced the affected area. The estimation of the activity concentrations was less accurate for both the NN and MRA; however, both methods gave statistically comparable results for activity concentrations obtained by gamma spectrometry (Student's t-test and Fisher's F-test).


Assuntos
Cobre , Mineração , Redes Neurais de Computação , Monitoramento de Radiação , Poluentes Radioativos do Solo , Cobre/análise , Poluentes Radioativos do Solo/análise , Monitoramento de Radiação/métodos , Análise de Regressão
14.
Environ Geochem Health ; 46(9): 337, 2024 Jul 29.
Artigo em Inglês | MEDLINE | ID: mdl-39073619

RESUMO

The first verification of a tool developed to improve the work of controlling bodies, managers and employees of underground facilities subject to radiation protection requirements was conducted. The recommended values of correction factors were verified using archival results of measurements conducted for the Institute of Occupational Medicine in Lódz in seven underground workplaces in Poland over exposure periods of a month (10,8678 data) and a quarter of a year (53,688 data). In a cave two groups of monthly factors, produced estimates with almost 70% to 99% consistency with the measured values. Along tourist routes located in mines, a similar fit was obtained using three groups of correction factors for measurement results from March, June and July. In the extraction areas of active underground mines, the best fit was produced by factors calculated as averages for spaces varying in the degree of insulation and ventilation method, while in other departments of mining plants, by correction factors recommended for facilities equipped with mechanical ventilation systems. All the quarterly correction factors produced the best fit between estimated mean annual concentrations and measurement results obtained in the second quarter of the calendar year. A wide variation in result consistency (from 20-30 to 65-80%) obtained for two underground tourist routes in the fourth quarter of the year demonstrates that it is best not to adopt results from this measurement period (October-December) for estimating mean annual radon concentration using the set of quarterly correction factors.


Assuntos
Poluentes Radioativos do Ar , Exposição Ocupacional , Monitoramento de Radiação , Radônio , Radônio/análise , Polônia , Monitoramento de Radiação/métodos , Exposição Ocupacional/análise , Poluentes Radioativos do Ar/análise , Mineração , Humanos , Proteção Radiológica/métodos , Local de Trabalho
15.
Environ Geochem Health ; 46(6): 181, 2024 May 02.
Artigo em Inglês | MEDLINE | ID: mdl-38695964

RESUMO

This study determined natural and artificial radionuclide concentrations to evaluate natural radioactivity and health risk levels of nine travertines in the Yaprakhisar and Balkayasi regions in Turkey. The samples coded B1-M, B2, B5, B7, B8, and B10 represent waste derived from the Yaprakhisar travertines, as well as samples T5-M, T12, and Z1 travertines derived from Balkayasi. The levels of natural and artificial radionuclide concentrations (232Th, 40K, and 137Cs) were measured using a high-purity germanium (HpGe) detector system. The travertine activity ranged from 2.09 to 12.07 Bq kg-1 for 232Th, 4.21 to 13.41 Bq kg-1 for 40K, and 0.42-3.26 Bq kg-1 for 137Cs. The results showed that the activity concentration values for 232Th, 40K, and 137Cs were coherent with the travertine analysis results in the UNSCEAR, 2000; 2008 publications. The values obtained were lower than the average values in the UNSEAR reports. The radiological hazard parameters calculated in this study were absorbed gamma dose rate (D), radium equivalent activity (Raeq), annual gonadal dose equivalent (AGDE), exposure dose (ER), total annual effective dose (AEDEtotal), excess lifetime cancer risk (ELCRtotal), gamma representative level (GRL), internal hazard index (Hin) and external hazard index (Hex).


Assuntos
Radioisótopos de Césio , Radioisótopos de Potássio , Monitoramento de Radiação , Turquia , Monitoramento de Radiação/métodos , Radioisótopos de Potássio/análise , Radioisótopos de Césio/análise , Tório/análise , Poluentes Radioativos do Solo/análise , Radiação de Fundo , Humanos , Medição de Risco
16.
Environ Geochem Health ; 46(10): 412, 2024 Sep 04.
Artigo em Inglês | MEDLINE | ID: mdl-39230594

