Watt-level tunable Ti:Sapphire laser directly pumped with green laser diodes.

We demonstrate a Ti:Sapphire laser generating in excess of 1.2 W in continuous-wave operation when pumped directly with four green laser diodes eliminating the need for a complex pump laser. As a result, improvement of laser efficiency is achieved without sacrificing beam quality. Tunability within the range of 740-840 nm is attained validating the concept of a direct laser-diode pumped Ti:Sapphire laser.

450†W pulsed laser system with M2 < 1.2 based on a 969-nm laser diode end-pumped Yb:YAG rod amplifier.

We demonstrated a compact and power-efficient multi-stage pulsed end-pumped amplifier with stabilized output power of 450 W and near-diffraction-limited beam quality (M2 < 1.2) at a repetition rate of 1 MHz. The pulsed amplifier produced an exceptional average power and optimal beam quality achieved in laser diode (LD) end-pumped Yb:YAG thin rod configuration at room temperature. A preliminary pulse compression with a chirped volume Bragg grating (CVBG) was performed reducing pulse duration to ∼730 fs at a compression efficiency of 90%. With the combined features, including compactness, reliability, and efficiency, of the end-pumped scheme, the demonstrated laser system would be of great value in both industry and scientific research.

589†nm yellow laser pumped Kerr-lens mode-locked Alexandrite laser producing sub-50†fs pulses.

We report a femtosecond Kerr-lens mode-locked (KLM) Alexandrite laser resonantly pumped by a 589 nm yellow laser. The 4 nJ pulses as short as 42 fs were obtained corresponding to a peak power of 100 kW. With the repetition rate of 104 MHz, the average power of 420 mW was attained. The time-bandwidth product of generated laser pulse was measured to be 0.324 with a beam quality factor of M2 ≤ 1.13. The exceptional performance of visible femtosecond laser may find potential applications in various fields.

Atomic-Void van der Waals Channel Waveguides.

Layered van der Waals materials allow creating unique atomic-void channels with subnanometer dimensions. Coupling light into these channels may further advance sensing, quantum information, and single molecule chemistries. Here, we examine theoretically limits of light guiding in atomic-void channels and show that van der Waals materials exhibiting strong resonances, excitonic and polaritonic, are ideally suited for deeply subwavelength light guiding. We predict that excitonic transition metal dichalcogenides can squeeze >70% of optical power in just <λ/100 thick channel in the visible and near-infrared. We also show that polariton resonances of hexagonal boron nitride allow deeply subwavelength (<λ/500) guiding in the mid-infrared. We further reveal effects of natural material anisotropy and discuss the influence of losses. Such van der Waals channel waveguides while offering extreme optical confinement exhibit significantly lower loss compared to plasmonic counterparts, thus paving the way to low-loss and deeply subwavelength optics.

The Role of Epsilon Near Zero and Hot Electrons in Enhanced Dynamic THz Emission from Nonlinear Metasurfaces.

We study theoretically and experimentally the nonlinear THz emission from plasmonic metasurfaces and show that a thin indium-tin oxide (ITO) film significantly affects the nonlinear dynamics of the system. Specifically, the presence of the ITO film leads to 2 orders of magnitude stronger THz emission compared to a metasurface on glass. It also shows a different power law, signifying different dominant emission mechanisms. In addition, we find that the hot-electron dynamics in the system strongly modify the coupling between the plasmonic metasurface and the free electrons in the ITO at the picosecond time scale. This results in striking dynamic THz emission phenomena that were not observed to date. Specifically, we show that the generated THz pulse can be shortened in time and thus broadened in frequency with twice the bandwidth compared to previous studies and to an uncoupled system. Our findings open the door to design efficient and dynamic metasurface THz emitters.

Electrical control of all-optical graphene switches.

Graphene has emerged as an ultrafast photonic material for on-chip all-optical switching applications. However, its atomic thickness limits its interaction with guided optical modes, resulting in a high switching energy per bit. Herein, we propose a novel technique to electrically control the switching energy of an all-optical graphene switch on a silicon nitride waveguide. Using this technique, we theoretically demonstrate a 120 µm long all-optical graphene switch with an 8.9 dB extinction ratio, 2.4 dB insertion loss, a switching time of <100 fs, a fall time of <5 ps, and a 235 fJ switching energy at 2.5 V bias, where the applied voltage reduces the switching energy by ∼16×. This technique paves the way for the emergence of ultra-efficient all-optical graphene switches that will meet the energy demands of next-generation photonic computing systems, and it is a promising alternative to lossy plasmon-enhanced devices.

On-chip low-loss all-optical MoSe2 modulator.

