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1.
Nature ; 614(7948): 440-444, 2023 02.
Artigo em Inglês | MEDLINE | ID: mdl-36792742

RESUMO

In a flat band superconductor, the charge carriers' group velocity vF is extremely slow. Superconductivity therein is particularly intriguing, being related to the long-standing mysteries of high-temperature superconductors1 and heavy-fermion systems2. Yet the emergence of superconductivity in flat bands would appear paradoxical, as a small vF in the conventional Bardeen-Cooper-Schrieffer theory implies vanishing coherence length, superfluid stiffness and critical current. Here, using twisted bilayer graphene3-7, we explore the profound effect of vanishingly small velocity in a superconducting Dirac flat band system8-13. Using Schwinger-limited non-linear transport studies14,15, we demonstrate an extremely slow normal state drift velocity vn ≈ 1,000 m s-1 for filling fraction ν between -1/2 and -3/4 of the moiré superlattice. In the superconducting state, the same velocity limit constitutes a new limiting mechanism for the critical current, analogous to a relativistic superfluid16. Importantly, our measurement of superfluid stiffness, which controls the superconductor's electrodynamic response, shows that it is not dominated by the kinetic energy but instead by the interaction-driven superconducting gap, consistent with recent theories on a quantum geometric contribution8-12. We find evidence for small Cooper pairs, characteristic of the Bardeen-Cooper-Schrieffer to Bose-Einstein condensation crossover17-19, with an unprecedented ratio of the superconducting transition temperature to the Fermi temperature exceeding unity and discuss how this arises for ultra-strong coupling superconductivity in ultra-flat Dirac bands.

2.
Nano Lett ; 22(13): 5094-5099, 2022 Jul 13.
Artigo em Inglês | MEDLINE | ID: mdl-35715214

RESUMO

Conventionally, magnetism arises from the strong exchange interaction among the magnetic moments of d- or f-shell electrons. It can also emerge in perfect lattices from nonmagnetic elements, such as that exemplified by the Stoner criterion. Here we report tunable magnetism in suspended rhombohedral-stacked few-layer graphene (r-FLG) devices with flat bands. At small doping levels (n ∼ 1011 cm-2), we observe prominent conductance hysteresis and giant magnetoconductance that exceeds 1000% as a function of magnetic fields. Both phenomena are tunable by density and temperature and disappear at n > 1012 cm-2 or T > 5 K. These results are confirmed by first-principles calculations, which indicate the formation of a half-metallic state in doped r-FLG, in which the magnetization is tunable by electric field. Our combined experimental and theoretical work demonstrate that magnetism and spin polarization, arising from the strong electronic interactions in flat bands, emerge in a system composed entirely of carbon atoms.

3.
Nanoscale ; 12(46): 23488-23496, 2020 Dec 08.
Artigo em Inglês | MEDLINE | ID: mdl-33211783

RESUMO

Indium Selenide (In2Se3) is a newly emerged van der Waals (vdW) ferroelectric material, which unlike traditional insulating ferroelectric materials, is a semiconductor with a bandgap of about 1.36 eV. Ferroelectric diodes and transistors based on In2Se3 have been demonstrated. However, the interplay between light and electric polarization in In2Se3 has not been explored. In this paper, we found that the polarization in In2Se3 can be programmed by optical stimuli, due to its semiconducting nature, where the photo generated carriers in In2Se3 can alter the screening field and lead to polarization reversal. Utilizing these unique properties of In2Se3, we demonstrated a new type of multifunctional device based on 2D heterostructures, which can concurrently serve as a logic gate, photodetector, electronic memory and photonic memory. This dual electrical and optical operation of the memories can simplify the device architecture and offer additional functionalities, such as ultrafast optical erase of large memory arrays. In addition, we show that dual-gate structure can address the partial switching problem commonly observed in In2Se3 ferroelectric transistors, as the two gates can enhance the vertical electric field and facilitate the polarization switching in the semiconducting In2Se3. These discovered effects are of general nature and should be observable in any ferroelectric semiconductor. These findings deepen the understanding of polarization switching and light-polarization interaction in semiconducting ferroelectric materials and open up their applications in multifunctional electronic and photonic devices.

4.
J Phys Condens Matter ; 32(12): 12LT01, 2020 Mar 20.
Artigo em Inglês | MEDLINE | ID: mdl-31778977

RESUMO

Topological semimetal (TSM) AuTe2Br thin flakes have been studied by Raman spectroscopy and magneto-transport measurement. The angle-resolved polarized Raman spectrum of AuTe2Br (bulk and thin flake) shows strong anisotropy. Together with high resolution transmission electron microscopy (TEM), we establish a non-destructive method to determine the crystallographic orientation of AuTe2Br flakes. At high temperature (T > 50 K), the magneto-resistance (MR) of AuTe2Br thin flakes shows typical parabolic-like behavior, which can be well fitted by the two-fluid model. However, at low temperature (T ⩽ 30 K), the MR of thin flakes (<17 nm) clearly deviates from the two-fluid model as well as from the Kohler's rule, suggesting a new type of scattering emerging below 30 K. Several possible scattering mechanisms are discussed and the respective corrections to MR are compared with our experimental data. In addition, the conductivity of these metallic crystals is also found to be highly anisotropic, with the hole mobility along the a axis about five times higher than that along the c axis.

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