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1.
Environ Sci Technol ; 57(6): 2274-2285, 2023 02 14.
Artículo en Inglés | MEDLINE | ID: mdl-36657182

RESUMEN

Biomass burning (BB) is an important source of atmospheric persistent organic pollutants (POPs) across the world. However, there are few field-based regional studies regarding the POPs released from BB. Due to the current limitations of emission factors and satellites, the contribution of BB to airborne POPs is still not well understood. In this study, with the simultaneous monitoring of BB biomarkers and POPs based on polyurethane foam-based passive air sampling technique, we mapped the contribution of BB to polychlorinated biphenyls (PCBs) and organochlorine pesticides (OCPs) in the Indo-China Peninsula. Spearman correlations between levoglucosan and 16 PCBs (rs = 0.264-0.767, p < 0.05) and 2 OCPs (rs = 0.250-0.328, p < 0.05) confirmed that BB may facilitate POP emissions. Source apportionment indicated that BB contributed 9.3% to the total PCB and OCP mass. The high contribution of positive matrix factorization-resolved BB to PCBs and OCPs was almost consistent with their concentration distributions in the open BB season but not completely consistent with those in the pre-monsoon and/or monsoon seasons. Their contribution distributions may reflect the use history and geographic distribution in secondary sources of POPs. The field-based contribution dataset of BB to POPs is significant in improving regional BB emission inventories and model prediction.


Asunto(s)
Contaminantes Atmosféricos , Contaminantes Ambientales , Hidrocarburos Clorados , Plaguicidas , Bifenilos Policlorados , Bifenilos Policlorados/análisis , Contaminantes Orgánicos Persistentes , Biomasa , Contaminantes Atmosféricos/análisis , Hidrocarburos Clorados/análisis , Plaguicidas/análisis , China , Monitoreo del Ambiente/métodos
2.
Artículo en Inglés | MEDLINE | ID: mdl-23082575

RESUMEN

The purpose of this study was to assess a health impact assessment (HIA) tool to determine the perceived health impact by the public of a public park. The authors conducted a cross-sectional study from March to April, 2011, using this HIA questionnaire to collect data and through focus group discussions. We also assessed community concerns about the park and obtained recommendations of how to mitigate possible negative aspects of the parks. Four aspects were listed as possible benefits of the park: physical, mental, social, and spiritual health. The negative aspects mentioned by participants were that a park could be a potential place of assembly for teenagers, a place for theft and crime and accidents among children. The HIA tool used for this research seemed appropriate. The next challenge is to use this tool to assess a more controversial project.


Asunto(s)
Planificación de Ciudades , Planificación en Salud Comunitaria/métodos , Actividades Recreativas , Instalaciones Públicas , Adolescente , Adulto , Estudios Transversales , Femenino , Grupos Focales , Humanos , Entrevistas como Asunto , Masculino , Persona de Mediana Edad , Encuestas y Cuestionarios , Tailandia
3.
Environ Sci Process Impacts ; 24(3): 400-413, 2022 Mar 23.
Artículo en Inglés | MEDLINE | ID: mdl-35137735

RESUMEN

Oxidative stress is a key mechanism by which ambient particulate matter induces adverse health effects. Most studies have focused on the oxidative potential (OP) of water-soluble constituents, while there has been limited work on the OP of solvent-extractable organic matter (EOM OP). In this study, the EOM OP of ambient total suspended particulate (TSP) from Bangkok, Thailand, was determined using the dithiothreitol (DTT) assay. Positive matrix factorization (PMF), combined with chemical analysis of molecular markers, was employed to apportion the contributions of various emission sources to EOM OP. The volume-normalized OP initially increased with organic carbon (OC) concentration and plateaued gradually, while the mass-normalized OP fitted well with OC concentration using a power function. Fossil fuel combustion (62%) and plastic waste burning (23%) were the major contributors to EOM OP, while biomass burning demonstrated only a limited contribution. EOM OP correlated well with each group of polycyclic aromatic hydrocarbons (PAHs), suggesting that secondary formation of quinones associated with fossil fuel combustion and plastic waste burning could be an important pathway of TSP toxicity. This study underscores the importance of considering different emission sources when evaluating potential health impacts and the implementation of air pollution regulations.


Asunto(s)
Contaminantes Atmosféricos , Contaminantes Atmosféricos/análisis , Monitoreo del Ambiente , Estrés Oxidativo , Material Particulado/análisis , Solventes , Tailandia
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