Establishing the fundamental magnetic interactions in the chiral Skyrmionic Mott insulator Cu(2)OSeO(3) by terahertz electron spin resonance.

The recent discovery of Skyrmions in Cu(2)OSeO(3) has established a new platform to create and manipulate Skyrmionic spin textures. We use high-field electron spin resonance with a terahertz free-electron laser and pulsed magnetic fields up to 64 T to probe and quantify its microscopic spin-spin interactions. In addition to the previously observed long-wavelength Goldstone mode, this technique probes also the high-energy part of the excitation spectrum which is inaccessible by standard low-frequency electron spin resonance. Fitting the behavior of the observed modes in magnetic field to a theoretical framework establishes experimentally that the fundamental magnetic building blocks of this Skyrmionic magnet are rigid, highly entangled and weakly coupled tetrahedra.

Nanosecond pulses in a THz gyrotron oscillator operating in a mode-locked self-consistent Q-switch regime.

An experimental study of a nanosecond pulsed regime in a THz gyrotron oscillator operating in a self-consistent Q-switch regime has been carried out. The gyrotron is operated in the TE(7,2) transverse mode radiating at a frequency of 260.5 GHz. The 5 W nanosecond pulses are obtained in a self-consistent Q-switch regime in which the cavity diffraction quality factor dynamically varies by nearly 2 orders of magnitude on a subnanosecond time scale via the nonlinear interaction of different mode-locked frequency-equidistant sidebands. The experimental results are in good agreement with numerical simulations performed with the TWANG code based on a slow time scale formulation of the self-consistent time-dependent nonlinear wave particle interaction equations.

Evidence for thermal spin-transfer torque.

Large heat currents are obtained in Co/Cu/Co spin valves positioned at the middle of Cu nanowires. The second harmonic voltage response to an applied current is used to investigate the effect of the heat current on the switching of the spin valves. Both the switching field and the magnitude of the voltage response are found to be dependent on the heat current. These effects are evidence for a thermal spin-transfer torque acting on the magnetization and are accounted for by a thermodynamic model in which heat, charge and spin currents are linked by Onsager reciprocity relations.

Hyperpolarizing gases via dynamic nuclear polarization and sublimation.

A high throughput method was designed to produce hyperpolarized gases by combining low-temperature dynamic nuclear polarization with a sublimation procedure. It is illustrated by applications to 129Xe nuclear magnetic resonance in xenon gas, leading to a signal enhancement of 3 to 4 orders of magnitude compared to the room-temperature thermal equilibrium signal at 7.05 T.

Magnetotransport properties depending on the nanostructure of Fe(3)O(4) nanowires.

We have studied the magnetic behaviour of Fe(3)O(4) nanowires (NWs) with two different diameter ranges, above 150 nm and below 60 nm, made by electrodeposition techniques into a polymeric template. The nanowires were characterized using various techniques, in particular Mössbauer and thermoelectrical power measurements. The stoichiometric distribution of Fe cations showed clearly the presence of the magnetite inverse spinel electronic structure. Structural analysis performed using high-resolution transmission electron microscopy revealed two kinds of nanowire morphologies depending on the size. For nanowires above 150 nm in diameter, a contiguous network of well-bound nanoparticles was obtained. Instead, with a diameter of 60 nm, a polycrystalline structure was observed. The largest nanowires presented a magnetoresistance (MR) greater than 10%, whereas the thinner nanowires had almost none.

Note: three-dimensional stereolithography for millimeter wave and terahertz applications.

Metal-coated polymers shaped by 3D stereolithography are introduced as a new manufacturing method for passive components for millimeter to terahertz electromagnetic waves. This concept offers increased design capabilities and flexibilities while shortening the manufacturing process of complex shapes, e.g., corrugated horns, mirrors, etc. Tests at 92.5, 140, and 170 GHz are reported.

Note: stacked rings for terahertz wave-guiding.

