Compact multichannel spectrometer employed for soft x-ray spectrum diagnostics at the Shenguang-III Laser Facility.

The quantitative measurement of plasma soft x-ray spectra is an important diagnostic problem in indirect-drive laser inertial confinement fusion (ICF). We designed, built, and tested a compact multichannel soft x-ray spectrometer with both spatial and temporal resolution capabilities for the detection of the spatiotemporal distribution of soft x-ray spectra. The spectrometer occupies a small solid angle, and the close measurement angle used for each channel enables the measurement of the angular distribution of emitting soft x-rays in ICF experiments. The spectrometer comprises pinhole, filter, and multilayer flat mirror arrays, and an x-ray streak camera. Its energy range is 0.1 - 3 keV. The dispersive elements of the spectrometer were calibrated at the Beijing Synchrotron Radiation Facility. The accuracy of the calibration was ≤ 5%, and the combined energy resolution (E/ΔE) of the calibrated dispersive elements of each channel was higher than 10. Finally, the instrument was tested at the Shenguang-III Laser Facility. The measurement results of x-ray radiation flux are agreed well with the experimental results of the M-band flat-response x-ray diode, demonstrating the feasibility of the proposed spectrometer configuration.

Development of a quasi-coaxis dual-energy flat spectral response X-ray imaging instrument for measuring hotspot electron temperature.

The measurement of hotspot electron temperature is a paramount technique of implosion physics research in inertial confinement fusion. This study proposes a novel quasi-coaxis dual-energy flat spectral response high-resolution X-ray imaging instrument comprising a dual-channel total-reflection Kirkpatrick-Baez microscope and two flat non-periodic multilayer mirrors, which can image at 6.4 ± 0.5 and 9.67 ± 0.5 keV simultaneously. Various theoretical simulations were performed to verify the performance and feasibility of the imaging instrument, which was assembled and characterized in a laboratory. Experimental results show that the imaging instrument could achieve a high spatial resolution of 5 µm in a ± 150 µm field of view (FOV), the root mean square(RMS) deviation values of the measured reflection efficiency are 1.71% and 1.82% for the 6.4 keV and 9.67 keV imaging channels, respectively, in the ± 150 µm FOV.

Measurement of Time-Dependent Drive Flux on the Capsule for Indirectly Driven Inertial Confinement Fusion Experiments.

A new method for measuring the time-dependent drive flux at the hohlraum center is proposed as a better alternative to conventional wall-based techniques. The drive flux here is obtained by simultaneous measurement of the reemitted flux and shock velocity from a three-layered "cakelike" sample. With these two independent observables, the influence induced by the uncertainty of the material parameters of the sample can be effectively decreased. The influence from the closure of the laser entrance hole, which was the main challenge in conventional wall-based techniques, was avoided through localized reemitted flux measurement, facilitating drive flux measurement throughout the entire time history. These studies pave a new way for probing the time-dependent drive flux, for both cylindrical hohlraums and novel hohlraums with six laser entrance holes.

Development of a polar-view Kirkpatrick-Baez X-ray microscope for implosion asymmetry studies.

The development of a polar-view Kirkpatrick-Baez microscope, fielded in the upper polar zone of the Shenguang-III laser fusion facility, is presented. With this microscope, the resolving power of polar-direction X-ray imaging diagnostics is improved, to the 3 ~5 µm scale. The microscope is designed for implosion asymmetry studies, with response energy points at 1.2 keV, 3.5 keV, and 8 keV. A biperiodic multilayer scheme is adopted to accommodate multiple implosion stages. We present the overall optical system design, target aiming scheme, characteristic composite imaging diagnostic experiments and initial results. The inertial-driven quasi-one-dimensional spherical implosions were observed from orthogonal directions with a convergence ratio of ~14.4. Fine features of the stagnating hot spot core are also resolved.

First Octahedral Spherical Hohlraum Energetics Experiment at the SGIII Laser Facility.

