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1.
Phys Rev Lett ; 117(14): 147001, 2016 Sep 30.
Artigo em Inglês | MEDLINE | ID: mdl-27740782

RESUMO

We investigate transport and shot noise in lateral normal-metal-3D topological-insulator-superconductor contacts, where the 3D topological insulator (TI) is based on Bi. In the normal state, the devices are in the elastic diffusive transport regime, as demonstrated by a nearly universal value of the shot noise Fano factor F_{N}≈1/3 in magnetic field and in a reference normal-metal contact. In the absence of magnetic field, we identify the Andreev reflection (AR) regime, which gives rise to the effective charge doubling in shot noise measurements. Surprisingly, the Fano factor F_{AR}≈0.22±0.02 is considerably reduced in the AR regime compared to F_{N}, in contrast to previous AR experiments in normal metals and semiconductors. We suggest that this effect is related to a finite thermal conduction of the proximized, superconducting TI owing to a residual density of states at low energies.

2.
Nat Mater ; 12(10): 882-6, 2013 Oct.
Artigo em Inglês | MEDLINE | ID: mdl-23892787

RESUMO

As the oldest known magnetic material, magnetite (Fe3O4) has fascinated mankind for millennia. As the first oxide in which a relationship between electrical conductivity and fluctuating/localized electronic order was shown, magnetite represents a model system for understanding correlated oxides in general. Nevertheless, the exact mechanism of the insulator-metal, or Verwey, transition has long remained inaccessible. Recently, three-Fe-site lattice distortions called trimerons were identified as the characteristic building blocks of the low-temperature insulating electronically ordered phase. Here we investigate the Verwey transition with pump-probe X-ray diffraction and optical reflectivity techniques, and show how trimerons become mobile across the insulator-metal transition. We find this to be a two-step process. After an initial 300 fs destruction of individual trimerons, phase separation occurs on a 1.5±0.2 ps timescale to yield residual insulating and metallic regions. This work establishes the speed limit for switching in future oxide electronics.

3.
Nat Commun ; 15(1): 4581, 2024 May 29.
Artigo em Inglês | MEDLINE | ID: mdl-38811546

RESUMO

The anomalous strange metal phase found in high-Tc cuprates does not follow the conventional condensed-matter principles enshrined in the Fermi liquid and presents a great challenge for theory. Highly precise experimental determination of the electronic self-energy can provide a test bed for theoretical models of strange metals, and angle-resolved photoemission can provide this as a function of frequency, momentum, temperature and doping. Here we show that constant energy cuts through the nodal spectral function in (Pb,Bi)2Sr2-xLaxCuO6+δ have a non-Lorentzian lineshape, consistent with a self-energy that is k dependent. This provides a new test for aspiring theories. Here we show that the experimental data are captured remarkably well by a power law with a k-dependent scaling exponent smoothly evolving with doping, a description that emerges naturally from anti-de Sitter/conformal-field-theory based semi-holography. This puts a spotlight on holographic methods for the quantitative modelling of strongly interacting quantum materials like the cuprate strange metals.

4.
Phys Rev Lett ; 108(5): 057001, 2012 Feb 03.
Artigo em Inglês | MEDLINE | ID: mdl-22400952

RESUMO

We report a high-pressure single crystal study of the topological superconductor Cu{x}Bi{2}Se{3}. Resistivity measurements under pressure show superconductivity is depressed smoothly. At the same time the metallic behavior is gradually lost. The upper-critical field data B{c2}(T) under pressure collapse onto a universal curve. The absence of Pauli limiting and the comparison of B{c2}(T) to a polar-state function point to spin-triplet superconductivity, but an anisotropic spin-singlet state cannot be discarded completely.

