Effective dose assessment due to inhalation of 222Rn, 220Rn, and their progeny: highlighting the major contribution of thoron in a thoron-prone area in Cameroon.

To assess public exposure to radon, thoron, and their progeny, measurements were conducted in 50 dwellings within the bauxite-rich area of Fongo-Tongo in western Cameroon. Passive integrating radon-thoron discriminative detectors (specifically RADUET) were employed for radon and thoron measurements. Additionally, concentrations of short-lived radon and thoron progeny were estimated using Direct Radon Progeny Sensors (DRPSs) and Direct Thoron Progeny Sensors (DTPSs) based on LR-115 detectors. The findings revealed indoor radon concentrations ranging from 31 to 123 Bq m-3 with a geometric mean (GM) of 62 Bq m-3, and indoor thoron concentrations ranging from 36 to 688 Bq m-3 with a GM of 242 Bq m-3. The Equilibrium Equivalent Radon Concentration (EERC) ranged from 3 to 86 Bq m-3 with a GM of 25 Bq m-3, while the Equilibrium Equivalent Thoron Concentration (EETC) ranged from 1.2 to 12.5 Bq m-3 with a GM of 7.6 Bq m-3. Notably, all dwellings recorded radon concentrations below 100 Bq m-3. Arithmetic means of radon and thoron equilibrium factors were calculated as 0.47 and 0.04, respectively. To assess annual effective doses from radon and thoron inhalation, equilibrium factors were used along with direct measurements of EERC and EETC. The differences observed in annual effective doses were 4.5% for radon and 42.5% for thoron. Furthermore, the contribution of thoron and its decay products to the annual effective dose from radon, thoron, and their progeny ranged from 12 to 94%, with an average contribution of 58%. Thus, this study found that the effective dose due to thoron inhalation in the study area exceeded that due to radon inhalation. It is concluded that, when evaluating radiation doses and health risks, it is crucial to consider both thoron and its progeny alongside radon and its progeny. This underscores the importance of considering direct measurements for accurately estimating radiation doses.

Relevance of radon progeny measurements for the assessment of inhalation doses in groundwater utilities.

The high radon concentrations measured in the indoor air of groundwater facilities and the prevalence of the problem have been known for several years. Unlike in other workplaces, in groundwater plants, radon is released into the air from the water treatment processes. During the measurements of this study, the average radon concentrations varied from 500 to 8800 Bq m-3. In addition, the indoor air of the treatment plants is filtered and there are no significant internal aerosol sources. However, only a few published studies on groundwater plants have investigated the properties of the radon progeny aerosol, such as the equilibrium factor (F) or the size distribution of the aerosol, which are important for assessing the dose received by workers. Moreover, the International Commission on Radiological Protection has not provided generic aerosol parameter values for dose assessment in groundwater treatment facilities. In this study, radon and radon progeny measurements were carried out at three groundwater plants. The results indicate surprisingly high unattached fractions (fp= 0.27-0.58), suggesting a low aerosol concentration in indoor air. The correspondingFvalues were 0.09-0.42, well below those measured in previous studies. Based on a comparison of the effective dose rate calculations, either the determination of thefpor, with certain limitations, the measurement of radon is recommended. Dose rate calculation based on the potential alpha energy concentration alone proved unreliable.

Changes induced in the human respiratory tract by chronic cigarette smoking can reduce the dose to the lungs from exposure to radon progeny.

Chronic cigarette smoking leads to changes in the respiratory tract that might affect the dose received from exposure to radon progeny. In this study, changes induced by cigarette smoking in the respiratory tract were collected from the literature and used for calculation of the dose received by the lungs and organs outside the respiratory tract. Morphological and physiological parameters affected by chronic smoking were implemented in the human respiratory tract model (HRTM) used by the International Commission of Radiological Protection (ICRP). Smokers were found to receive lung doses 3% smaller than the ICRP reference worker (non-smoking reference adult male) in mines and 14% smaller in indoor workplaces and tourist caves. A similar dose reduction was found for the extrathoracic region of the HRTM. Conversely, kidneys, brain, and bone marrow of smokers were found to receive from 2.3- up to 3-fold of the dose received by the respective organ in the ICRP reference worker, although they remained at least two orders of magnitude smaller than the lung dose. These results indicate that the differences in the lung dose from radon progeny exposure in cigarette smokers and non-smokers are smaller than 15%.

