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1.
Nature ; 607(7918): 260-265, 2022 07.
Artigo em Inglês | MEDLINE | ID: mdl-35831598

RESUMO

In spite of the high-density and strongly correlated nature of the atomic nucleus, experimental and theoretical evidence suggests that around particular 'magic' numbers of nucleons, nuclear properties are governed by a single unpaired nucleon1,2. A microscopic understanding of the extent of this behaviour and its evolution in neutron-rich nuclei remains an open question in nuclear physics3-5. The indium isotopes are considered a textbook example of this phenomenon6, in which the constancy of their electromagnetic properties indicated that a single unpaired proton hole can provide the identity of a complex many-nucleon system6,7. Here we present precision laser spectroscopy measurements performed to investigate the validity of this simple single-particle picture. Observation of an abrupt change in the dipole moment at N = 82 indicates that, whereas the single-particle picture indeed dominates at neutron magic number N = 82 (refs. 2,8), it does not for previously studied isotopes. To investigate the microscopic origin of these observations, our work provides a combined effort with developments in two complementary nuclear many-body methods: ab initio valence-space in-medium similarity renormalization group and density functional theory (DFT). We find that the inclusion of time-symmetry-breaking mean fields is essential for a correct description of nuclear magnetic properties, which were previously poorly constrained. These experimental and theoretical findings are key to understanding how seemingly simple single-particle phenomena naturally emerge from complex interactions among protons and neutrons.

2.
Nature ; 581(7809): 396-400, 2020 05.
Artigo em Inglês | MEDLINE | ID: mdl-32461650

RESUMO

Molecular spectroscopy offers opportunities for the exploration of the fundamental laws of nature and the search for new particle physics beyond the standard model1-4. Radioactive molecules-in which one or more of the atoms possesses a radioactive nucleus-can contain heavy and deformed nuclei, offering high sensitivity for investigating parity- and time-reversal-violation effects5,6. Radium monofluoride, RaF, is of particular interest because it is predicted to have an electronic structure appropriate for laser cooling6, thus paving the way for its use in high-precision spectroscopic studies. Furthermore, the effects of symmetry-violating nuclear moments are strongly enhanced5,7-9 in molecules containing octupole-deformed radium isotopes10,11. However, the study of RaF has been impeded by the lack of stable isotopes of radium. Here we present an experimental approach to studying short-lived radioactive molecules, which allows us to measure molecules with lifetimes of just tens of milliseconds. Energetically low-lying electronic states were measured for different isotopically pure RaF molecules using collinear resonance ionisation at the ISOLDE ion-beam facility at CERN. Our results provide evidence of the existence of a suitable laser-cooling scheme for these molecules and represent a key step towards high-precision studies in these systems. Our findings will enable further studies of short-lived radioactive molecules for fundamental physics research.

3.
Phys Rev Lett ; 131(22): 222502, 2023 Dec 01.
Artigo em Inglês | MEDLINE | ID: mdl-38101341

RESUMO

Collinear laser spectroscopy was performed on the isomer of the aluminium isotope ^{26m}Al. The measured isotope shift to ^{27}Al in the 3s^{2}3p ^{2}P_{3/2}^{○}→3s^{2}4s ^{2}S_{1/2} atomic transition enabled the first experimental determination of the nuclear charge radius of ^{26m}Al, resulting in R_{c}=3.130(15) fm. This differs by 4.5 standard deviations from the extrapolated value used to calculate the isospin-symmetry breaking corrections in the superallowed ß decay of ^{26m}Al. Its corrected Ft value, important for the estimation of V_{ud} in the Cabibbo-Kobayashi-Maskawa matrix, is thus shifted by 1 standard deviation to 3071.4(1.0) s.

4.
Phys Rev Lett ; 128(15): 152501, 2022 Apr 15.
Artigo em Inglês | MEDLINE | ID: mdl-35499902

RESUMO

The impact of nuclear deformation can been seen in the systematics of nuclear charge radii, with radii generally expanding with increasing deformation. In this Letter, we present a detailed analysis of the precise relationship between nuclear quadrupole deformation and the nuclear size. Our approach combines the first measurements of the changes in the mean-square charge radii of well-deformed palladium isotopes between A=98 and A=118 with nuclear density functional calculations using Fayans functionals, specifically Fy(std) and Fy(Δr,HFB), and the UNEDF2 functional. The changes in mean-square charge radii are extracted from collinear laser spectroscopy measurements on the 4d^{9}5s ^{3}D_{3}→4d^{9}5p ^{3}P_{2} atomic transition. The analysis of the Fayans functional calculations reveals a clear link between a good reproduction of the charge radii for the neutron-rich Pd isotopes and the overestimated odd-even staggering: Both aspects can be attributed to the strength of the pairing correlations in the particular functional which we employ.