5.
Phys Rev Lett ; 109(12): 127001, 2012 Sep 21.
Artigo em Inglês | MEDLINE | ID: mdl-23005977

RESUMO

We establish in a combination of ab initio theory and experiments that the tunneling process in scanning tunneling microscopy or spectroscopy on the A-122 iron pnictide superconductors-in this case BaFe(2-x)Co(x)As(2)-involves a strong adatom filtering of the differential conductance from the near-E(F) Fe-3d states, which in turn originates from the topmost subsurface Fe layer of the crystal. The calculations show that the dominance of surface Ba-related tunneling pathways leaves fingerprints found in the experimental differential conductance data, including large particle-hole asymmetry and energy-dependent contrast inversion in conductance maps.

6.
Nat Commun ; 10(1): 1618, 2019 04 03.
Artigo em Inglês | MEDLINE | ID: mdl-30944326

RESUMO

The original version of this Article contained an error in the right-hand y-axis of Fig. 2c, which incorrectly read 'S/2e (pA)'. The correct version states 'nA' in place of 'pA'. This has been corrected in both the PDF and HTML versions of the Article.

7.
Nat Commun ; 10(1): 544, 2019 02 01.
Artigo em Inglês | MEDLINE | ID: mdl-30710086

RESUMO

Dopants and impurities are crucial in shaping the ground state of host materials: semiconducting technology is based on their ability to donate or trap electrons, and they can even be used to transform insulators into high temperature superconductors. Due to limited time resolution, most atomic-scale studies of the latter materials focussed on the effect of dopants on the electronic properties averaged over time. Here, by using atomic-scale current-noise measurements in optimally doped Bi2Sr2CaCu2O8+x, we visualize sub-nanometre sized objects where the tunnelling current-noise is enhanced by at least an order of magnitude. We show that these objects are previously undetected oxygen dopants whose ionization and local environment leads to unconventional charge dynamics resulting in correlated tunnelling events. The ionization of these dopants opens up new routes to dynamically control doping at the atomic scale, enabling the direct visualization of local charging on e.g. high-Tc superconductivity.

8.
Sci Rep ; 5: 16309, 2015 Nov 06.
Artigo em Inglês | MEDLINE | ID: mdl-26543011

RESUMO

In an ideal 3D topological insulator (TI), the bulk is insulating and the surface conducting due to the existence of metallic states that are localized on the surface; these are the topological surface states. Quaternary Bi-based compounds of Bi(2-x)Sb(x)Te(3-y)Se(y) with finely-tuned bulk stoichiometries are good candidates for realizing ideal 3D TI behavior due to their bulk insulating character. However, despite its insulating bulk in transport experiments, the surface region of Bi(2-x)Sb(x)Te(3-y)Se(y) crystals cleaved in ultrahigh vacuum also exhibits occupied states originating from the bulk conduction band. This is due to adsorbate-induced downward band-bending, a phenomenon known from other Bi-based 3D TIs. Here we show, using angle-resolved photoemission, how an EUV light beam of moderate flux can be used to exclude these topologically trivial states from the Fermi level of Bi1.46Sb0.54Te1.7Se1.3 single crystals, thereby re-establishing the purely topological character of the low lying electronic states of the system. We furthermore prove that this process is highly local in nature in this bulk-insulating TI, and are thus able to imprint structures in the spatial energy landscape at the surface. We illustrate this by 'writing' micron-sized letters in the Dirac point energy of the system.

10.
Phys Rev Lett ; 96(10): 107007, 2006 Mar 17.
Artigo em Inglês | MEDLINE | ID: mdl-16605782

RESUMO

By combining surprising new results from a full polarization analysis of nodal angle-resolved photoemission data from pristine and modulation-free Bi(2)Sr(2)CaCu(2)O(8+delta) with structural information from LEED and ab initio one-step photoemission simulations, we prove that the shadow Fermi surface in these systems is of structural origin, being due to orthorhombic distortions from tetragonal symmetry present both in surface and bulk. Consequently, one of the longest standing open issues in the investigation of the Fermi surface of these widely studied systems finally meets its resolution.