Impact of humidity and flowrate on the thoron measurement sensitivity of electrostatic radon monitors.

The accurate measurement of thoron activity concentration is an important issue in both thoron exposure evaluation and in reducing its influence on radon measurement. For radon monitors based on electrostatic collection technique and an alpha spectrometry analyser, air humidity and sampling flowrate are key factors influencing the sensitivity of thoron activity concentration measurement. For the purpose of improving thoron measurement sensitivity and stability, theoretical derivation and experimental studies were systemically performed in this study. The results show that thoron measurement sensitivity decreases as a negative exponential function with absolute humidity increasing, and the sensitivity of thoron is much lower than that of radon under the same conditions, which is mainly caused by the small value of the concentration ratio of thoron inside to outside of the chamber. When the air exchange rate of the measurement chamber (sampling flowrate/inner volume) increases, the measurement sensitivity of thoron gas first increases rapidly and then decreases slowly after reaching its maximum at the air exchange rate of 0.24 s-1. In practice, in the normal air exchange rate range (for example <0.05 s-1), increasing the sampling flowrate could greatly improve the thoron measurement sensitivity, which consequently suggests an effective way to update thoron measurement under the present conditions of the monitor.

Does protracted radon exposure play a role in the development of dementia?

Radon is a ubiquitous radioactive gas that decays into a series of solid radioactive decay products. Radon, and its decay products, enter the human body primarily through inhalation and can be delivered to various tissues including the brain through systemic circulation. It can also reach the brain by neuronal pathways via the olfactory system. While ionizing radiation has been suggested as a risk factor of dementia for decades, studies exploring the possible role of radon exposure in the development of Alzheimer's Diseases (AD) and other dementias are sparse. We systematically reviewed the literature and found several lines of evidence suggesting that radon decay products (RDPs) disproportionally deposit in the brain of AD patients with selective accumulation within the protein fractions. Ecologic study findings also indicate a significant positive correlation between geographic-level radon distribution and AD mortality in the US. Additionally, pathologic studies of radon shed light on the potential pathways of radon decay product induced proinflammation and oxidative stress that may result in the development of dementia. In summary, there are plausible underlying biological mechanisms linking radon exposure to the risk of dementia. Since randomized clinical trials on radon exposure are not feasible, well-designed individual-level epidemiologic studies are urgently needed to elucidate the possible association between radon (i.e., RDPs) exposure and the onset of dementia.

Assessment of thoron contribution to indoor radon exposure in Canada.

From 2007 to 2013, simultaneous radon (222Rn) and thoron (220Rn) measurements were conducted in a total of 3534 residential homes in 34 metropolitan areas covering 71% of the Canadian population. While radon levels were above the detector's detection limit in almost all homes, thoron concentrations were measurable in only 1738 homes. When analysis was limited to homes where thoron concentrations exceeded the detection limit, a pooled analysis confirmed that thoron is log-normally distributed in the indoor environment, and the distribution was characterized by a population-weighted geometric mean of 13 Bq/m3 and a geometric standard deviation of 1.89. Thoron contribution to indoor radon dose varied widely, ranging from 1.3 to 32% geographically. This study indicated that on average, thoron contributes 4% of the radiation dose due to total indoor radon exposure (222Rn and 220Rn) in Canada.

Novel Algorithm for Radon Real-Time Measurements with a Pixelated Detector.