Monolayer transition metal dichalcogenides (TMDCs), like MoS2, MoSe2, WS2, and WSe2, feature direct bandgaps, strong spin-orbit coupling, and exciton-polariton interactions at the atomic scale, which could be harnessed for efficient light emission, valleytronics, and polaritonic lasing, respectively. Nevertheless, to build next-generation photonic devices that make use of these features, it is first essential to model the all-optical control mechanisms in TMDCs. Herein, a simple model is proposed to quantify the performance of a 35-µm-long Si3N4 waveguide-integrated all-optical MoSe2 modulator. Using this model, a switching energy of 14.6 pJ is obtained for a transverse-magnetic (TM) and transverse-electric (TE) polarized pump signals at λ = 480 nm. Moreover, maximal extinction ratios of 20.6 dB and 20.1 dB are achieved for a TM and TE polarized probe signal, respectively, at λ = 500 nm with an ultra-low insertion loss of <0.3 dB. Moreover, the device operates with an ultrafast recovery time of 50 ps, while maintaining a high extinction ratio for practical applications. These findings facilitate modeling and designing novel TMDC-based photonic devices.

All-optical linearized Mach-Zehnder modulator.

A practical, broadband, all-optical linearization concept for a Mach-Zehnder modulator (MZM) is proposed and demonstrated. The unique transmitter design includes an amplitude modulated (AM) standard MZM with two optical outputs, where the alternative (or complimentary) output is combined with the laser carrier to create a linearizing optical local oscillator, which when coherently combined with the AM signal fully cancels 3rd order intermodulation distortion components. Using this scheme, record linearity is achieved for a non-amplified RF photonic link, with spurious free dynamic range (SFDR) of 118.5 dB.Hz2/3 and 123 dB.Hz2/3 for single and dual fiber/photodetector schemes.

Mitigating offset frequency drift in frequency combs using a customized power law dispersion.

We introduce a new, to the best of our knowledge, passive technique of mitigating the phase noise in optical frequency combs (FC) by reducing the drift of offset frequency. This can be achieved by customizing the dispersion to attain a power law dependence of the wave vector on frequency, k(ω)∼ωα, ensuring a constant ratio between group and phase velocities. When this condition is maintained, the drift offset frequency is passively mitigated, and phase noise is reduced. Using quantum cascade laser (QCL) FCs as an example, we demonstrate, analytically and numerically, that the desired dispersion can be easily engineered by properly adjusting the thickness of the QCL active region and that stable offset frequency can be combined with low residual group dispersion.

Role of surface passivation in integrated sub-bandgap silicon photodetection.

We study experimentally the effect of oxide removal on the sub-bandgap photodetection in silicon waveguides at the telecom wavelength regime. Depassivating the device allows for the enhancement of the quantum efficiency by about 2-3 times. Furthermore, the propagation loss within the device is significantly reduced by the oxide removal. Measuring the device 60 days after the depassivation shows slight differences. We provide a possible explanation for these observations. Clearly, passivation and depassivation play an essential role in the design and the implementation of such sub-bandgap photodetector devices for applications such as on-chip light monitoring.

Reversible MoS2 Origami with Spatially Resolved and Reconfigurable Photosensitivity.

Two-dimensional layered materials (2DLMs) have been extensively studied in a variety of planar optoelectronic devices. Three-dimensional (3D) optoelectronic structures offer unique advantages including omnidirectional responses, multipolar detection, and enhanced light-matter interactions. However, there has been limited success in transforming monolayer 2DLMs into reconfigurable 3D optoelectronic devices due to challenges in microfabrication and integration of these materials in truly 3D geometries. Here, we report an origami-inspired self-folding approach to reversibly transform monolayer molybdenum disulfide (MoS2) into functional 3D optoelectronic devices. We pattern and integrate monolayer MoS2 and gold (Au) onto differentially photo-cross-linked thin polymer (SU8) films. The devices reversibly self-fold due to swelling gradients in the SU8 films upon solvent exchange. We fabricate a wide variety of optically active 3D MoS2 microstructures including pyramids, cubes, flowers, dodecahedra, and Miura-oris, and we simulate the self-folding mechanism using a coarse-grained mechanics model. Using finite-difference time-domain (FDTD) simulation and optoelectronic characterization, we demonstrate that the 3D self-folded MoS2 structures show enhanced light interaction and are capable of angle-resolved photodetection. Importantly, the structures are also reversibly reconfigurable upon solvent exchange with high tunability in the optical detection area. Our approach provides a versatile strategy to reversibly configure 2D materials in 3D optoelectronic devices of broad relevance to flexible and wearable electronics, biosensing, and robotics.

Hot carriers generated by plasmons: where are they generated and where do they go from there?

