Simultaneous spatio-temporal focusing with pulse front symmetrization.

Simultaneous spatio-temporal focusing of ultrashort pulses is usually performed by single-channel stretcher-compressor geometries where pulse front tilt leads to spatial asymmetry. Here, the basic approach is extended by superimposing two reciprocal sub-beams in a dual-channel stretcher-compressor setup. Spatio-temporal properties of the symmetrized focal zones of few-cycle near-infrared pulses are studied by parametric numerical simulations with physical optics software. Spatial modulations of focal zones depending on focusing conditions appear. Relationships to specific ultrafast interference phenomena are addressed.

Self-imaging of tailored vortex pulse arrays and spectral Gouy rotation echoes.

Self-imaging of femtosecond pulses with orbital angular momentum is studied in spectral domain by illuminating the orthogonal arrays of spiral gratings. Spectral Gouy rotation, i.e., the characteristic circulation of extremal regions near phase singularities in spatial spectral maps, is found to partially reappear at discrete distances. The self-imaging of co-rotating and counter-rotating vortices is compared in intensity and spectral behavior. High-selectivity pattern recognition from weakly modulated spectral maps is demonstrated by analyzing spectral moments. By our experiments, the classical Talbot effect is extended to polychromatic pulsed vortex arrays with controlled maps of rotation sign.

Nondiffracting self-imaging of ultrashort wavepackets.

Self-imaging of ultrashort-pulsed nondiffracting needle beams, i.e., fringe-free Bessel beams, is analyzed. In contrast to the classical diffractive Talbot effect, pulse revivals with minimum spectral and temporal distortion are obtained. Robustness is further enhanced by self-reconstruction. The high-fidelity pulse transfer enables spatial and temporal multiplexing in free space without the need for a nonlinear medium, even at pulse durations down to the few-cycle range.

Refractive-diffractive dispersion compensation for optical vortex beams with ultrashort pulse durations.

Wave fields, which are described mathematically by higher order Bessel functions, carry an orbital angular momentum and thus represent particular types of optical vortex beams with helical wavefronts. For the generation of such vortex beams, one may use, for instance, diffractive spiral axicons. Diffraction, however, leads invariably to strong dispersion, which is detrimental for ultrashort pulses since it leads to severe pulse broadening. This pulse broadening can be minimized or reduced completely (at least, in a specific plane of propagation) if the pulses propagate additionally through a medium with normal refractive dispersion. The refractive-diffractive generation of ultrashort vortex pulses was demonstrated earlier for a pulse duration of approximately 8 fs [Opt. Lett.37, 3804 (2012)10.1364/OL.37.003804OPLEDP0146-9592]. Here, we present an analytical description of the generation and propagation of these vortex beams and of the refractive-diffractive compensation of the dispersion.

Sub-3-cycle vortex pulses of tunable topological charge.

Novel types of reflective spiral micro-electro-mechanical systems were used to generate few-cycle vortex pulses of variable topological charge from a Ti:sapphire laser oscillator. The phase profile of these components was controlled by varying the temperature. The temporal properties of the pulses were characterized with spatially resolved nonlinear autocorrelation. The beam structure resembles a slightly distorted Laguerre-Gaussian distribution. The different topological charges were indicated by detecting Poynting-vector maps with a programmable Shack-Hartmann sensor of enhanced angular sensitivity.

Few-cycle high-contrast vortex pulses.

Few-cycle high-contrast vortex beams with pulse durations around 8 fs were generated from a Ti:sapphire laser oscillator with a single diffractive-refractive component. Angular and temporal pulse properties were characterized with an advanced time-wavefront sensor. The temporal transfer indicates a fairly complete self-compensation.

Reconfigurable wavefront sensor for ultrashort pulses.

A highly flexible Shack-Hartmann wavefront sensor for ultrashort pulse diagnostics is presented. The temporal system performance is studied in detail. Reflective operation is enabled by programming tilt-tolerant microaxicons into a liquid-crystal-on-silicon spatial light modulator. Nearly undistorted pulse transfer is obtained by generating nondiffracting needle beams as subbeams. Reproducible wavefront analysis and spatially resolved second-order autocorrelation are demonstrated at incident angles up to 50° and pulse durations down to 6 fs.

Highly efficient THG in TiO2 nanolayers for third-order pulse characterization.