Nowadays, radon gas exposure is considered one of the main health concerns for the population because, by carrying about half the total dose due to environmental radioactivity, it is the second cause of lung cancer after smoking. Due to a relatively long half-life of 3.82 days, the chemical inertia and since its parent Ra-226 is largely diffuse on the earth's crust and especially in the building materials, radon can diffuse and potentially saturate human habitats, with a concentration that can suddenly change during the 24 h day depending on temperature, pressure, and relative humidity. For such reasons, 'real-time' measurements performed by an active detector, possibly of small dimensions and a handy configuration, can play an important role in evaluating the risk and taking the appropriate countermeasures to mitigate it. In this work, a novel algorithm for pattern recognition was developed to exploit the potentialities of silicon active detectors with a pixel matrix structure to measure radon through the α emission, in a simple measurement configuration, where the device is placed directly in air with no holder, no collection filter or electrostatic field to drift the radon progenies towards the detector active area. This particular measurement configuration (dubbed as bare) requires an α/ß-discrimination method that is not based on spectroscopic analysis: as the gas surrounds the detector the α particles are emitted at different distances from it, so they lose variable energy amount in air depending on the traveled path-length which implies a variable deposited energy in the active area. The pixels matrix structure allows overcoming this issue because the interaction of α, ß and γ particles generate in the active area of the detector clusters (group of pixels where a signal is read) of different shape and energy dispersion. The novel algorithm that exploits such a phenomenon was developed using a pixelated silicon detector of the TimePix family with a compact design. An α (Am-241) and a ß (Sr-90) source were used to calibrate the algorithm and to evaluate its performances in terms of ß rejection capability and α recognition efficiency. Successively, the detector was exposed to different radon concentrations at the ENEA-INMRI radon facility in 'bare' configuration, in order to check the linearity of the device response over a radon concentration range. The results for this technique are presented and discussed, highlighting the potential applications especially the possibility to exploit small and handy detectors to perform radon active measurements in the simplest configuration.

Radiological risk estimation from indoor radon, thoron, and their progeny concentrations using nuclear track detectors.

In this paper, we report the results of seasonal variations of indoor radon and thoron concentrations, equilibrium factors for gas progeny, and radiological risks to dwellers in the hilly area of Guwahati City, Assam, India. Twin-cup dosemeters with LR-115 (II) nuclear track detectors were used in this study. The findings show that values vary significantly, with winter having the highest values and summer having the lowest, with spring and autumn having moderate values. In winter, radon concentrations range from 61.6 ± 11.2 Bq m-3 (Mud) to 115.3 ± 34.3 Bq m-3 (AT), with geometric mean values of 69.2 ± 13.8 Bq m-3 and 109.4 ± 27.9 Bq m-3, and in summer, they range from 21.1 ± 5.9 Bq m-3 (Mud) to 28.4 ± 8.3 Bq m-3 (AT), with geometric mean values of 22.7 ± 6.3 Bq m-3 and 26.1 ± 7.1 Bq m-3, whereas thoron concentrations range from 13.1 ± 5.1 Bq m-3 (Mud) to 58.8 ± 12.6 Bq m-3 (AT), with geometric mean values of 27.6 ± 7.0 Bq m-3 and 52.9 ± 10.1 Bq m-3 in winter, respectively, and in summer, from 8.8 ± 2.3 Bq m-3 (Mud) to 13.0 ± 5.5 Bq m-3 (Mud), with a geometric mean value of 1.87 ± 1.29 Bq m-3. Radon and thoron progeny levels are reported to vary from 4.1 ± 0.3 mWL (Mud) to 15.1 ± 4.3 mWL (AT) and 2.6 ± 0.9 mWL (Mud) to 14.3 ± 4.2 mWL (AT) in winter and from 1.5 ± 0.7 mWL (AT) to 3.0 ± 2.5 mWL (Mud) and 0.9 ± 0.3 mWL (AT) to 2.7 ± 0.5 mWL (Mud) in summer, respectively. The equilibrium factors for radon and its progeny have been reported to range from 0.23 ± 0.1 (Mud) to 0.51 ± 0.3 (AT) in winter, whereas from 0.23 ± 0.1 (AT) to 0.48 ± 0.4 (Mud) in summer, respectively. The equilibrium factors for thoron and its progeny have been estimated in the range of 0.02 ± 0.01 (Mud) to 0.09 ± 0.06 (AT) in winter, whereas 0.02 ± 0.02 (AT) to 0.07 ± 0.05 (Mud) in summer, respectively. The inhalation dose rates differed from house to house, having values in the range of 1.2 ± 0.2 mSv year-1 (Mud) to 4.6 ± 1.3 mSv year-1 (AT) in winter, whereas 0.5 ± 0.3 mSv year-1 (AT) to 0.9 ± 0.5 mSv year-1 (Mud) in summer, respectively. The effective doses (EDs) due to the exposure of radon and thoron in the study area have been found to range from 2.5 ± 0.3 mSv (Mud) to 9.1 ± 2.7 mSv (AT) in winter and 0.9 ± 0.4 mSv (AT) to 1.8 ± 1.3 mSv (Mud) in summer, respectively. The levels of radon and thoron in similar types of construction were found to be significantly different from one house to another. The estimated radon and thoron concentrations in the houses of that region during winter are found to be substantially higher than the global averages as reported by UNSCEAR.

