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1.
Small ; 19(52): e2304877, 2023 Dec.
Artículo en Inglés | MEDLINE | ID: mdl-37635127

RESUMEN

Interfacial solar steam generators (ISSGs) can capture solar energy and concentrate the heat at the gas-liquid interface, resulting in efficient water evaporation. However, traditional ISSGs have limitations in long-term seawater desalination processes, such as limited light absorption area, slow water transport speed, severe surface salt accumulation, and weak mechanical performance. Inspired by lotus seedpods, a novel ISSG (rGO-SA-PSF) is developed by treating a 3D warp-knitted spacer fabric with plasma (PSF) and combining it with sodium alginate (SA) and reduces graphene oxide (rGO). The rGO-SA-PSF utilizes a core-suction effect to achieve rapid water pumping and employs aerogel to encapsulate the plasma-treated spacer yarns to create the lotus seedpod-inspired hydrophilic stems, innovatively constructing multiple directional water transport channels. Simultaneously, the large holes of rGO-SA-PSF on the upper layer form lotus seedpod-inspired head concave holes, enabling efficient light capture. Under 1 kW m-2 illumination, rGO-SA-PSF exhibits a rapid evaporation rate of 1.85 kg m-2  h-1 , with an efficiency of 96.4%. Additionally, it shows superior salt tolerance (with no salt accumulation during continuous evaporation for 10 h in 10% brine) and self-desalination performance during long-term seawater desalination processes. This biomimetic ISSG offers a promising solution for efficient and stable seawater desalination and wastewater purification.

2.
Sci Total Environ ; 903: 166212, 2023 Dec 10.
Artículo en Inglés | MEDLINE | ID: mdl-37567279

RESUMEN

Interfacial solar evaporators are widely used to purify water. However, photothermal materials commonly constituting most interfacial solar evaporators remain expensive; additionally, the inherent structure of the evaporators limits their performance. Furthermore, the large amount of waste cotton produced by the textile industry is an environmental threat. To address these issues, we propose an interfacial solar evaporator, H-CA-CS, with a hierarchical porous structure. This evaporator is made entirely of waste cotton and uses carbon microspheres (CMS) and cellulose aerogel (CA) as photothermal and substrate materials, respectively. Additionally, its photothermal layer (CS layer) has large pores and a high porosity, which promote light absorption and timely vapor escape. In contrast, the water transport layer (CA layer) has small pores, providing a robust capillary effect for water transport. Combined with the outstanding light absorption properties of CMS, H-CA-CS exhibited superior overall performance. We found that H-CA-CS has an excellent evaporation rate (1.68 kg m-2 h-1) and an efficiency of 90.6 % under one solar illumination (1 kW m-2), which are superior to those of many waste-based solar evaporators. Moreover, H-CA-CS maintained a mean evaporation rate of 1.61 kg m-2 h-1, ensuring sustainable evaporation performance under long-term scenarios. Additionally, H-CA-CS can be used to purify seawater and various types of wastewater with removal efficiencies exceeding 99 %. In conclusion, this study proposes a method for efficiently using waste cotton to purify water and provides novel ideas for the high-value use of other waste fibers to further mitigate ongoing environmental degradation.

3.
Macromol Biosci ; 23(2): e2200356, 2023 02.
Artículo en Inglés | MEDLINE | ID: mdl-36382353

RESUMEN

A microclimate with ventilation and proper wettability near the wound is vital for wound healing. In the case of pressure or absorption of large amounts of wound exudate, maintaining air circulation around the wound is currently a challenge for wound dressings. In this study, a novel self-pumping dressing (FAED) with multiple liquid transport channels is designed by combining a 3D spacer fabric, sodium alginate aerogel, and electrospun membrane. This unique structural design allows FAED to unidirectionally rapidly remove excess biofluid from the wound and transfer it through a special liquid transport channel to a liquid storage layer with a high absorption ratio. Importantly, the air circulation layer of FAED composed of liquid transport channels and spacer yarns provides excellent air permeability in both the horizontal (12.3 L min-1 ) and vertical (272.02 mm s-1 ) directions. Additionally, a lower compression modulus (0.14 MPa) and higher compression strength (0.15 MPa) enable the novel dressing to adapt to body contours and provide good supporting performance, as compared to foam dressings. Combined with its high biocompatibility, this unique dressing has significant potential for wound treatment and intensive care.


Asunto(s)
Vendajes , Microclima , Cicatrización de Heridas , Permeabilidad , Humectabilidad
4.
Polymers (Basel) ; 12(2)2020 Feb 01.
Artículo en Inglés | MEDLINE | ID: mdl-32024154

RESUMEN

In this study, a new type ternary composite, called warp-knitted spacer fabric reinforced syntactic foam (WKSF-SF), with the advantages of high mechanical properties and a lower density, was proposed. Then, a meso-mechanics theoretical model based on the Eshelby-Mori-Tanaka equivalent inclusion method, average stress method and composite hybrid theory was established to predict the compression modulus of WKSF-SF. In order to verify the validity of this model, compression modulus values of theoretical simulations were compared with the quasi-static compression experiment results. The results showed that the addition of suitable WKSF produces at least 15% improvement in the compressive modulus of WKSF-SF compared with neat syntactic foam (NSF). Meanwhile, the theoretical model can effectively simulate the values and variation tendency of the compression modulus for different WKSF-SF samples, and is especially suitable for the samples with smaller wall thickness or a moderate volume fraction of microballoons (the deviations is less than 5%). The study of the meso-mechanical properties of WKSF-SF will help to increase understanding of the compression properties of this new type composite deeply. It is expected that WKSF-SF can be used in aerospace, marine, transportation, construction, and other fields.

5.
Polymers (Basel) ; 11(8)2019 Aug 01.
Artículo en Inglés | MEDLINE | ID: mdl-31374983

RESUMEN

The effects of reinforcement structures and hybrid types on the inter-laminar shear strength (ILSS) of carbon-glass hybrid fibers/bismaleimide composites under thermo-oxidative aging conditions were investigated. The process resulted in progressive deterioration of the matrix and fiber/matrix interfaces, in the form of chain scissions, weight loss, and fiber/matrix debonding, which significantly led to the decrease of the ILSS of composites. Moreover, the three-dimensional orthogonal woven hybrid composites (3D composites) showed higher ILSS retention rate than those of the laminated orthogonal hybrid composites (laminated composites). No delamination occurred in the aged 3D composites like in the aged laminated composites. This was because the Z-binder yarns in the 3D composites resisted the inter-laminar shear load, although the resin was damaged and the adhesive force between fiber bundles and resin decreased seriously after thermo-oxidative aging. Meanwhile, the ILSS retention rate of the laminated composites with the carbon fiber as intermediate layers was higher than that of the laminated composites with the glass fiber as the intermediate layers. This was because the carbon fiber/bismaleimide interface bonding performance was stronger than that of the glass fiber/bismaleimide at the same thermo-oxidative aging condition.

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