Time-resolved observation of coherent multi-body interactions in quantum phase revivals.

Interactions lie at the heart of correlated many-body quantum phases. Typically, the interactions between microscopic particles are described as two-body interactions. However, it has been shown that higher-order multi-body interactions could give rise to novel quantum phases with intriguing properties. So far, multi-body interactions have been observed as inelastic loss resonances in three- and four-body recombinations of atom-atom and atom-molecule collisions. Here we demonstrate the presence of effective multi-body interactions in a system of ultracold bosonic atoms in a three-dimensional optical lattice, emerging through virtual transitions of particles from the lowest energy band to higher energy bands. We observe such interactions up to the six-body case in time-resolved traces of quantum phase revivals, using an atom interferometric technique that allows us to precisely measure the absolute energies of atom number states at a lattice site. In addition, we show that the spectral content of these time traces can reveal the atom number statistics at a lattice site, similar to foundational experiments in cavity quantum electrodynamics that yield the statistics of a cavity photon field. Our precision measurement of multi-body interaction energies provides crucial input for the comparison of optical-lattice quantum simulators with many-body quantum theory.

Decoherence of matter waves by thermal emission of radiation.

Emergent quantum technologies have led to increasing interest in decoherence--the processes that limit the appearance of quantum effects and turn them into classical phenomena. One important cause of decoherence is the interaction of a quantum system with its environment, which 'entangles' the two and distributes the quantum coherence over so many degrees of freedom as to render it unobservable. Decoherence theory has been complemented by experiments using matter waves coupled to external photons or molecules, and by investigations using coherent photon states, trapped ions and electron interferometers. Large molecules are particularly suitable for the investigation of the quantum-classical transition because they can store much energy in numerous internal degrees of freedom; the internal energy can be converted into thermal radiation and thus induce decoherence. Here we report matter wave interferometer experiments in which C70 molecules lose their quantum behaviour by thermal emission of radiation. We find good quantitative agreement between our experimental observations and microscopic decoherence theory. Decoherence by emission of thermal radiation is a general mechanism that should be relevant to all macroscopic bodies.

Impurities as a quantum thermometer for a Bose-Einstein Condensate.

We introduce a primary thermometer which measures the temperature of a Bose-Einstein Condensate in the sub-nK regime. We show, using quantum Fisher information, that the precision of our technique improves the state-of-the-art in thermometry in the sub-nK regime. The temperature of the condensate is mapped onto the quantum phase of an atomic dot that interacts with the system for short times. We show that the highest precision is achieved when the phase is dynamical rather than geometric and when it is detected through Ramsey interferometry. Standard techniques to determine the temperature of a condensate involve an indirect estimation through mean particle velocities made after releasing the condensate. In contrast to these destructive measurements, our method involves a negligible disturbance of the system.

Anomalous expansion of attractively interacting fermionic atoms in an optical lattice.

The interplay of thermodynamics and quantum correlations can give rise to counterintuitive phenomena in many-body systems. We report on an isentropic effect in a spin mixture of attractively interacting fermionic atoms in an optical lattice. As we adiabatically increase the attraction between the atoms, we observe that the gas expands instead of contracting. This unexpected behavior demonstrates the crucial role of the lattice potential in the thermodynamics of the fermionic Hubbard model.

Wave nature of biomolecules and fluorofullerenes.

We demonstrate quantum interference for tetraphenylporphyrin, the first biomolecule exhibiting wave nature, and for the fluorofullerene C60F48 using a near-field Talbot-Lau interferometer. For the porphyrins, which are distinguished by their low symmetry and their abundant occurrence in organic systems, we find the theoretically expected maximal interference contrast and its expected dependence on the de Broglie wavelength. For C60F48, the observed fringe visibility is below the expected value, but the high contrast still provides good evidence for the quantum character of the observed fringe pattern. The fluorofullerenes therefore set the new mark in complexity and mass (1632 amu) for de Broglie wave experiments, exceeding the previous mass record by a factor of 2.

Collisional decoherence observed in matter wave interferometry.

We study the loss of spatial coherence in the extended wave function of fullerenes due to collisions with background gases. From the gradual suppression of quantum interference with increasing gas pressure we are able to support quantitatively both the predictions of decoherence theory and our picture of the interaction process. We thus explore the practical limits of matter wave interferometry at finite gas pressures and estimate the required experimental vacuum conditions for interferometry with even larger objects.

Matter-wave interferometer for large molecules.

We demonstrate a near-field Talbot-Lau interferometer for C70 fullerene molecules. Such interferometers are particularly suitable for larger masses. Using three free-standing gold gratings of 1 microm period and a transversally incoherent but velocity-selected molecular beam, we achieve an interference fringe visibility of 40% with high count rate. Both the high visibility and its velocity dependence are in good agreement with a quantum simulation that takes into account the van der Waals interaction of the molecules with the gratings and are in striking contrast to a classical moiré model.