Seasonal variation of indoor radon, thoron and their progeny in Belagavi district of Karnataka, India.

Systematic investigations on the seasonal variation of indoor radon, thoron and their progeny levels have been carried out in Belagavi district of Karnataka, India. The radon and thoron levels were measured using LR-115 type II dosimeter in cups with single-entry pinhole. The measurements were carried out in all the four season, viz, monsoon, autumn, winter and summer, in selected houses of the region. The higher indoor radon levels were observed during autumn with an average concentration of 56.45 Bq m-3. The minimum in radon levels was observed in summer with an average concentration of 21.8 Bq m-3. The indoor thoron concentration was also maximum during autumn with an average value of 36.44 Bq m-3 and minimum in summer with an average value of 15.9 Bq m-3. The radon and thoron levels were also found to depend on the nature of walls and floorings of dwellings. The lung dose rate to the population due to radon ranged from 1.195 to 9.557 mSv year-1, with an average of 4.572 mSv year-1. Risk levels were found to be significant during autumn and winter due to the inhalation of indoor radon and thoron. The study forms the first comprehensive report on the indoor radon and thoron levels and the resulting population dose in the Belagavi region. The studies reveal that the major contributor to the population is radon and its progeny. However, a sizable dose also comes from indoor thoron and its progeny. The study emphasises the need to provide better ventilation system to future dwellings to reduce the risk from indoor radon and thoron.

Implications on dose estimation and dispersion patterns of thoron in a typical indoor environment.

A model that describes the pollutant sources/sinks and inlet-outlet can help to assess the indoor exposure. Short half-life of radioactive thoron (220Rn) makes it vital and an interesting element to study its dispersion behavior. This work presents an extensive depiction of the influence of indoor environment thoron dispersion under fixed boundary conditions within the volume domain of 90 m3 using computational fluid dynamics (CFD) software. For the desirable air flow, inlet and outlet are considered in the room and the k-ɛ model is used. The thoron distribution is studied at different locations and different heights to cover the whole room. Obtained dispersion patterns vary at different locations and indicate non-uniformity of thoron level with elevated values in the room corners. Mean concentration was found to be 11 Bq/m3 with the exhalation rate of 0.102 Bqm-2 s-1. Some stagnant zones were found especially at the corners where the concentration is almost 5 times the average concentration. Such varying thoron level results in the overestimation and underestimation of the dose. The inhomogeneous behavior of thoron may cause variation in equilibrium factor. A simulated model is beneficial in understanding the radioactive gas behavior and has its importance in planning to find the correct dose estimation and, therefore, the best mitigation techniques.

Radon-222: environmental behavior and impact to (human and non-human) biota.