The first octahedral spherical hohlraum energetics experiment is accomplished at the SGIII laser facility. For the first time, the 32 laser beams are injected into the octahedral spherical hohlraum through six laser entrance holes. Two techniques are used to diagnose the radiation field of the octahedral spherical hohlraum in order to obtain comprehensive experimental data. The radiation flux streaming out of laser entrance holes is measured by six flat-response x-ray detectors (FXRDs) and four M-band x-ray detectors, which are placed at different locations of the SGIII target chamber. The radiation temperature is derived from the measured flux of FXRD by using the blackbody assumption. The peak radiation temperature inside hohlraum is determined by the shock wave technique. The experimental results show that the octahedral spherical hohlraum radiation temperature is in the range of 170-182 eV with drive laser energies of 71 kJ to 84 kJ. The radiation temperature inside the hohlraum determined by the shock wave technique is about 175 eV at 71 kJ. For the flat-top laser pulse of 3 ns, the conversion efficiency of gas-filled octahedral spherical hohlraum from laser into soft x rays is about 80% according to the two-dimensional numerical simulation.

Development of high resolution dual-energy KBA microscope with large field of view for RT-instability diagnostics at SG-III facility.

High resolution X-ray diagnosis is a significant method for obtaining ablation-front and trajectory measurements targeting Rayleigh-Taylor (RT)-instability growth in initial confinement fusion (ICF) experiments. In this paper, a novel Kirkpatrick-Baez-type structure, as a kind of essential X-ray micro-imaging apparatus, has been developed that realizes a large field of view (FOV) and images with high resolution and energy response. Zoned multilayer coating technology is applied to the Kirkpatrick-Baez mirrors to transmit two specific quasi-monochromatic light through the same mirror and enables a compact dual-channel structure. This microscope has been assembled in the laboratory and later implemented at the Chinese SG-III laser facility. The characterization results show that this imaging system can achieve a good spatial resolution of 5 µm in a large FOV of 500 µm, while maintaining a strong monochromatic performance with bandwidth of 0.5 keV at 2.5 keV and 4.3 keV respectively.

Development of an x-ray eight-image Kirkpatrick-Baez diagnostic system for China's laser fusion facility.

This article presents the development of an x-ray eight-image Kirkpatrick-Baez diagnostic system to be used at China's Shenguang-III (SG-III) laser facility in aspects of the optical design, multilayers, and online/offline tests. Six pieces of concave spherical substrates are used for constituting a special optical structure. Dual-periodic tungsten/carbon (W/C) multilayers are used for high reflectivity and large angular bandwidth of ∼0.1°. The global spatial resolution is ∼5 µm in the ±100 µm range. The schemes of system installation, transport, collimation, and image acquisition at China's SG-III facility are also discussed.

Realization of a flat-response photocathode for x-ray streak cameras.

We present a novel photocathode which can make x-ray streak cameras to be of a flat spectral response in the x-ray energy range of 0.1-5 keV. The photocathode consists of two layers of gold foils with optimized thickness ratio and structures. The photocathode was calibrated, and it is shown that a flat spectral response has been achieved.

Direct measurement of x-ray flux for a pre-specified highly-resolved region in hohlraum.

A space-resolving flux detector (SRFD) is developed to measure the X-ray flux emitted from a specified region in hohlraum with a high resolution up to 0.11mm for the first time. This novel detector has been used successfully to measure the distinct X-ray fluxes emitted from hot laser spot and cooler re-emitting region simultaneously, in the hohlraum experiments on SGIII prototype laser facility. According to our experiments, the ratio of laser spot flux to re-emitted flux shows a strong time-dependent behavior, and the area-weighted flux post-processed from the measured laser spot flux and re-emitting wall flux agrees with that measured from Laser Entrance Hole by using flat-response X-ray detector (F-XRD). The experimental observations is reestablished by our two-dimensional hydrodynamic simulations and is well understood with the power balance relationship.

Extreme ultraviolet spectrometer for the Shenguang III laser facility.

An extreme ultraviolet spectrometer has been developed for high-energy density physics experiments at the Shenguang-III (SG-III) laser facility. Alternative use of two different varied-line-spacing gratings covers a wavelength range of 10-260 Å. A newly developed x-ray framing camera with single wide strip line is designed to record time-gated spectra with ~70 ps temporal resolution and 20 lp/mm spatial resolution. The width of the strip line is up to 20 mm, enhancing the capability of the spatial resolving measurements. All components of the x-ray framing camera are roomed in an aluminum air box. The whole spectrometer is mounted on a diagnostic instrument manipulator at the SG-III laser facility for the first time. A new alignment method for the spectrometer based on the superimposition of two laser focal spots is developed. The approaches of the alignment including offline and online two steps are described. A carbon spectrum and an aluminum spectrum have been successfully recorded by the spectrometer using 2400 l/mm and 1200 l/mm gratings, respectively. The experimental spectral lines show that the spectral resolution of the spectrometer is about 0.2 Å and 1 Å for the 2400 l/mm and 1200 l/mm gratings, respectively. A theoretical calculation was carried out to estimate the maximum resolving power of the spectrometer.