A physically transparent unified theory of optically- and plasmon-induced hot carrier generation in metals is developed with all of the relevant mechanisms included. Analytical expressions that estimate the carrier generation rates and their locations, energies and directions of motion are obtained. Among the four mechanisms considered: interband absorption, phonon and defect assisted absorption, electron-electron scattering assisted absorption and surface-collision assisted absorption (Landau damping), it is the last one that generates hot carriers, which are most useful for practical applications in photodetection and photocatalysis.

Plasmonic Hot Carriers-Controlled Second Harmonic Generation in WSe2 Bilayers.

Modulating second harmonic generation (SHG) by a static electric field through either electric-field-induced SHG or charge-induced SHG has been well documented. Nonetheless, it is essential to develop the ability to dynamically control and manipulate the nonlinear properties, preferably at high speed. Plasmonic hot carriers can be resonantly excited in metal nanoparticles and then injected into semiconductors within 10-100 fs, where they eventually decay on a comparable time scale. This allows one to rapidly manipulate all kinds of characteristics of semiconductors, including their nonlinear properties. Here we demonstrate that plasmonically generated hot electrons can be injected from plasmonic nanostructure into bilayer (2L) tungsten diselenide (WSe2), breaking the material inversion symmetry and thus inducing an SHG. With a set of pump-probe experiments we confirm that it is the dynamic separation electric field resulting from the hot carrier injection (rather than a simple optical field enhancement) that is the cause of SHG. Transient absorption measurement further substantiate the plasmonic hot electrons injection and allow us to measure a rise time of ∼120 fs and a fall time of 1.9 ps. Our study creates opportunity for the ultrafast all-optical control of SHG in an all-optical manner that may enable a variety of applications.

Excitonic Emission of Monolayer Semiconductors Near-Field Coupled to High-Q Microresonators.

We present quantum yield measurements of single layer WSe2 (1L-WSe2) integrated with high-Q ( Q > 106) optical microdisk cavities, using an efficient (η > 90%) near-field coupling scheme based on a tapered optical fiber. Coupling of the excitonic emission is achieved by placing 1L-WSe2 in the evanescent cavity field. This preserves the microresonator high intrinsic quality factor ( Q > 106) below the bandgap of 1L-WSe2. The cavity quantum yield is QYc ≈ 10-3, consistent with operation in the broad emitter regime (i.e., the emission lifetime of 1L-WSe2 is significantly shorter than the bare cavity decay time). This scheme can serve as a precise measurement tool for the excitonic emission of layered materials into cavity modes, for both in plane and out of plane excitation.

Time, space, and spectral multiplexing for radiation balanced operation of semiconductor lasers.

Radiation balanced lasing (RBL) is an attractive pathway towards the development of high power and good beam quality lasers because heat removal via anti-Stokes luminescence (optical refrigeration) does not require additional connections and components and the heat is dissipated away from the active medium. Optical refrigeration had been demonstrated in the rare-earth doped laser medium but is far more difficult to achieve it in semiconductors laser medium. The main obstacle to achieve RBL in semiconductors is that the most efficient cooling occurs at relatively low carrier densities, while the gain required to sustain laser operation occurs at much higher densities. In this study, we explore the means of resolving this conundrum by separating the optical refrigeration and lasing in temporal, spatial, and/or spectral domains. Time multiplexing involves modulating the pump and operating the laser in pulse modes with lasing and cooling intervals. Space multiplexing involves having separate regions (quantum wells and dots) for lasing and cooling. The spectral multiplexing involves operating with two separate pumps - one for lasing and one for cooling. These methods will be compared in the study with the goal of selecting the optimal path RBL in semiconductor lasers.

Bandgap engineering and prospects for radiation-balanced vertical-external-cavity surface-emitting semiconductor lasers.

The vertical-external-cavity surface-emitting laser (VECSEL) has shown promise in becoming an efficient source of high power and high beam quality coherent radiation. In order to live up to its true potential, the VECSEL must be thermally managed in order to avoid thermal damage as thermal lensing and filamentation causing preventing it from operating in a single mode regime. For an optically pumped VECSEL, optical cooling presents an elegant solution for thermal management as it does not require electrical or thermal conduction. The goal of optical refrigeration is to achieve radiation balance lasing (RBL) when the active medium is maintained at a steady uniform temperature. In this work, we investigate the active medium characteristics and operating conditions that can lead to RBL in a semiconductor medium and show that to achieve RBL, the gain medium should be engineered to create a density of states that simultaneously allows gain and strong anti-Stokes luminescence. Such a medium may incorporate bandtail states, impurities or quantum dots. We provide a recipe for optimization of such band structure-engineered materials to achieve the lowest threshold and highest output power.