As an inert radioactive gas, 222Rn could be easily transported to the atmosphere via emanation, migration, or exhalation. Research measurements pointed out that 222Rn activity concentration changes during the winter and summer months, as well as during wet and dry season periods. Changes in radon concentration can affect the atmospheric electric field. At the boundary layer near the ground, short-lived daughters of 222Rn can be used as natural tracers in the atmosphere. In this work, factors controlling 222Rn pathways in the environment and its levels in soil gas and outdoor air are summarized. 222Rn has a short half-life of 3.82 days, but the dose rate due to radon and its radioactive progeny could be significant to the living beings. Epidemiological studies on humans pointed out that up to 14% of lung cancers are induced by exposure to low and moderate concentrations of radon. Animals that breed in ground holes have been exposed to the higher doses due to radiation present in soil air. During the years, different dose-effect models are developed for risk assessment on human and non-human biota. In this work are reviewed research results of 222Rn exposure of human and non-human biota.

Wire mesh capped DRPS based bronchial dosimeter for personal inhalation dosimetry due to radon progeny.

A study has been carried out to experimentally determine the calibration factor (CF) of the passive bronchial dosimeter, which consists of a direct radon progeny sensor capped with a 100-wire mesh. First, the CF was determined in controlled environmental conditions simulated in a calibration chamber. With aerosol concentrations varying from 104p cm-3to 105p cm-3and relative humidity varying from 60% to 80% in the chamber, CF was observed to be nearly constant with an average value of (3.8 ± 0.5) × 10-3mSv tracks-1cm2. Then, the CF was determined in real indoor environments in which it was again observed to be almost constant and the mean value was found to be (5.6 ± 0.1) × 10-3mSv tracks-1cm2. Pooling all the data on CFs obtained under controlled conditions and in real indoor environments, a lognormal distribution of the CF was observed with a geometric mean and geometric standard deviation of 0.0052 mSv tracks-1cm2and 1.28 respectively. The experimentally determined value of CF was found to be in close agreement with the theoretically estimated value, taking into consideration the unattached fraction of radon progeny. This dosimeter is passive, cheap, lightweight and, moreover, the CF being stable against environmental variations, will be useful in monitoring inhalation doses due to radon progeny for occupational workers.

Lung cancer risk and effective dose coefficients for radon: UNSCEAR review and ICRP conclusions.

The United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR) has provided a detailed and authoritative update of its reviews of the epidemiology and dosimetry of radon and progeny. Lifetime risk of lung cancer calculated using data for several miner cohorts were 2.4-7.5 × 10-4per working level month (WLM) of radon-222 progeny exposure for a mixed male/female population and 3.0-9.6 × 10-4per WLM for a male population. Dosimetric models gave mean values of effective dose coefficients from radon-222 progeny of 12 mSv per WLM for mines, 16 mSv per WLM for indoor workplaces and 11 mSv per WLM for homes. The lifetime risk coefficient used by the International Commission on Radiological Protection (ICRP) is 5 × 10-4per WLM and it has recently recommended an effective dose coefficient for radon-222 and progeny of 3 mSv per mJ h m-3(about 10 mSv per WLM) for most circumstances of exposure. The ICRP risk and dose coefficients are supported by the UNSCEAR review and provide a clear and firm basis for current international advice and standards for protection from radon. Notwithstanding this evidence and the ICRP advice, UNSCEAR will continue to use a lower value of effective dose coefficient of 5.7 mSv per WLM for assessments of population exposures.

The analysis of results of radon/thoron measurements performed with the use of nuclear track detectors.