RESUMO

This paper presents findings on groundwater physiochemical composition and radioactivity levels in households in Bac Lieu province, Vietnam. Through discriminant analysis, it was observed that groundwater quality exhibits spatial variations corresponding to saline intrusion zones. The paired-samples T-tests revealed significantly different ratios of Ra-224, Ra-226, and Ra-228 isotopes between Na-Cl and Ca-Na-HCO3 water types. All three water types had a ratio of Ra-226/Ra-228 of approximately one, indicating the presence of groundwater aquifers beneath the crust and fluvial marine sediment. Furthermore, strong associations between sulfate and calcium suggest that CO2 enrichment in groundwater aquifers indicates anoxic aquatic environments. Twenty-five of the thirty-three evaluated samples exceeded the national technical regulations for domestic water quality with parameters such as chloride, sulfate, sodium, gross alpha, or total dissolved solids. Fifteen samples exceeded gross alpha's allowable contamination threshold of 0.1 Bq/L. The combination of Ra-226 and Ra-228 did not surpass the U.S. Environmental Protection Agency's recommended limit of 0.185 Bq/L. However, nineteen samples exhibited annual committed effective doses of radium isotopes for infants that exceeded the WHO recommendation of 0.1 mSv/year.


Assuntos
Água Subterrânea , Rádio (Elemento) , Poluentes Radioativos da Água , Vietnã , Água Subterrânea/química , Poluentes Radioativos da Água/análise , Humanos , Rádio (Elemento)/análise , Monitoramento de Radiação/métodos , Características da Família , Sulfatos/análise
17.
Environ Geochem Health ; 46(9): 355, 2024 Jul 31.
Artigo em Inglês | MEDLINE | ID: mdl-39083074

RESUMO

The inherent radioactivity of radon gas presents potential exposure risks to human beings through ingestion and inhalation of its radioisotopes 222Rn (radon) and 220Rn (thoron) from water sources. Recent studies have been conducted to assess radon concentrations in different environmental matrices such as water, air, and soil, due to their detrimental impact on human health. As the main cause of lung cancer in non-smokers and an acknowledged contributor to stomach cancer when ingested, the present study aimed to preliminarily assess radon and thoron levels in the Uranium bearing area of Poli in the Faro division of Cameroon, known for its significant U-deposits. The assessment included measuring 220, 222Rn concentrations in drinking water, emanation, and exhalation, with a specific focus on evaluating the exposure of different age groups within the local population. The radon/thoron levels in water and their related exposure and cancer risk data indicated no immediate health hazards. However, continuous monitoring and prospective measures are deemed essential due to the area's abundant U-minerals. The emanation measurements showed sparsely distributed data with a singularity at Salaki, where the equipment recorded values of 8.14 × 1012 Bqm-3 and 3.27 × 1012 Bqm-3 for radon and thoron, respectively. Moreover, radon/thoron transfer coefficients from the soil to the air indicated levels below unity. While the calculated doses suggest minimum potential risk in line with WHO and UNSCEAR guidelines, the obtained results are expected to significantly contribute to the establishment of national standards for radon levels in drinking water, emanation, and exhalation. Furthermore, these findings can play a crucial role in monitoring radon/thoron levels to ensure public health safety.


Assuntos
Água Potável , Radônio , Poluentes Radioativos da Água , Radônio/análise , Água Potável/química , Camarões , Humanos , Poluentes Radioativos da Água/análise , Monitoramento de Radiação/métodos , Urânio/análise , Adulto , Adolescente , Criança , Pessoa de Meia-Idade , Adulto Jovem , Pré-Escolar , Masculino , Expiração , Feminino , Lactente , Medição de Risco
18.
J Radiol Prot ; 44(1)2024 Mar 28.
Artigo em Inglês | MEDLINE | ID: mdl-38507784

RESUMO

In Korea, decommissioning of nuclear power plants and transportation of the decommissioning waste are expected to expand in the near future. It is necessary to confirm that radiological risks to the public and workers are not significant through radiological safety assessment. The objective of this study is to assess the radiological safety for transportation of RPV waste, which is a major decommissioning waste with relatively high level of radioactivity. It was assumed that the waste would be transported to the Gyeongju disposal facility by land transportation. First, the source term and transportation method of the RPV waste were determined, and the external dose rates from the waste were calculated using MCNP. Then, transportation scenarios were assumed under both normal and accident conditions. Under the scenarios, radiation doses were calculated using the RADTRAN. Under normal operation scenarios without a transportation accident, assuming 40 shipments per year, the average individual doses for the public ranged from 6.56×10-6to 2.18×10-2mSv yr-1. The maximum individual doses for only a single shipment ranged from 2.43×10-6to 3.14×10-1mSv. For cargo handlers and vehicle crew members, the average doses were 2.26×101mSv yr-1and 2.95 mSv yr-1, respectively. Under transportation accident scenarios, average individual radiological risks which are product of the radiation doses and the annual accident rates ranged from 1.14×10-11to 1.61×10-10mSv yr-1by transportation route segment when considering the transportation accident rate. Average individual doses assuming transportation accident occurrence ranged from 2.62×10-4to 1.42×10-3mSv. The maximum individual dose under accident conditions was 7.99×10-2mSv. The calculated doses were below the regulatory limits in Korea. However, relatively high doses were observed for cargo handlers and vehicle crew members because of conservative assumptions. This study results can be used as basic data for the radiological safety assessment for the decommissioning waste transportation in the future.


