Certification of Genuine Multipartite Entanglement with General and Robust Device-Independent Witnesses.

Genuine multipartite entanglement represents the strongest type of entanglement, which is an essential resource for quantum information processing. Standard methods to detect genuine multipartite entanglement, e.g., entanglement witnesses, state tomography, or quantum state verification, require full knowledge of the Hilbert space dimension and precise calibration of measurement devices, which are usually difficult to acquire in an experiment. The most radical way to overcome these problems is to detect entanglement solely based on the Bell-like correlations of measurement outcomes collected in the experiment, namely, device independently. However, it is difficult to certify genuine entanglement of practical multipartite states in this way, and even more difficult to quantify it, due to the difficulty in identifying optimal multipartite Bell inequalities and protocols tolerant to state impurity. In this Letter, we explore a general and robust device-independent method that can be applied to various realistic multipartite quantum states in arbitrary finite dimension, while merely relying on bipartite Bell inequalities. Our method allows us both to certify the presence of genuine multipartite entanglement and to quantify it. Several important classes of entangled states are tested with this method, leading to the detection of genuinely entangled states. We also certify genuine multipartite entanglement in weakly entangled Greenberger-Horne-Zeilinger states, showing that the method applies equally well to less standard states.

Experimental optimal generation of hybrid entangled states in photonic quantum walks.

While the existence of disorders is commonly believed to weaken the unique properties of quantum systems, recent progress has predicted that it can exhibit a counterintuitive enhanced effect on the behavior of entanglement generation, which is even independent of the chosen initial conditions and physical platforms. However, to achieve a maximally entangled state in such disordered quantum systems, the key limitation of this is the scarcity of an infinite coherence time, which makes its experimental realization challenging. Here, we experimentally investigate the entanglement entropy dynamics in a photonic quantum walk with disorders in time. Through the incorporation of a classic optimization algorithm, we experimentally demonstrate that such disordered systems can relax to a high-entanglement hybrid state at any given time step. Moreover, this prominent entangling ability is universal for a wide variety of initial conditions. Our results may inspire achieving a well-controlled entanglement generator for quantum computation and information tasks.

Experimental extraction of nonlocal weak values for demonstrating the failure of a product rule.

We experimentally demonstrate an alternative method for measuring nonlocal weak values in linear optics, avoiding the use of second-order interaction. The method is based on the concept of modular values. The paths of two photons, initialized in hyperentangled states, are adopted as the meter with the polarization acting as the system. The modular values are read out through the reconstructed final states of the meter. The weak value of nonlocal observables is given through its connection to the modular value. Comparing the weak values of local and nonlocal observables, we demonstrate the failure of product rules for an entangled system. Our results significantly simplify the task of measuring nonlocal weak values and will play an important role in the application of weak measurement.

Experimental Optimal Verification of Entangled States Using Local Measurements.

The initialization of a quantum system into a certain state is a crucial aspect of quantum information science. While a variety of measurement strategies have been developed to characterize how well the system is initialized, for a given one, there is in general a trade-off between its efficiency and the accessible information of the quantum state. Conventional quantum state tomography can characterize unknown states while requiring exponentially expensive time-consuming postprocessing. Alternatively, recent theoretical breakthroughs show that quantum state verification provides a technique to quantify the prepared state with significantly fewer samples, especially for multipartite entangled states. In this Letter, we modify the original proposal to be robust to practical imperfections, and experimentally implement a scalable quantum state verification on two-qubit and four-qubit entangled states with nonadaptive local measurements. For all the tested states, the estimated infidelity is inversely proportional to the number of samples, which illustrates the power to characterize a quantum state with a small number of samples. Compared to the globally optimal strategy which requires nonlocal measurements, the efficiency in our experiment is only worse by a small constant factor (<2.5). We compare the performance difference between quantum state verification and quantum state tomography in an experiment to characterize a four-photon Greenberger-Horne-Zeilinger state, and the results indicate the advantage of quantum state verification in both the achieved efficiency and precision.

Experimental Investigation of Quantum PT-Enhanced Sensor.