Radon has been identified as one of the most important hazards, causing lung cancer. The most important isotope of radon is222Rn (3.83 d), while thoron220Rn (55 s) is treated as the less important isotope due to its short half-life. The radon/thoron hazard for people is related to inhalation of their decay products, but usually, only measurements of radon gas are done in dwellings. For such a purpose nuclear track detectors are used in most of the cases. Since several years simultaneous measurements are done to estimate thoron contribution to indoor radon and thoron exposure with the use of track detectors, too. Typically, a set of two detectors are applied and thoron concentrations are calculated on the basis of discriminative calculations. Unfortunately, very often results of these surveys are not accurate due to underestimation of the lower limit of detection (LLD) for thoron in the presence of elevated radon concentrations. Therefore an analysis of thoron LLDs in relationship to radon concentrations is presented.

A method for the simultaneous measurement of radon and thoron PAEC concentrations in air using a TLD monitor.

The idea of using a device with thermo-luminescent detectors (TLD) for the simultaneous measurement of radon (Rn-222) and thoron (Rn-220) decay products' concentrations was invented and developed in the Silesian Centre for Environmental Radioactivity at the Central Mining Institute, Katowice, Poland. The results of a preliminary analysis of the technical applicability, the required minimum period of air sampling and the optimised time schedule proved that such measurements can provide information about the potential alpha energy concentrations (PAECs) of radon and thoron decay products (TnDP).Following the analysis, preliminary measurements were performed at several locations-in a thoron chamber, in dwellings and even outdoors. Surprisingly, the maximum PAEC of the TnDP in the basement of a twin house in the Upper Silesia region was as high as 0.68 ± 0.15µJ m-3. This paper presents the results of those measurements.

Comparison measurement of unattached radon progeny concentration in three different environments.

Accurate measurement of unattached radon progeny is important for dose evaluation of radon exposure. For quality control of field surveys, a series of comparison measurements were carried out using three commercial unattached radon progeny monitors in real environments as well as in a radon chamber. The results show that the radon equilibrium equivalent concentrations (EECs) of different monitors agree very well, mostly within ±3.0% where there is no thoron progeny interference in the radon chamber. However, the unattached fraction of radon progeny is not so consistent, and the relative difference is 3.3% ~ 39.5% in different environments. The unattached fraction of radon progeny is affected by aerosol concentration. Anomalously high unattached fraction was found in the environment with extremely high humidity and low aerosol concentration. For accurate measurement of unattached radon progeny, specific attention should be paid to the collection efficiency of unattached radon progeny and the interference of attached radon progeny on a wire screen.

Variations in radon dosimetry under different assessment approaches in the Altamira Cave.

The atmosphere of caves is a special environment where it is necessary to take into account some particular characteristics when assessing the radon dose. The equilibrium factor (F) between radon and its progeny, and especially its unattached fraction (f p), is a key parameter in radon dose evaluation. In order to consider the specific features of the atmosphere in the Altamira Cave, the radon and particle concentrations have been measured. The mean annual radon concentration inside the cave over the period 2013-2019 is around 3500 Bq m-3 with a standard deviation of 1833 Bq m-3 and this exhibits seasonal variations. This value surpasses all international (WHO, IAEA, ICRP) upper action and reference levels (occupational and non-occupational). Dose rate levels expressed in µSv h-1 were estimated for four different equilibrium scenarios between radon and its progeny 218Po, 214Pb, 214Bi and 214Po. The most recent dose conversion factors have been used and the contribution made to the dose by the unattached fraction of radon progeny f p has been also assessed from the particle concentration. The results suggest that the mean annual dose levels show variations of up to 500% due to the range of F and the f p considered in this study. Given the high radon concentrations usually found in show caves, the best way to reduce this variability and its associated uncertainty in dose assessment is to conduct specific studies aimed at determining both F and f p.

In vivo measurement of pre-operational spallation source workers: baseline body burden levels and detection limits of relevant gamma emitters using high-resolution gamma spectrometry.

