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Alternative Pathway to Double-Core-Hole States.
Ismail, Iyas; Ferté, Anthony; Penent, Francis; Guillemin, Renaud; Peng, Dawei; Marchenko, Tatiana; Travnikova, Oksana; Inhester, Ludger; Taïeb, Richard; Verma, Abhishek; Velasquez, Nicolas; Kukk, Edwin; Trinter, Florian; Koulentianos, Dimitris; Mazza, Tommaso; Baumann, Thomas M; Rivas, Daniel E; Ovcharenko, Yevheniy; Boll, Rebecca; Dold, Simon; De Fanis, Alberto; Ilchen, Markus; Meyer, Michael; Goldsztejn, Gildas; Li, Kai; Doumy, Gilles; Young, Linda; Sansone, Giuseppe; Dörner, Reinhard; Piancastelli, Maria Novella; Carniato, Stéphane; Bozek, John D; Püttner, Ralph; Simon, Marc.
Afiliação
  • Ismail I; Sorbonne Université, CNRS, Laboratoire de Chimie Physique-Matière et Rayonnement, LCPMR, F-75005 Paris Cedex 05, France.
  • Ferté A; Sorbonne Université, CNRS, Laboratoire de Chimie Physique-Matière et Rayonnement, LCPMR, F-75005 Paris Cedex 05, France.
  • Penent F; Sorbonne Université, CNRS, Laboratoire de Chimie Physique-Matière et Rayonnement, LCPMR, F-75005 Paris Cedex 05, France.
  • Guillemin R; Sorbonne Université, CNRS, Laboratoire de Chimie Physique-Matière et Rayonnement, LCPMR, F-75005 Paris Cedex 05, France.
  • Peng D; Sorbonne Université, CNRS, Laboratoire de Chimie Physique-Matière et Rayonnement, LCPMR, F-75005 Paris Cedex 05, France.
  • Marchenko T; European XFEL, Holzkoppel 4, 22869 Schenefeld, Germany.
  • Travnikova O; Sorbonne Université, CNRS, Laboratoire de Chimie Physique-Matière et Rayonnement, LCPMR, F-75005 Paris Cedex 05, France.
  • Inhester L; Sorbonne Université, CNRS, Laboratoire de Chimie Physique-Matière et Rayonnement, LCPMR, F-75005 Paris Cedex 05, France.
  • Taïeb R; Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY, Notkestraße 85, 22607 Hamburg, Germany.
  • Verma A; Sorbonne Université, CNRS, Laboratoire de Chimie Physique-Matière et Rayonnement, LCPMR, F-75005 Paris Cedex 05, France.
  • Velasquez N; Sorbonne Université, CNRS, Laboratoire de Chimie Physique-Matière et Rayonnement, LCPMR, F-75005 Paris Cedex 05, France.
  • Kukk E; Sorbonne Université, CNRS, Laboratoire de Chimie Physique-Matière et Rayonnement, LCPMR, F-75005 Paris Cedex 05, France.
  • Trinter F; Sorbonne Université, CNRS, Laboratoire de Chimie Physique-Matière et Rayonnement, LCPMR, F-75005 Paris Cedex 05, France.
  • Koulentianos D; Department of Physics and Astronomy, University of Turku, FI-20014 Turku, Finland.
  • Mazza T; Institut für Kernphysik, Goethe-Universität Frankfurt, Max-von-Laue-Straße 1, 60438 Frankfurt am Main, Germany.
  • Baumann TM; Molecular Physics, Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4-6, 14195 Berlin, Germany.
  • Rivas DE; Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY, Notkestraße 85, 22607 Hamburg, Germany.
  • Ovcharenko Y; Chemical Sciences and Engineering Division, Argonne National Laboratory, 9700 South Cass Avenue, Argonne, Illinois 60439, USA.
  • Boll R; Department of Physics, Universität Hamburg, Luruper Chaussee 149, 22761 Hamburg, Germany.
  • Dold S; European XFEL, Holzkoppel 4, 22869 Schenefeld, Germany.
  • De Fanis A; European XFEL, Holzkoppel 4, 22869 Schenefeld, Germany.
  • Ilchen M; European XFEL, Holzkoppel 4, 22869 Schenefeld, Germany.
  • Meyer M; European XFEL, Holzkoppel 4, 22869 Schenefeld, Germany.
  • Goldsztejn G; European XFEL, Holzkoppel 4, 22869 Schenefeld, Germany.
  • Li K; European XFEL, Holzkoppel 4, 22869 Schenefeld, Germany.
  • Doumy G; European XFEL, Holzkoppel 4, 22869 Schenefeld, Germany.
  • Young L; European XFEL, Holzkoppel 4, 22869 Schenefeld, Germany.
  • Sansone G; European XFEL, Holzkoppel 4, 22869 Schenefeld, Germany.
  • Dörner R; Université Paris-Saclay, Institut des Sciences Moléculaires d'Orsay ISMO, UMR CNRS 8214, F-91405 Orsay, France.
  • Piancastelli MN; Chemical Sciences and Engineering Division, Argonne National Laboratory, 9700 South Cass Avenue, Argonne, Illinois 60439, USA.
  • Carniato S; Chemical Sciences and Engineering Division, Argonne National Laboratory, 9700 South Cass Avenue, Argonne, Illinois 60439, USA.
  • Bozek JD; Chemical Sciences and Engineering Division, Argonne National Laboratory, 9700 South Cass Avenue, Argonne, Illinois 60439, USA.
  • Püttner R; Department of Physics and James Franck Institute, The University of Chicago, Chicago, Illinois, USA.
  • Simon M; Institute of Physics, University of Freiburg, Hermann-Herder-Straße 3, 79104 Freiburg, Germany.
Phys Rev Lett ; 131(25): 253201, 2023 Dec 22.
Article em En | MEDLINE | ID: mdl-38181353
ABSTRACT
Excited double-core-hole states of isolated water molecules resulting from the sequential absorption of two x-ray photons have been investigated. These states are formed through an alternative pathway, where the initial step of core ionization is accompanied by the shake-up of a valence electron, leading to the same final states as in the core-ionization followed by core-excitation pathway. The capability of the x-ray free-electron laser to deliver very intense, very short, and tunable light pulses is fully exploited to identify the two different pathways.

Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Revista: Phys Rev Lett Ano de publicação: 2023 Tipo de documento: Article País de afiliação: França

Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Revista: Phys Rev Lett Ano de publicação: 2023 Tipo de documento: Article País de afiliação: França