PT-symmetric theory is developed to extend quantum mechanics to a complex region, but it wins its great success first in classical systems, for example, optical waveguides and electric circuits, etc., because there are so many counterintuitive phenomena and striking applications, including unidirectional light transport, PT-enhanced sensors (one kind of exceptional-point-based sensor), and wireless power transfer. However, these phenomena and applications are mostly based on the ability to approach a PT-symmetric broken region, which makes it difficult to transfer them to the quantum regime, since the broken quantum PT-symmetric system has not been constructed effectively, until recently several methods have been raised. Here, we construct a quantum PT-symmetric system assisted by weak measurement, which can effectively transit from the unbroken region to the broken region. The full energy spectrum including the real and imaginary parts is directly measured using weak values. Furthermore, based on the ability of approaching a broken region, we for the first time translate the previously mentioned PT-enhanced sensor into the quantum version, and investigate its various features that are associated to the optimal conditions for sensitivity enhancement. In this experiment, we obtain an enhancement of 8.856 times over the conventional Hermitian sensor. Moreover, by separately detecting the real and imaginary parts of energy splitting, we can derive the additional information of the direction of perturbations. Our work paves the way of leading classical interesting PT phenomena and applications to their quantum counterparts. More generally, since the PT system is a subset of non-Hermitian systems, our work will be also helpful in the studies of general exception point in the quantum regime.

Direct Measurement of a Nonlocal Entangled Quantum State.

Entanglement and the wave function description are two of the core concepts that make quantum mechanics such a unique theory. A method to directly measure the wave function, using weak values, was demonstrated by Lundeen et al. [Nature 474, 188 (2011)]. However, it is not applicable to a scenario of two disjoint systems, where nonlocal entanglement can be a crucial element, since that requires obtaining weak values of nonlocal observables. Here, for the first time, we propose a method to directly measure a nonlocal wave function of a bipartite system, using modular values. The method is experimentally implemented for a photon pair in a hyperentangled state, i.e., entangled both in polarization and momentum degrees of freedom.

Measurements of Nonlocal Variables and Demonstration of the Failure of the Product Rule for a Pre- and Postselected Pair of Photons.

We report the first implementation of the von Neumann instantaneous measurements of nonlocal variables, which becomes possible due to technological achievements in creating hyperentangled photons. Tests of reliability and of the nondemolition property of the measurements have been performed with high precision, showing the suitability of the scheme as a basic ingredient of numerous quantum information protocols. The method allows us to demonstrate for the first time with strong measurements a special feature of pre- and postselected quantum systems: the failure of the product rule. It has been verified experimentally that for a particular pre- and postselected pair of particles, a single measurement on particle A yields with certainty σ_{x}^{A}=-1, a single measurement on particle B yields with certainty σ_{y}^{B}=-1, and a single nonlocal measurement on particles A and B yields with certainty σ_{x}^{A}σ_{y}^{B}=-1.

Measuring the Winding Number in a Large-Scale Chiral Quantum Walk.

We report the experimental measurement of the winding number in an unitary chiral quantum walk. Fundamentally, the spin-orbit coupling in discrete time quantum walks is implemented via a birefringent crystal collinearly cut based on a time-multiplexing scheme. Our protocol is compact and avoids extra loss, making it suitable for realizing genuine single-photon quantum walks at a large scale. By adopting a heralded single photon as the walker and with a high time resolution technology in single-photon detection, we carry out a 50-step Hadamard discrete-time quantum walk with high fidelity up to 0.948±0.007. Particularly, we can reconstruct the complete wave function of the walker that starts the walk in a single lattice site through the local tomography of each site. Through a Fourier transform, the wave function in quasimomentum space can be obtained. With this ability, we propose and report a method to reconstruct the eigenvectors of the system Hamiltonian in quasimomentum space and directly read out the winding numbers in different topological phases (trivial and nontrivial) in the presence of chiral symmetry. By introducing nonequivalent time frames, we show that whole topological phases in a periodically driven system can also be characterized by two different winding numbers. Our method can also be extended to the high winding number situation.

Experimental demonstration of efficient quantum state tomography of matrix product states.

Quantum state tomography is a key technology for fully determining a quantum state. Unfortunately, standard quantum state tomography is intractable for general many-body quantum states, because the number of measurements and the post-processing time increase exponentially with the size of the system. However, for the matrix product states (MPSs), there exists an efficient method using linearly scaled local measurements and polynomially scaled post-processing times. In this study, we demonstrate the validity of the method in practice by reconstructing a four-photon MPS from its local two- or three-photon reduced-density matrices with the presence of statistical errors and systematical errors in experiment.

Measurement of the inhomogeneous broadening of a bi-exciton state in a quantum dot using Franson-type nonlocal interference.

The inhomogeneous broadening of the bi-exciton state in quantum dots, i.e., the inhomogeneous broadening of the upper level of the cascade process, is not only a fundamental problem in quantum dots, but also closely related with the coherent control of this complex system and the quality of the entangled photon pairs, especially the time-bin entangled photon pairs. This inhomogeneous broadening is inherently a two-photon correlated phenomenon. In this work, we construct a genuine Franson-type nonlocal interference process to measure the inhomogeneous broadening of the bi-exciton state. The results show that the inhomogeneous broadening of the bi-exciton state is considerably smaller than that of the exciton state, that is why the entangled photon pairs can be generated by the cascade process in the quantum dot.

