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1.
Phys Rev Lett ; 128(7): 075001, 2022 Feb 18.
Artículo en Inglés | MEDLINE | ID: mdl-35244411

RESUMEN

A new method for measuring the time-dependent drive flux at the hohlraum center is proposed as a better alternative to conventional wall-based techniques. The drive flux here is obtained by simultaneous measurement of the reemitted flux and shock velocity from a three-layered "cakelike" sample. With these two independent observables, the influence induced by the uncertainty of the material parameters of the sample can be effectively decreased. The influence from the closure of the laser entrance hole, which was the main challenge in conventional wall-based techniques, was avoided through localized reemitted flux measurement, facilitating drive flux measurement throughout the entire time history. These studies pave a new way for probing the time-dependent drive flux, for both cylindrical hohlraums and novel hohlraums with six laser entrance holes.

2.
J Synchrotron Radiat ; 27(Pt 2): 436-445, 2020 Mar 01.
Artículo en Inglés | MEDLINE | ID: mdl-32153282

RESUMEN

A systematic investigation on the theoretical framework of the ultra-fast measurement of temperature by extended X-ray absorption fine structure (EXAFS) applied in laser-driven-compression experiments has been carried out and a new temperature measurement scheme based on the EXAFS cumulant expansion analysis and anharmonic correlated Debye model has been advanced. By considering the anharmonic effect of thermal vibration and avoiding the employment of the empirical model as well as parameters which have large inherent uncertainties in the temperature determination, this new scheme is theoretically more accurate than traditional ones. Then the performance of the new measurement scheme and traditional methods were validated on a synchrotron radiation platform by temperature-dependent EXAFS (TDEXAFS) experiments on Au, Fe, V and Ti; the results showed that the new scheme could provide the most accurate measured temperatures with much lower uncertainties. This accurate scheme gives a firmer physical ground to the EXAFS temperature measurement technique and can expect to be applied in laser-driven compression experiments and promote the development of matter state research at extreme conditions.

3.
Phys Chem Chem Phys ; 17(6): 4089-95, 2015 Feb 14.
Artículo en Inglés | MEDLINE | ID: mdl-25560204

RESUMEN

We perform detailed first principles calculations of the structural parameters at zero pressure and high pressure, the elastic properties, phonon dispersion relation, and ideal strengths of U2Mo with the C11b structure. In contrast to previous theoretical studies, we show that the I4/mmm structure is indeed a mechanically and dynamically unstable phase, which is confirmed by the negative elastic constant C66 as well as the imaginary phonon modes observed along the Σ1-N-P line. The calculations of ideal strengths for U2Mo are performed along the [100], [001], and [110] directions for tension and on (001)[010] and (010)[100] slip systems for shear load. The ideal shear strength is about 8.1 GPa, much smaller than a tension of 18-28 GPa, which indicates that the ductile U2Mo alloy will fail by shear rather than by tension.

4.
Chemosphere ; 337: 139057, 2023 Oct.
Artículo en Inglés | MEDLINE | ID: mdl-37268234

RESUMEN

Advanced oxidation processes (AOPs) using strongly oxidizing radicals are promising for wastewater treatment and gas purification. Nevertheless, the short half-life of radicals and the limited mass transfer in traditional reactors cause under-utilization of radicals and low pollutant removal efficiency. High-gravity technology (HiGee)-enhanced AOPs (HiGee-AOPs) have been demonstrated a promising way to enhance radical utilization in a rotating packed bed reactor (RPB). Here, we review the potential mechanisms of intensified radical utilization in HiGee-AOPs, structures and performance of RPB, and applications of HiGee in AOPs. The intensification mechanisms are described from three aspects: enhanced generation of radicals by efficient mass transfer, in-situ radical utilization under frequent liquid film renewal, and selective effect on radical utilization due to micromixing in RPB. Based on these mechanisms, we propose a novel High-gravity flow reaction with the essence of efficiency, in-situ, and selectivity in order to better explain the strengthening mechanisms in HiGee-AOPs. HiGee-AOPs possess great potential for treating effluent and gaseous pollutants due to characteristics of High-gravity flow reaction. We discuss the pros and cons of different RPBs and their applications to specific HiGee-AOPs. HiGee improve the following AOPs: (1) facilitate interfacial mass transfer in homogeneous AOPs, (2) enhance mass transfer to expose more catalytically active sites and mass-produce nanocatalysts for heterogeneous AOPs, (3) inhibit bubble accumulation on the electrode surface of electrochemical AOPs, (4) increase the mass transfer between liquid and catalysts in UV-assisted AOPs, (5) improve the micromixing efficiency of ultrasound-based AOPs. Strategies outlined in this paper should inspire further development of HiGee-AOPs.


Asunto(s)
Contaminantes Ambientales , Contaminantes Químicos del Agua , Purificación del Agua , Gases , Oxidación-Reducción , Radicales Libres , Radical Hidroxilo/química , Contaminantes Químicos del Agua/análisis
5.
Phys Rev E Stat Nonlin Soft Matter Phys ; 80(1 Pt 2): 016202, 2009 Jul.
Artículo en Inglés | MEDLINE | ID: mdl-19658787

RESUMEN

In this paper, we report the experimental results on the characteristics of plasma patterns with different planar electrode shapes in dielectric barrier glow discharge. The formation and the evolution of the discharge patterns at different voltages were investigated. The results show that the plasma patterns in this glow-barrier system form at the beginning of the discharge pulse. The limited size of planar electrodes and the electric field distribution are important factors for the pattern formation.

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