We demonstrate the construction of corrugated waveguides using stacked rings to propagate terahertz frequencies. The waveguide allows propagation of the same fundamental mode as an optical-fiber, namely, the HE(11) mode. This simple concept opens the way for corrugated wave-guides up to several terahertz, maintaining beam characteristics as for terahertz applications.

THz-waves channeling in a monolithic saddle-coil for Dynamic Nuclear Polarization enhanced NMR.

A saddle coil manufactured by electric discharge machining (EDM) from a solid piece of copper has recently been realized at EPFL for Dynamic Nuclear Polarization enhanced Nuclear Magnetic Resonance experiments (DNP-NMR) at 9.4 T. The corresponding electromagnetic behavior of radio-frequency (400 MHz) and THz (263 GHz) waves were studied by numerical simulation in various measurement configurations. Moreover, we present an experimental method by which the results of the THz-wave numerical modeling are validated. On the basis of the good agreement between numerical and experimental results, we conducted by numerical simulation a systematic analysis on the influence of the coil geometry and of the sample properties on the THz-wave field, which is crucial in view of the optimization of DNP-NMR in solids.

Template nanowires for spintronics applications: nanomagnet microwave resonators functioning in zero applied magnetic field.

Low-cost spintronic devices functioning in zero applied magnetic field are required for bringing the idea of spin-based electronics into the real-world industrial applications. Here we present first microwave measurements performed on nanomagnet devices fabricated by electrodeposition inside porous membranes. In the paper, we discuss in details a microwave resonator consisting of three nanomagnets, which functions in zero external magnetic field. By applying a microwave signal at a particular frequency, the magnetization of the middle nanomagnet experiences the ferromagnetic resonance (FMR), and the device outputs a measurable direct current (spin-torque diode effect). Alternatively, the nanodevice can be used as a microwave oscillator functioning in zero field. To test the resonators at microwave frequencies, we developed a simple measurement setup.

Low temperature charge and orbital textures in La0.875Sr0.125MnO3.

By using nuclear magnetic resonance techniques we show that for T<30 K the La0.875Sr0.125MnO3 compound displays a nonuniform charge distribution, comprised of two interconnected Mn ion subsystems with different spin, orbital, and charge couplings. The NMR results agree very well with the two spin wave stiffness constants observed at small q values in the spin wave dispersion curves [Phys. Rev. B 67, 214430 (2003)]. This picture is probably related to a yet undetermined charge and orbital superstructure occurring in the ferromagnetic insulating state of the La0.875Sr0.125MnO3 compound.

Evolution of magnetic polarons and spin-carrier interactions through the metal-insulator transition in Eu(1-x)Gd(x)O.

Raman scattering studies as functions of temperature, magnetic field, and Gd substitution are used to investigate the evolution of magnetic polarons and spin-carrier interactions through the metal-insulator transition in Eu(1-x)Gd(x)O. These studies reveal a spin-fluctuation-dominated paramagnetic (PM) regime for T>T*>T(C), and a coexistence regime for T

Current-induced two-level fluctuations in pseudo-spin-valve (Co/Cu/Co) nanostructures.

Two-level fluctuations of the magnetization state of pseudo-spin-valve pillars Co(10 nm)/Cu(10 nm)/Co(30 nm) embedded in electrodeposited nanowires ( approximately 40 nm in diameter, 6000 nm in length) are triggered by spin-polarized currents of 10(7) A/cm(2) at room temperature. The statistical properties of the residence times in the parallel and antiparallel magnetization states reveal two effects with qualitatively different dependences on current intensity. The current appears to have the effect of a field determined as the bias field required to equalize these times. The bias field changes sign when the current polarity is reversed. At this field, the effect of a current density of 10(7) A/cm(2) is to lower the mean time for switching down to the microsecond range. This effect is independent of the sign of the current and is interpreted in terms of an effective temperature for the magnetization.