Experimental Test of Compatibility-Loophole-Free Contextuality with Spatially Separated Entangled Qutrits.

The physical impact and the testability of the Kochen-Specker (KS) theorem is debated because of the fact that perfect compatibility in a single quantum system cannot be achieved in practical experiments with finite precision. Here, we follow the proposal of A. Cabello and M. T. Cunha [Phys. Rev. Lett. 106, 190401 (2011)], and present a compatibility-loophole-free experimental violation of an inequality of noncontextual theories by two spatially separated entangled qutrits. A maximally entangled qutrit-qutrit state with a fidelity as high as 0.975±0.001 is prepared and distributed to separated spaces, and these two photons are then measured locally, providing the compatibility requirement. The results show that the inequality for noncontextual theory is violated by 31 standard deviations. Our experiments pave the way to close the debate about the testability of the KS theorem. In addition, the method to generate high-fidelity and high-dimension entangled states will provide significant advantages in high-dimension quantum encoding and quantum communication.

Nonlocality from Local Contextuality.

We experimentally show that nonlocality can be produced from single-particle contextuality by using two-particle correlations which do not violate any Bell inequality by themselves. This demonstrates that nonlocality can come from an a priori different simpler phenomenon, and connects contextuality and nonlocality, the two critical resources for, respectively, quantum computation and secure communication. From the perspective of quantum information, our experiment constitutes a proof of principle that quantum systems can be used simultaneously for both quantum computation and secure communication.

Quantum Storage of Three-Dimensional Orbital-Angular-Momentum Entanglement in a Crystal.

Here we present the quantum storage of three-dimensional orbital-angular-momentum photonic entanglement in a rare-earth-ion-doped crystal. The properties of the entanglement and the storage process are confirmed by the violation of the Bell-type inequality generalized to three dimensions after storage (S=2.152±0.033). The fidelity of the memory process is 0.993±0.002, as determined through complete quantum process tomography in three dimensions. An assessment of the visibility of the stored weak coherent pulses in higher-dimensional spaces demonstrates that the memory is highly reliable for 51 spatial modes. These results pave the way towards the construction of high-dimensional and multiplexed quantum repeaters based on solid-state devices. The multimode capacity of rare-earth-based optical processors goes beyond the temporal and the spectral degree of freedom, which might provide a useful tool for photonic information processing.

Quantum simulation of Landau-Zener model dynamics supporting the Kibble-Zurek mechanism.

The Kibble-Zurek mechanism (KZM) captures the key physics of nonequilibrium dynamics in second order phase transitions, and accurately predicts the density of topological defects formed in such processes. However, the central prediction of KZM--i.e., the scaling of the density of defects with the quench rate--still needs further experimental confirmation, particularly for quantum transitions. Here, we perform a quantum simulation of the nonequilibrium dynamics of the Landau-Zener model based on a nine-stage optical interferometer with an overall visibility of 0.975±0.008. The results support the adiabatic-impulse approximation, which is the core of Kibble-Zurek theory. Moreover, the developed high-fidelity multistage optical interferometer can support more complex linear optical quantum simulations.

Efficient learning of mixed-state tomography for photonic quantum walk.

Noise-enhanced applications in open quantum walk (QW) has recently seen a surge due to their ability to improve performance. However, verifying the success of open QW is challenging, as mixed-state tomography is a resource-intensive process, and implementing all required measurements is almost impossible due to various physical constraints. To address this challenge, we present a neural-network-based method for reconstructing mixed states with a high fidelity (∼97.5%) while costing only 50% of the number of measurements typically required for open discrete-time QW in one dimension. Our method uses a neural density operator that models the system and environment, followed by a generalized natural gradient descent procedure that significantly speeds up the training process. Moreover, we introduce a compact interferometric measurement device, improving the scalability of our photonic QW setup that enables experimental learning of mixed states. Our results demonstrate that highly expressive neural networks can serve as powerful alternatives to traditional state tomography.

A von-Neumann-like photonic processor and its application in studying quantum signature of chaos.