11.
J Healthc Risk Manag ; 18(2): 18-26, 1998.
Artigo em Inglês | MEDLINE | ID: mdl-10185074

RESUMO

Many healthcare organizations maintain two systems for documenting incidents reports: A paper incident report system completed by staff and managers and A computerized system where clerical staff duplicate the same information in a database. This article discusses the way risk managers in hospitals and healthcare organizations can reduce paperwork and more rapidly address the implementation of a point of service computerized system to document incidents. The benefits of such a system include: Real-time information and trending of occurrences. Reduced liability by securing reports earlier. Maintaining a higher level of confidentiality. Earlier problem resolution. Providing a valuable link between the risk, quality, and safety functions of the organization.


Assuntos
Sistemas de Informação Hospitalar , Erros Médicos , Sistemas Automatizados de Assistência Junto ao Leito , Gestão de Riscos/métodos , Sistemas de Notificação de Reações Adversas a Medicamentos , Confidencialidade , Controle de Formulários e Registros , Humanos , Satisfação do Paciente , Software , Estados Unidos
12.
N Engl J Med ; 303(16): 897-902, 1980 Oct 16.
Artigo em Inglês | MEDLINE | ID: mdl-7412821

RESUMO

To define the prevalence of total coronary occlusion in the hours after transmural myocardial infarction, we used coronary arteriography to study the degree of coronary obstruction in 322 patients admitted within 24 hours of infarction. Total coronary occlusion was observed in 110 of 126 patients (87 per cent) who were evaluated within four hours of the onset of symptoms; this proportion decreased significantly, to 37 of 57 (65 per cent), when patients were studied 12 to 24 hours after the onset of symptoms. Among 59 patients with angiographic features of coronary thrombosis, the thrombus was retrieved by Fogarty catheter in 52 (88 per cent) but was absent in seven (12 per cent false positive). Among an additional 20 patients without angiographic features of thrombosis, a thrombus was discovered in five (25 per cent false negative). Thus, total coronary occlusion is frequent during the early hours of transmural infarction and decreases in frequency during the initial 24 hours, suggesting that coronary spasm or thrombus formation with subsequent recanalization or both may be important in the evolution of infarction.


Assuntos
Angiografia , Angiografia Coronária , Circulação Coronária , Infarto do Miocárdio/fisiopatologia , Adulto , Idoso , Arritmias Cardíacas/etiologia , Cateterismo Cardíaco , Doença das Coronárias/diagnóstico , Doença das Coronárias/diagnóstico por imagem , Feminino , Hospitalização , Humanos , Masculino , Pessoa de Meia-Idade , Infarto do Miocárdio/diagnóstico , Infarto do Miocárdio/diagnóstico por imagem , Infarto do Miocárdio/etiologia , Estudos Prospectivos , Choque Cardiogênico/etiologia , Fatores de Tempo
13.
Phys Rev Lett ; 90(20): 207001, 2003 May 23.
Artigo em Inglês | MEDLINE | ID: mdl-12785915

RESUMO

High-resolution angle-resolved photoemission with variable excitation energies is used to disentangle bilayer splitting effects and intrinsic (self-energy) effects in the electronic spectral function near the (pi,0) point of differently doped (Pb,Bi)(2)Sr(2)CaCu(2)O(8+delta). In contrast to overdoped samples, where intrinsic effects at the (pi,0) point are virtually absent, we find in underdoped samples intrinsic effects in the superconducting-state (pi,0) spectra of the antibonding band. This intrinsic effect is present only below the critical temperature and weakens considerably with doping. Our results give strong support for models which involve a strong coupling of electronic excitations with the resonance mode seen in inelastic neutron scattering experiments.

14.
Phys Rev Lett ; 89(7): 077003, 2002 Aug 12.
Artigo em Inglês | MEDLINE | ID: mdl-12190550

RESUMO

From detailed high-resolution measurements of the photon energy dependence of the (pi,0) superconducting-state photoemission spectrum of the bilayer Bi high-temperature superconductors, we show that the famous peak-dip-hump line shape is dominated by a superposition of spectral features originating from different electronic states which reside at different binding energies, but are each describable by essentially identical single-particle spectral functions. The previously identified bilayer-split CuO2 bands are the culprit: with the "superconducting" peak being due to the antibonding band, while the hump is mainly formed by its bonding bilayer-split counterpart.

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