As a measure to prepare for long-term internal dose monitoring of workers at the European Spallation Source (ESS) in Lund, Sweden, operated by the European Research Infrastructure Consortium (ERIC), as well as to enhance emergency preparedness against accidental releases, a series of in vivo measurements were conducted using a high-resolution HPGe detector with a 123% relative efficiency (1.332 MeV). This study describes the whole-body counting set-up, calibration procedure, and subsequent validation measurements using conventional NaI(Tl)-scanning-bed geometry on a selection of workers from the ESS. Detection limits for the relevant gamma emitters 7Be, 172Hf, and 182Ta were determined to be 65 Bq, 130 Bq, and 22 Bq, respectively, using a 2400 s acquisition time. The baseline measurements suggest that care must be taken to ensure that the fluctuations in the presence of radon daughters 214Bi and 214Pb are minimised by, for example, ensuring a minimum air exchange between the measuring room and the ambient air, and by demanding that the measured subjects change clothes and shower before measurement. Furthermore, in a monitoring program for internal doses to spallation source workers, the presence of radionuclides originating from non-work-related sources (such as 226Ra from private water wells or 137Cs from intakes of Chernobyl contaminated foodstuffs), or radionuclides from previous work history (such as 60Co within the nuclear power industry), must be considered.

Measurement of radon, thoron and their daughters in the air of marble factories and resulting alpha-radiation doses to the lung of workers.

Concentrations of radon (222Rn) and thoron (220Rn) were measured in the air of different marble factories by using a nuclear track technique. The influence of the marble dust nature and ventilation on radon and thoron concentrations was investigated. It was observed that measured radon and thoron concentration ranged from 310 to 903 Bq m-3 and 6 to 48 Bq m-3, respectively. In addition, alpha-activities due to the unattached and attached fractions of 218Po and 214Po radon short-lived progeny were evaluated in the marble factories studied. Committed equivalent doses due to the attached and unattached fractions of 218Po and 214Po nuclei were evaluated in the lung tissues of marble factory workers. The dependence of the resulting committed equivalent dose on the concentration of the attached and unattached fractions of the 218Po and 214Po radionuclides and mass of the tissue was investigated. The resulting annual committed effective doses to the lung of marble factory workers due to the attached and unattached fractions of the 218Po and 214Po radionuclides were calculated. The obtained results show that about 80% of the global committed effective doses received by workers in the studied marble factories are due to the attached fraction of the 218Po and 214Po radon short-lived daughters from the inhalation of polluted air. Male workers spending 8 h per day (2080 h per year) in a marble factory receive a maximum dose of 34.46 mSv y-1 which is higher than the (3-10 mSv y-1) dose limit interval given by the ICRP. Good agreement was found between data obtained for the average effective dose gotten by using this method and the UNSCEAR and ICRP conversion dose coefficients.

Validation of a rapid, conservative transuranic alpha activity estimation method in air samples.

In air filter assay for radiological emergency response, radon (222Rn) and thoron (220Rn) progeny are known interferents to transuranic activity estimation. Previous work detailed a conservative, graded approach for TRU alpha activity estimation from air samples void of transuranic activity yet containing varying amounts of radon and thoron progeny. Validation of this method to produce rapid, conservative and defensible transuranic alpha activity estimates was accomplished through introduction of surrogate transuranic activity, 239Pu and 230Th check sources, along with the naturally occurring radioactive progeny from an environmental air filter. Following air collection, the filter was centre hole-punched with the transuranic check source placed underneath the filter during counting. With the surrogate transuranic activity introduced into the measurement, verification of the previously studied methodology for rapid transuranic activity estimation was determined with quantifiable conservative bias. 70 environmental filters with various levels of radon progeny and air sampling duration were collected; 35 examined with the 239Pu check source and 35 studied with the 230Th check source. To characterise the expected transuranic activity introduced to the counting experiment without the environmental interferents of radon and thoron progeny, 30 blank filters were counted using the described experimental setup with each of the respective surrogate sources. Following characterisation of the sources with blank filters, transuranic activity estimation comparison against the 70 environmental filters with natural background radioactive progeny interferents was accomplished. This work contributes to the comprehensive analysis of operational air samples by detailing validation results for a rapid and conservative transuranic alpha activity estimation methodology.