K-shell photoabsorption edge of strongly coupled matter driven by laser-converted radiation.

The first observation of the K-shell photoabsorption edge of strongly coupled matter with an ion-ion coupling parameter of about 65 generated by intense x-ray radiation-driven shocks is reported. The soft x-ray radiation generated by laser interaction with a "dog bone" high-Z hohlraum is used to ablate two thick CH layers, which cover a KCl sample, to create symmetrical inward shocks. While the two shocks impact at the central KCl sample, a highly compressed KCl is obtained with a density of 3-5 times solid density and a temperature of about 2-4 eV. The photoabsorption spectra of chlorine near the K-shell edge are measured with a crystal spectrometer using a short x-ray backlighter. The redshift of the K edge up to 11.7 eV and broadening of 15.2 eV are obtained for the maximum compression. A comparison of the measured redshifts and broadenings with dense plasma calculations are made, and it indicates potential improvements in the theoretical description.

Determination of the hohlraum M-band fraction by a shock-wave technique on the SGIII-prototype laser facility.

The proposal of simultaneously determining the hohlraum peak radiation temperature T(R) and M-band fraction f(M) by shock velocity measurement technique [Y. S. Li et al. Phys. Plasmas 18, 022701 (2011)] is demonstrated for the first time in recent experiments conducted on SGIII-prototype laser facility. In the experiments, T(R) and f(M) are determined by using the observed shock velocities in Al and Ti. For the Au hohlraum used in the experiments, T(R) is about 160 eV and f(M) is around 4.3% under a 1 ns laser pulse of 2 kJ. The results from this method are complementary to those from the broadband x-ray spectrometer, and the technique can be further used to determine T(R) and f(M) inside an ignition hohlraum.

Quasi-sinusoidal single-order diffraction transmission grating used in x-ray spectroscopy.

A novel design of quasi-sinusoidal single-order diffraction transmission grating (QSTG) is proposed, which can achieve a line density up to thousands line/millimeter as that of traditional transmission gratings with the current level of nanofabrication technique. We fabricate a 1000 line/mm QSTG using the new design approach, and display the calibration results of such QSTG on the soft x-ray beam of synchrotron radiation.

First exploration of radiation temperatures of the laser spot, re-emitting wall and entire hohlraum drive source.

This study explores the radiation field temperatures introduced by the laser spot, the re-emitting wall in a hohlraum and the entire hohlraum drive source. This investigation, which is the first of its kind, is based on the radiation fluxes from the laser spot and the re-emitting wall, which have been accurately measured using time- and space-resolving flux detectors in a recent work, and additional flux data. The temperature difference between the laser spot and the entire hohlraum drive source was 6.08-35.35% of the temperature of the latter throughout the entire laser pulse, whilst that for the re-emitting wall was 3.90-12.81%. The radiation temperature of the cooler re-emitting wall had more influence on the temperature increase of the entire hohlraum drive source than the hot laser-spot temperature, which has been quantitatively discussed. Experimentally, we established the average distributions of the temperature fields of all the emitting sources, namely laser spot and re-emitting wall, of the irradiating fluxes on the capsule region in the hohlraum radiation field. This important progress in the exploration of radiation temperature distributions within a hohlraum will provide a foundation for determination of the irradiating radiation on the capsule and evaluation of capsule symmetry.

Metal-coordination crosslinked N-polyindoles as recyclable high-performance thermosets and nondestructive detection for their tensile strength and glass transition temperature.

Metal coordination crosslinking between stiff N-polyindole chains was constructed, and the crosslinked films exhibited high tensile strength, high heat resistance and excellent polar solvent resistance. The noncovalent crosslinking can be further removed via external pyrophosphate, which endows the crosslinked polymer with a recyclable behavior. The tensile strength and glass transition temperature of the polymers can be nondestructively detected by taking advantage of the fluorescence quenching effect of metal coordination to the adjacent bipyridine structure.

Direct intensity calibration of X-ray grazing-incidence microscopes with home-lab source.