Photonic quantum computation plays an important role and offers unique advantages. Two decades after the milestone work of Knill-Laflamme-Milburn, various architectures of photonic processors have been proposed, and quantum advantage over classical computers has also been demonstrated. It is now the opportune time to apply this technology to real-world applications. However, at current technology level, this aim is restricted by either programmability in bulk optics or loss in integrated optics for the existing architectures of processors, for which the resource cost is also a problem. Here we present a von-Neumann-like architecture based on temporal-mode encoding and looped structure on table, which is capable of multimode-universal programmability, resource-efficiency, phase-stability and software-scalability. In order to illustrate these merits, we execute two different programs with varying resource requirements on the same processor, to investigate quantum signature of chaos from two aspects: the signature behaviors exhibited in phase space (13 modes), and the Fermi golden rule which has not been experimentally studied in quantitative way before (26 modes). The maximal program contains an optical interferometer network with 1694 freely-adjustable phases. Considering current state-of-the-art, our architecture stands as the most promising candidate for real-world applications.

Realization of exceptional points along a synthetic orbital angular momentum dimension.

Exceptional points (EPs), at which more than one eigenvalue and eigenvector coalesce, are unique spectral features of non-Hermiticity (NH) systems. They exist widely in open systems with complex energy spectra. We experimentally demonstrate the appearance of paired EPs in a periodical-driven degenerate optical cavity along the synthetic orbital angular momentum dimension with a tunable parameter. The complex-energy band structures and the key features of EPs, i.e., their bulk Fermi arcs, parity-time symmetry breaking transition, energy swapping, and half-integer band windings, are directly observed by detecting the wavefront angle-resolved transmission spectrum. Our results demonstrate the flexibility of using the photonic synthetic dimensions to implement NH systems beyond their geometric dimension and EP-based sensing.

Topological band structure via twisted photons in a degenerate cavity.

Synthetic dimensions based on particles' internal degrees of freedom, such as frequency, spatial modes and arrival time, have attracted significant attention. They offer ideal large-scale lattices to simulate nontrivial topological phenomena. Exploring more synthetic dimensions is one of the paths toward higher dimensional physics. In this work, we design and experimentally control the coupling among synthetic dimensions consisting of the intrinsic photonic orbital angular momentum and spin angular momentum degrees of freedom in a degenerate optical resonant cavity, which generates a periodically driven spin-orbital coupling system. We directly characterize the system's properties, including the density of states, energy band structures and topological windings, through the transmission intensity measurements. Our work demonstrates a mechanism for exploring the spatial modes of twisted photons as the synthetic dimension, which paves the way to design rich topological physics in a highly compact platform.

Optical demonstration of quantum fault-tolerant threshold.

A major challenge in practical quantum computation is the ineludible errors caused by the interaction of quantum systems with their environment. Fault-tolerant schemes, in which logical qubits are encoded by several physical qubits, enable to the output of a higher probability of correct logical qubits under the presence of errors. However, strict requirements to encode qubits and operators render the implementation of a full fault-tolerant computation challenging even for the achievable noisy intermediate-scale quantum technology. Especially the threshold for fault-tolerant computation still lacks experimental verification. Here, based on an all-optical setup, we experimentally demonstrate the existence of the threshold for the fault-tolerant protocol. Four physical qubits are represented as the spatial modes of two entangled photons, which are used to encode two logical qubits. The experimental results clearly show that when the error rate is below the threshold, the probability of correct output in the circuit, formed with fault-tolerant gates, is higher than that in the corresponding non-encoded circuit. In contrast, when the error rate is above the threshold, no advantage is observed in the fault-tolerant implementation. The developed high-accuracy optical system may provide a reliable platform to investigate error propagation in more complex circuits with fault-tolerant gates.

Experimental verification of generalized eigenstate thermalization hypothesis in an integrable system.

Identifying the general mechanics behind the equilibration of a complex isolated quantum system towards a state described by only a few parameters has been the focus of attention in non-equilibrium thermodynamics. And several experimentally unproven conjectures are proposed for the statistical description of quantum (non-)integrable models. The plausible eigenstate thermalization hypothesis (ETH), which suggests that each energy eigenstate itself is thermal, plays a crucial role in understanding the quantum thermalization in non-integrable systems; it is commonly believed that it does not exist in integrable systems. Nevertheless, integrable systems can still relax to the generalized Gibbs ensemble. From a microscopic perspective, understanding the origin of this generalized thermalization that occurs in an isolated integrable system is a fundamental open question lacking experimental investigations. Herein, we experimentally investigated the spin subsystem relaxation in an isolated spin-orbit coupling quantum system. By applying the quantum state engineering technique, we initialized the system with various distribution widths in the mutual eigenbasis of the conserved quantities. Then, we compared the steady state of the spin subsystem reached in a long-time coherent dynamics to the prediction of a generalized version of ETH and the underlying mechanism of the generalized thermalization is experimentally verified for the first time. Our results facilitate understanding the origin of quantum statistical mechanics.