Giant Photoluminescence Enhancement of Monolayer WSe2 Using a Plasmonic Nanocavity with On-Demand Resonance.

Monolayer transition metal dichalcogenides (TMDs) are considered promising building blocks for next-generation photonic and optoelectronic devices, owing to their fascinating optical properties. However, their inherent weak light absorption and low quantum yield severely hinder their practical applications. Here, we report up to 18000-fold photoluminescence (PL) enhancement in a monolayer WSe2-coupled plasmonic nanocavity. A spectroscopy-assisted nanomanipulation technique enables the assembly of a nanocavity with customizable resonances to simultaneously enhance the excitation and emission processes. In particular, precise control over the magnetic cavity mode facilitates spectral and spatial overlap with the exciton, resulting in plasmon-exciton intermediate coupling that approaches the maximum emission rate in the hybrid system. Meanwhile, the cavity mode exhibits high radiation directivity, which overwhelmingly directs surface-normal PL emission and leads to a 17-fold increase in the collection efficiency. Our approach opens up a new avenue to enhance the PL intensity of monolayer TMDs, facilitating their implementation in highly efficient optoelectronic devices.

Precisely constructing hybrid nanogap arrays via wet-transfer of dielectric metasurfaces onto a plasmonic mirror.

We propose a new method for fabricating hybrid metasurfaces by combining Mie and plasmonic resonances. Our approach involves obtaining an ultrasmooth gold film and separately structuring monocrystalline silicon (c-Si) nanoantenna arrays, which are then wet-transferred and finally immobilized onto the gold film. The experimental and simulation analysis reveals the importance of the native oxide layer of Si and demonstrates fascinating dispersion curves with nanogap resonances and bound states in the continuum. The localized field enhancements in the nanogap cavities result from the coupling between multipolar Mie resonances and their mirror images in the gold film. This effective method improves our understanding of hybrid modes and offers opportunities for developing active metasurfaces, such as depositing c-Si nanoantenna arrays onto stretchable polydimethylsiloxane substrates or electro-optic and piezoelectric sensitive lithium niobate films for potential applications in MEMS, LiDAR, and beyond.

Nanometric displacement sensor with a switchable measuring range using a cylindrical vector beam excited silicon nanoantenna.

We demonstrate a nanometric displacement sensor with a switchable measuring range by using a single silicon nanoantenna. It is revealed that the interference between the longitudinal and transverse dipolar scattering can be well tuned by moving the nanoantenna in the focal field of the cylindrical vector beam. As a result, a position related scattering directivity is found and is used as a displacement sensor with a 4.5 nm lateral resolution. Interestingly, the measuring range of this displacement sensor can be extended by twice through simply changing the excitation from the azimuthally polarized beam to the radially polarized beam. Our results provide a facile way to tune the measuring range of the nanometric displacement sensor and may open up an avenue to super-resolution microscopy and optical nanometrology.

Double-arrow metasurface for dual-band and dual-mode polarization conversion.

We present experimentally a double-arrow metasurface for high-efficiently manipulating the polarization states of electromagnetic waves in the dual-band. The metasurface is capable of converting a linearly polarized (LP) incident wave into a circularly polarized (CP) wave or its cross-polarized LP wave at different frequencies. It is numerically shown that in the two bands from 14.08 to 15.71 GHz and from 17.63 to 19.55 GHz the metasurface can convert the LP wave into CP wave, of which the axis ratio is lower than 3 dB. Meanwhile, the proposed metasurface also can convert the LP wave into its cross-polarized LP wave at 13.39 GHz and 20.29 GHz. To validate the theoretical analysis and simulated results, a prototype is fabricated and measured. The experimental results are reasonably consistent with the theoretical and simulated results, which demonstrates that such a metasurface can successfully achieve dual-band and dual-mode polarization conversion.

Reversible optical binding force in a plasmonic heterodimer under radially polarized beam illumination.

We investigated the optical binding force in a plasmonic heterodimer structure consisting of two nano-disks. It is found that when illuminated by a tightly focused radially polarized beam (RPB), the plasmon modes of the two nano-disks are strongly hybridized, forming bonding/antibonding modes. An interesting observation of this setup is that the direction of the optical binding force can be controlled by changing the wavelength of illumination, the location of the dimer, the diameter of the nano-disks, and the dimer gap size. Further analysis yields that the inhomogeneous polarization state of RPB can be utilized to readily control the bonding type of plasmon modes and distribute the underlying local field confined in the gap (the periphery) of the dimer, leading to a positive (negative) optical binding force. Our findings provide a clear strategy to engineer optical binding forces via changes in device geometry and its illumination profile. Thus, we envision a significant role for our device in emerging nanophotonics structures.

Structured light beams created through a multimode fiber via virtual Fourier filtering based on digital optical phase conjugation.

Digital optical phase conjugation (DOPC) is a newly developed technique in wavefront shaping to control light propagation through complex media. Currently, DOPC has been demonstrated for the reconstruction of two- and three-dimensional targets and enabled important applications in many areas. Nevertheless, the reconstruction results are only phase conjugated to the original input targets. Herein, we demonstrate that DOPC could be further developed for creating structured light beams through a multimode fiber (MMF). By applying annular filtering in the virtual Fourier domain of the acquired speckle field, we realize the creation of the quasi-Bessel and donut beams through the MMF. In principle, arbitrary amplitude and/or phase circular symmetry filtering could be performed in the Fourier domain, thus generating the corresponding point spread functions. We expect that the reported technique can be useful for super-resolution endoscopic imaging and optical manipulation through MMFs.