5.
Phys Rev Lett ; 127(27): 272301, 2021 Dec 31.
Artigo em Inglês | MEDLINE | ID: mdl-35061421

RESUMO

The ground state to ground state electron-capture Q value of ^{159}Dy (3/2^{-}) has been measured directly using the double Penning trap mass spectrometer JYFLTRAP. A value of 364.73(19) keV was obtained from a measurement of the cyclotron frequency ratio of the decay parent ^{159}Dy and the decay daughter ^{159}Tb ions using the novel phase-imaging ion-cyclotron resonance technique. The Q values for allowed Gamow-Teller transition to 5/2^{-} and the third-forbidden unique transition to 11/2^{+} state with excitation energies of 363.5449(14) keV and 362.050(40) keV in ^{159}Tb were determined to be 1.18(19) keV and 2.68(19) keV, respectively. The high-precision Q value of transition 3/2^{-}→5/2^{-} from this work, revealing itself as the lowest electron-capture Q value, is used to unambiguously characterize all the possible lines that are present in its electron-capture spectrum. We performed atomic many-body calculations for both transitions to determine electron-capture probabilities from various atomic orbitals and found an order of magnitude enhancement in the event rates near the end point of energy spectrum in the transition to the 5/2^{-} nuclear excited state, which can become very interesting once the experimental challenges of identifying decays into excited states are overcome. The transition to the 11/2^{+} state is strongly suppressed and found unsuitable for measuring the neutrino mass. These results show that the electron-capture in the ^{159}Dy atom, going to the 5/2^{-} state of the ^{159}Tb nucleus, is a new candidate that may open the way to determine the electron-neutrino mass in the sub-eV region by studying electron-capture. Further experimental feasibility studies, including coincidence measurements with realistic detectors, will be of great interest.

6.
Phys Rev Lett ; 127(3): 033001, 2021 Jul 16.
Artigo em Inglês | MEDLINE | ID: mdl-34328758

RESUMO

Isotope shifts of ^{223-226,228}Ra^{19}F were measured for different vibrational levels in the electronic transition A^{2}Π_{1/2}←X^{2}Σ^{+}. The observed isotope shifts demonstrate the particularly high sensitivity of radium monofluoride to nuclear size effects, offering a stringent test of models describing the electronic density within the radium nucleus. Ab initio quantum chemical calculations are in excellent agreement with experimental observations. These results highlight some of the unique opportunities that short-lived molecules could offer in nuclear structure and in fundamental symmetry studies.

7.
Sci Rep ; 13(1): 4783, 2023 Mar 23.
Artigo em Inglês | MEDLINE | ID: mdl-36959230

RESUMO

High-precision hyperfine structure measurements were performed on stable, singly-charged [Formula: see text]Co ions at the IGISOL facility in Jyväskylä, Finland using the collinear laser spectroscopy technique. A newly installed light collection setup enabled the study of transitions in the 230 nm wavelength range from low-lying states below 6000 cm[Formula: see text]. We report a 100-fold improvement on the precision of the hyperfine A parameters, and furthermore present newly measured hyperfine B paramaters.

8.
Nat Commun ; 12(1): 4596, 2021 Jul 28.
Artigo em Inglês | MEDLINE | ID: mdl-34321487

RESUMO

Understanding the evolution of the nuclear charge radius is one of the long-standing challenges for nuclear theory. Recently, density functional theory calculations utilizing Fayans functionals have successfully reproduced the charge radii of a variety of exotic isotopes. However, difficulties in the isotope production have hindered testing these models in the immediate region of the nuclear chart below the heaviest self-conjugate doubly-magic nucleus 100Sn, where the near-equal number of protons (Z) and neutrons (N) lead to enhanced neutron-proton pairing. Here, we present an optical excursion into this region by crossing the N = 50 magic neutron number in the silver isotopic chain with the measurement of the charge radius of 96Ag (N = 49). The results provide a challenge for nuclear theory: calculations are unable to reproduce the pronounced discontinuity in the charge radii as one moves below N = 50. The technical advancements in this work open the N = Z region below 100Sn for further optical studies, which will lead to more comprehensive input for nuclear theory development.

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