Assuntos
Acidente Nuclear de Fukushima , Monitoramento de Radiação , Humanos , Centrais Nucleares , Doses de Radiação , Monitoramento de Radiação/métodos , República da Coreia
19.
J Radiol Prot ; 44(3)2024 Jul 26.
Artigo em Inglês | MEDLINE | ID: mdl-39019049

RESUMO

This paper presents a proposed revision of the International Atomic Energy Agency transport regulations, related to theA1andA2limit values used to determine the radioactive transport classification. Based on the 'Qsystem', a novel methodology was introduced to deriveQAandQBvalues related to scenarios involving external exposure from a distant source. These values are key parameters that respectively represent the total effective dose and total equivalent dose to the skin, from all primary and secondary particles contributing to radiation exposure. The International Working Group (WGA1/A2) is established and associated with the TRANSSC Technical Expert Group on Radiation Protection. A review of theA1andA2values is performed in response to identified limitations within the existingQsystem. The followed approach is based on Monte Carlo simulations that enabled the development of transfer functions aimed at reducing computational time and increasing the flexibility of dose evaluations for any radionuclide with known particle emission spectra. This method allows updating theQAandQBvalues to account for future data evolutions (decay data, fluence-to-dose conversion coefficients) and standardizing the calculation of regulation limits across all referenced radionuclides and scenarios related to external exposure. The transfer functions are established using three Monte Carlo simulation codes-FLUKA, Geant4, and MCNP-and address the previous limitations of the 'Qsystem', reflecting the latest International Commission for Radiation Protection recommendations and improvements in calculation techniques. The results of the WG show consistent agreement across the codes, with minor discrepancies observed at low primary energies due to statistical uncertainties and different handling of stopping power for electrons/positrons in the codes. This revised approach aligns with current standards and recommendations, ensuring that the radiological consequences of transport accidents are acceptable for the newA1andA2limits from a radiological protection perspective.


Assuntos
Método de Monte Carlo , Proteção Radiológica , Proteção Radiológica/normas , Humanos , Doses de Radiação , Meios de Transporte , Agências Internacionais , Monitoramento de Radiação/métodos , Simulação por Computador
20.
J Radiol Prot ; 44(3)2024 Aug 07.
Artigo em Inglês | MEDLINE | ID: mdl-38964307

RESUMO

The accident at Fukushima Daiichi Nuclear Power Plant (FDNPP) in 2011 resulted in the dispersion of radioactive materials throughout the surrounding area and an increase in the air dose rate was even confirmed in Fukushima City, which is located approximately 60 km northeast of FDNPP. A Tokyo Electric Power Company (TEPCO) Holdings employee, who has lived and worked in Fukushima City since the FDNPP accident, measured individual external doses, GPS data, and his activities in Fukushima Prefecture over a 9 year period beginning in 2014. This data provides valuable information about the area. The data show the following results. (i) Comparison of the air dose rate at the home location to the individual external dose per hour at the home shows that the average conversion factor has increased over the 9 years and exceeded 0.3 since 2019, indicating an overall relatively good correlation. (ii) Individual external doses measured in the office on the fourth floor of a concrete structure in Fukushima City have not changed significantly from 2014 to 2022, when air dose rates showed a decrease. (iii) Outdoor individual external doses, such as those measured when commuting on foot, have a relatively strong correlation with air dose rates from airborne monitoring with the conversion factor of about 0.6. The conversion factor do not differ significantly from 2014 to 2022.In this study, the individual external dose data is applicable to the TEPCO measurer and is not necessarily representative of all residents of Fukushima City. However individual external dose data for 9 consecutive years will be useful for estimating individual external doses from air dose rates, and estimating annual additional exposure doses, if even some of them are applicable to similar life patterns and lifestyles.


Assuntos
Poluentes Radioativos do Ar , Acidente Nuclear de Fukushima , Exposição Ocupacional , Doses de Radiação , Monitoramento de Radiação , Humanos , Monitoramento de Radiação/métodos , Poluentes Radioativos do Ar/análise , Exposição Ocupacional/análise , Japão , Centrais Nucleares
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