Third harmonic generation (THG) of femtosecond laser pulses in sputtered nanocrystalline TiO2 thin films is investigated. Using layers of graded thickness, the dependence of THG on the film parameters is studied. The maximum THG signal is observed at a thickness of 180 nm. The corresponding conversion efficiency is 26 times larger compared to THG at the air-glass interface. For a demonstration of the capabilities of such a highly nonlinear material for pulse characterization, third-order autocorrelation and interferometric frequency-resolved optical gating (IFROG) traces are recorded with unamplified nanojoule pulses directly from a broadband femtosecond laser oscillator.

Extended-area nanostructuring of TiO2 with femtosecond laser pulses at 400 nm using a line focus.

An efficient way to generate nanoscale laser-induced periodic surface structures (LIPSS) in rutile-type TiO(2) with frequency-converted femtosecond laser pulses at wavelengths around 400 nm is reported. Extended-area structuring on fixed and moving substrates was obtained by exploiting the line focus of a cylindrical lens. Under defined conditions with respect to pulse number, pulse energy and scanning velocity, two types of ripple-like LIPSS with high and low spatial frequencies (HSFL, LSFL) with periods in the range of 90 nm and 340 nm, respectively, were formed. In particular, lower numbers of high energetic pulses favour the generation of LSFL whereas higher numbers of lower energetic pulses enable the preferential creation of HSFL. Theoretical calculations on the basis of the Drude model support the assumption that refractive index changes by photo-excited carriers are a major mechanism responsible for LSFL. Furthermore, the appearance of random substructures as small as 30 nm superimposing low spatial frequency ripples is demonstrated and their possible origin is discussed.

Synthesized femtosecond laser pulse source for two-wavelength contouring with simultaneously recorded digital holograms.

A dual-wavelength femtosecond laser pulse source and its application for digital holographic single-shot contouring are presented. The synthesized laser source combines sub-picosecond time scales with a wide reconstruction range. A center wavelength distance of the two separated pulses of only 15 nm with a high contrast was demonstrated by spectral shaping of the 50 nm broad seed spectrum centered at 800 nm. Owing to the resulting synthetic wavelength, the scan depth range without phase ambiguity is extended to the 100-microm-range. Single-shot dual-wavelength imaging is achieved by using two CMOS cameras in a Twyman-Green interferometer, which is extended by a polarization encoding sequence to separate the holograms. The principle of the method is revealed, and experimental results concerning a single axis scanner mirror operating at a resonance frequency of 0.5 kHz are presented. Within the synthetic wavelength, the phase difference information of the object was unambiguously retrieved and the 3D-shape calculated. To the best of our knowledge, this is the first time that single-shot two-wavelength contouring on a sub-ps time scale is reported.

Prospects of target nanostructuring for laser proton acceleration.

In laser-based proton acceleration, nanostructured targets hold the promise to allow for significantly boosted proton energies due to strong increase of laser absorption. We used laser-induced periodic surface structures generated in-situ as a very fast and economic way to produce nanostructured targets capable of high-repetition rate applications. Both in experiment and theory, we investigate the impact of nanostructuring on the proton spectrum for different laser-plasma conditions. Our experimental data show that the nanostructures lead to a significant enhancement of absorption over the entire range of laser plasma conditions investigated. At conditions that do not allow for efficient laser absorption by plane targets, i.e. too steep plasma gradients, nanostructuring is found to significantly enhance the proton cutoff energy and conversion efficiency. In contrast, if the plasma gradient is optimized for laser absorption of the plane target, the nanostructure-induced absorption increase is not reflected in higher cutoff energies. Both, simulation and experiment point towards the energy transfer from the laser to the hot electrons as bottleneck.

Angular tolerance of Shack-Hartmann wavefront sensors with microaxicons.

Wavefront sensing under nonparaxial conditions was studied with Shack-Hartmann setups based on arrays of microaxicons. The robustness of the generated pseudonondiffracting subbeams against tilt and axial displacement was demonstrated for ultraflat Gaussian- and inverse-Gaussian-shaped elements in transmission and reflection. To characterize slight aberrations and to identify optimum parameter fields, spatial moments of intensity profiles were analyzed with high sensitivity. Reflective design enables for wavefront sensing at oblique incidence as necessary for low-feedback detection and phase diagnostics of ultrashort pulses.

Scalable multichannel micromachining with pseudo-nondiffracting vacuum ultraviolet beam arrays generated by thin-film axicons.

Scalable multichannel microstructuring was demonstrated by multiplexing a focused molecular fluorine laser beam with cylindrical nanolayer microaxicons into an array of converging pseudo-nondiffracting subbeams. The axicons were fabricated by shadow-mask vapor deposition of magnesium fluoride onto substrates of identical material. Long-period surface gratings of variable pitch were generated on poly(methyl methacrylate) by varying the target position within the converging periodic focal lines.