Correlation of circular differential optical absorption with geometric chirality in plasmonic meta-atoms.

We report a strong correlation between the calculated broadband circular differential optical absorption (CDOA) and the geometric chirality of plasmonic meta-atoms with two-dimensional chirality. We investigate this correlation using three common gold meta-atom geometries: L-shapes, triangles, and nanorod dimers, over a broad range of geometric parameters. We show that this correlation holds for both contiguous plasmonic meta-atoms and non-contiguous structures which support plasmonic coupling effects. A potential application for this correlation is the rapid optimization of plasmonic nanostructure for maximum broadband CDOA.

Benchmarking five numerical simulation techniques for computing resonance wavelengths and quality factors in photonic crystal membrane line defect cavities.

We present numerical studies of two photonic crystal membrane microcavities, a short line-defect cavity with a relatively low quality (Q) factor and a longer cavity with a high Q. We use five state-of-the-art numerical simulation techniques to compute the cavity Q factor and the resonance wavelength λ for the fundamental cavity mode in both structures. For each method, the relevant computational parameters are systematically varied to estimate the computational uncertainty. We show that some methods are more suitable than others for treating these challenging geometries.

Insights into directional scattering: from coupled dipoles to asymmetric dimer nanoantennas.

Strong and directionally specific forward scattering from optical nanoantennas is of utmost importance for various applications in the broader context of photovoltaics and integrated light sources. Here, we outline a simple yet powerful design principle to perceive a nanoantenna that provides directional scattering into a higher index substrate based on the interference of multiple electric dipoles. A structural implementation of the electric dipole distribution is possible using plasmonic nanoparticles with a fairly simple geometry, i.e. two coupled rectangular nanoparticles, forming a dimer, on top of a substrate. The key to achieve directionality is to choose a sufficiently large size for the nanoparticles. This promotes the excitation of vertical electric dipole moments due to the bi-anisotropy of the nanoantenna. In turn, asymmetric scattering is obtained by ensuring the appropriate phase relation between the vertical electric dipole moments. The scattering strength and angular spread for an optimized nanoantenna can be shown to be broadband and robust against changes in the incidence angle. The scattering directionality is maintained even for an array configuration of the dimer. It only requires the preferred scattering direction of the isolated nanoantenna not to be prohibited by interference.

Optical Chirality of Time-Harmonic Wavefields for Classification of Scatterers.

We derive expressions for the scattering, extinction and conversion of the chirality of monochromatic light scattered by bodies which are characterized by a T-matrix. In analogy to the conditions obtained from the conservation of energy, these quantities enable the classification of arbitrary scattering objects due to their full, i.e. either chiral or achiral, electromagnetic response. To this end, we put forward and determine the concepts of duality and breaking of duality symmetry, anti-duality, helicity variation, helicity annhiliation and the breaking of helicity annihilation. Different classes, such as chiral and dual scatterers, are illustrated in this analysis with model examples of spherical and non-spherical shape. As for spheres, these concepts are analysed by considering non-Rayleigh dipolar dielectric particles of high refractive index, which, having a strong magnetic response to the incident wavefield, offer an excellent laboratory to test and interpret such changes in the chirality of the illumination. In addition, comparisons with existing experimental data are made.