Waveguide-based electro-absorption modulator performance: comparative analysis.

Electro-optic modulators perform a key function for data processing and communication. Rapid growth in data volume and increasing bits per second rates demand increased transmitter and thus modulator performance. Recent years have seen the introduction of new materials and modulator designs to include polaritonic optical modes aimed at achieving advanced performance in terms of speed, energy efficiency, and footprint. Such ad hoc modulator designs, however, leave a universal design for these novel material classes of devices missing. Here we execute a holistic performance analysis for waveguide-based electro-absorption modulators and use the performance metric switching energy per unit bandwidth (speed). We show that the performance is fundamentally determined by the ratio of the differential absorption cross-section of the switching material's broadening and the waveguide effective mode area. We find that the former shows highest performance for a broad class of materials relying on Pauli-blocking (absorption saturation), such as semiconductor quantum wells, quantum dots, graphene, and other 2D materials, but is quite similar amongst these classes. In this respect these materials are clearly superior to those relying on free carrier absorption, such as Si and ITO. The performance improvement on the material side is fundamentally limited by the oscillator sum rule and thermal broadening of the Fermi-Dirac distribution. We also find that performance scales with modal waveguide confinement. Thus, we find highest energy-bandwidth-ratio modulator designs to be graphene, QD, QW, or 2D material-based plasmonic slot waveguides where the electric field is in-plane with the switching material dimension. We show that this improvement always comes at the expense of increased insertion loss. Incorporating fundamental device physics, design trade-offs, and resulting performance, this analysis aims to guide future experimental modulator explorations.

Temporal characteristics of quantum cascade laser frequency modulated combs in long wave infrared and THz regions.

We consider here a time domain model representing the dynamics of quantum cascade lasers (QCLs) generating frequency combs (FCs) in both THz and long wave infrared (LWIR λ = 8-12µm) spectral ranges. Using common specifications for these QCLs we confirm that the free running laser enters a regime of operation yielding a pseudo-randomly frequency modulated (FM) radiation in the time domain corresponding to FCs with stable phase relations in the frequency domain. We provide an explanation for this unusual behavior as a consequence of competition for the most efficient regime of operation. Expanding the model previously developed in [Opt. Eng. 57(1), 011009 (2017)] we analyze the performance of realistic THz and LWIR QCLs and show, despite the vastly different scale of many parameters, that both types of lasers offer very similar characteristics, namely FM operation with an FM period commensurate with the gain recovery time and an FM amplitude comparable with the gain bandwidth. We also identify the true culprit behind pseudo-random dynamics of the FM comb to be spatial hole burning, rather than the more pervasive spectral hole burning.

Sub-wavelength field enhancement in the mid-IR: photonics versus plasmonics versus phononics.

The ability to concentrate the electrical field into sub-wavelength volumes is a key benefit sought and, to a certain degree, found within the discipline of plasmonics. This ability is restricted only by the ohmic loss in noble metals and, recently, in the infrared region, metals are beginning to face a challenge from emerging alternative media: phononic (i.e., relying on surface phonon polaritons) and photonic (i.e., relying on high refractive index) all-dielectric structures, and highly doped semiconductors, all of them having smaller intrinsic loss than metals. In this Letter, we compare the degree of enhancement and its spectral selectivity for different media and confirm that, while one can obtain sharper resonant features with all-dielectric structures, the magnitude of the field enhancement is invariably higher with metals such as gold and copper, primarily due to a higher density of electrons. On the whole, depending on the application, metals and dielectrics have their own unique advantages.

Attojoule-efficient graphene optical modulators.

Electro-optic modulation is a technology-relevant function for signal keying, beam steering, or neuromorphic computing through providing the nonlinear activation function of a perceptron. With silicon-based modulators being bulky and inefficient, here we discuss graphene-based devices heterogeneously integrated. This study provides a critical and encompassing discussion of the physics and performance of graphene. We provide a holistic analysis of the underlying physics of modulators including graphene's index tunability, the underlying optical mode, and discuss resulting performance vectors for this novel class of hybrid modulators. Our results show that reducing the modal area and reducing the effective broadening of the active material are key to improving device performance defined by the ratio of energy-bandwidth and footprint. We further show how the waveguide's polarization must be in-plane with graphene, such as given by plasmonic-slot structures, for performance improvements. A high device performance can be obtained by introducing multi- or bi-layer graphene modulator designs. Lastly, we present recent results of a graphene-based hybrid-photon-plasmon modulator on a silicon platform and discuss electron beam lithography treatments for transferred graphene for the relevant Fermi level tuning. Being physically compact, this 100 aJ/bit modulator opens the path towards a novel class of attojoule efficient opto-electronics.