Direct intensity calibration of X-ray grazing-incidence microscopes is urgently needed in quantitative studies of X-ray emission from laser plasma sources in inertial confinement fusion. The existing calibration methods for single reflecting mirrors, crystals, gratings, filters, and X-ray detectors are not applicable for such X-ray microscopes due to the specific optical structure and the restrictions of object-image relation. This article presents a reliable and efficient method that can be performed using a divergent X-ray source and an energy dispersive Si-PIN (silicon positive-intrinsic-negative) detector in an ordinary X-ray laboratory. The transmission theory of X-ray flux in imaging diagnostics is introduced, and the quantities to be measured are defined. The calibration method is verified by a W/Si multilayer-coated Kirkpatrick-Baez microscope with a field of view of ∼95 µm at 17.48 keV. The mirror reflectance curve in the 1D coordinate is drawn with a peak value of 20.9% and an uncertainty of ∼6.0%.

A time-gated multi-channel x-ray crystal spectrometer on the Shenguang-III laser facility.

An eight-channel x-ray flat crystal spectrometer was developed for high energy density physics research at the Shenguang-III (SG-III) laser facility. The spectrometer uses trihydroxymethylaminomethane crystals (2d = 8.78 Å) to record Ti K-shell emission in the photon energy range of 4.65-5.05 keV. The spectrometer couples to an x-ray framing camera to achieve time-resolution. This has four microstrips, and each strip records two snapshots of the emission image. Based on the intersection positioning system with a dual-charge coupled device, the alignment system is easily operated and efficient. The instrument was tested and used for Au hohlraum plasma diagnosis experiments on SG-III. The He-α line and its Li-like satellites and the Ly-α line of a Ti tracer were detected, from which the spectral resolution of the instrument was analyzed. The spectral resolution E/ΔE at the Ti He-α line ranges from about 500 to 880 and mainly limited by the x-ray source size.

Application of the space-resolving flux detector for radiation measurements from an octahedral-aperture spherical hohlraum.

Space-resolving flux detection is an important technique for the diagnostic of the radiation field within the hohlraum in inertial confinement fusion, especially for the radiation field diagnostic in the novel spherical hohlraum with octahedral six laser entrance holes (LEHs), where localized measurements are necessary for the discrimination of the radiation flux from different LEHs. A novel space-resolving flux detector (SRFD) is developed at the SG-III laser facility for the radiation flux measurement in the first campaign of the octahedral spherical hohlraum energetics experiment. The principle and configuration of the SRFD system is introduced. The radiation flux from the wall of a gas-filled octahedral spherical hohlraum is measured for the first time by placing the SRFD system at the equatorial position of the SG-III laser facility, aiming at the hohlraum wall through one of the six LEHs. The absolute radiation flux from the re-emission area on the hohlraum wall is measured, and good consistency is found between the experimental data and the calculated data from a three-dimensional view factor analysis.

Ion temperature measurements of indirect-drive implosions with the neutron time-of-flight detector on SG-III laser facility.

The accuracy of the determination of the burn-averaged ion temperature of inertial confinement fusion implosions depends on the unfold process, including deconvolution and convolution methods, and the function, i.e., the detector response, used to fit the signals measured by neutron time-of-flight (nToF) detectors. The function given by Murphy et al. [Rev. Sci. Instrum. 68(1), 610-613 (1997)] has been widely used in Nova, Omega, and NIF. There are two components, i.e., fast and slow, and the contribution of scattered neutrons has not been dedicatedly considered. In this work, a new function, based on Murphy's function has been employed to unfold nToF signals. The contribution of scattered neutrons is easily included by the convolution of a Gaussian response function and an exponential decay. The ion temperature is measured by nToF with the new function. Good agreement with the ion temperature determined by the deconvolution method has been achieved.

Implementation of ultraviolet Thomson scattering on SG-III laser facility.

An ultraviolet Thomson-scattering system has been designed and implemented on the Shenguang-III laser facility, a 48-beam, 3ω (351 nm), 180 kJ-level laser driver for high energy density physics and inertial confinement fusion researches. The 4ω (263.3 nm) probe beam of the Thomson-scattering system is injected from the north pole (top) of the target chamber, with an assistant beam-pointing monitor to achieve high pointing accuracy. The Thomson-scattered light is collected by a double-Cassegrain optical transmission system, which provides an achromatic image over a wide wavelength range of 200-800 nm. A novel on-line alignment method is developed and applied to the diagnostic system, ensuring a volumetric positioning accuracy of ∼30 µm for the scattering volume. An online calibration is also conducted to provide the wavelength benchmark and the spectral resolution of the system. This Thomson-scattering system has been tested in a complicated experimental environment with gas-filled hohlraums, and a high-quality ion feature of the scattered light has been obtained.