Unidirectional scattering exploited transverse displacement sensor with tunable measuring range.

We propose a scheme to extend the measuring range of a transverse displacement sensor by exploiting the interaction of an azimuthally polarized beam (APB) with a single metal-dielectric core-shell nanoparticle. The focused APB illumination induces a longitudinal magnetic dipole (MD) in the core-shell nanoparticle, which interferes with the induced transverse electric dipole (ED) to bring forth a transverse unidirectional scattering at a specific position within the focal plane. Emphatically, the rapidly varying electromagnetic field within the focal plane of an APB leads to a remarkable sensitivity of the far-field scattering directivity to nanoscale displacements as the nanoparticle moves away from the optical axis. Moreover, the scattering directivity of the APB illuminated core-shell nanoparticle is also a function of structure-dependent Mie scattering coefficients, rendering the measuring range of the transverse displacement sensor widely tunable. The culmination of all these features enables the continuous tuning of the displacement measuring range from several nanometers to a few micrometers. Thus, we envision the proposed scheme is of high value for modern optical nanometrology.

Radial breathing modes coupling in plasmonic molecules.

Metallic hexamer, very much the plasmonic analog of benzene molecule, provides an ideal platform to mimic modes coupling and hybridization in molecular systems. To demonstrate this, we present a detailed study on radial breathing mode (RBM) coupling in a plasmonic dual-hexamers. We excite RBMs of hexamers by symmetrically matching the polarization state of the illumination with the distribution of electric dipole moments of the dual-hexamer. It is found that the RBM coupling exhibits a nonexponential decay when the inter-hexamer separation is increased, owing to the dark mode nature of RBM. When the outer hexamer is subjected to the in-plane twisting, resonant wavelengths of two coupled RBMs as well as the coupling constant show cosine variations with the twist angle, indicating the symmetry of hexamer structure plays a critical role in the coupling of RBMs. Moreover, it is demonstrated that the coupling of RBMs is dominated by the in-plane interaction as the outer hexamer is under an out-of-plane tilting, causing convergence of resonant wavelengths of the two coupled RBMs with increasing tilt angle. Our results not only provide an insight into the plasmonic RBM coupling mechanism, but also pave the way to systematically control the spectral response of plasmonic molecules.

Enhanced second-harmonic generation assisted by breathing mode in a multi-resonant plasmonic trimer.

Boosting the nonlinear conversion rate in nanoscale is pivotal for practical applications such as highly sensitive biosensors, extreme ultra-violate light sources, and frequency combs. Here, we theoretically study the enhancement of second-harmonic generation (SHG) in a plasmonic trimer assisted by breathing modes. The geometry of the trimer is fine-tuned to produce strong plasmonic resonances at both the fundamental and SH wavelengths to boost SHG intensity. Moreover, it is found that breathing modes show remarkable ability to augment SHG by increasing the enhancement area. In particular, these breathing modes ensure a substantial spatial mode overlap at the fundamental and SH wavelengths, resulting in further promotion of the SHG conversation rate. We envision that our findings could enable applications in nanoscale frequency converters with high efficiency.

Characterizing localized surface plasmon resonances using focused radially polarized beam.

We demonstrate a scheme to characterize the localized surface plasmon resonances (LSPRs) of an individual metallic nanorod by employing a focused radially polarized beam (RPB) illumination under normal incidence. The focused RPB has a unique three-dimensional electric field polarization distribution in the focal plane, which can effectively and selectively excite the dipole and multipole plasmon resonances in a metallic nanorod by just moving the nanorod within the focal plane. This performance can be attributed to the mode matching between the excitation electric field of the incident RPB and the LSPRs in a metallic nanorod. Emphatically, in contrast to the commonly used oblique incidence illumination with the linearly polarized light, our proposed scheme is based on the normally incident light illumination and compatible with conventional optical microscopy, which is more scalable for spectroscopic characterization of individual nanostructures.

Water metamaterial for ultra-broadband and wide-angle absorption.

A subwavelength water metamaterial is proposed and analyzed for ultra-broadband perfect absorption at microwave frequencies. We experimentally demonstrate that this metamaterial shows over 90% absorption within almost the entire frequency band of 12-29.6 GHz. It is also shown that the proposed metamaterial exhibits a good thermal stability with its absorption performance almost unchanged for the temperature range from 0 to 100°C. The study of the angular tolerance of the metamaterial absorber shows its ability of working at wide angles of incidence. Given that the proposed water metamaterial absorber is low-cost and easy for manufacture, we envision it may find numerous applications in electromagnetics such as broadband scattering reduction and electromagnetic energy harvesting.

Reconstruction of structured laser beams through a multimode fiber based on digital optical phase conjugation.

The digital optical phase conjugation (DOPC) technique is being actively developed for optical focusing and imaging through or inside complex media. Due to its time-reversal nature, DOPC has been exploited to regenerate different intensity targets. However, whether the targets with three-dimensional information through complex media could be recovered has not been experimentally demonstrated, to the best of our knowledge. Here, we present a method to regenerate structured laser beams based on DOPC. Although only the phase of the original scattered wave is time reversed, the reconstruction of a quasi-Bessel beam and vortex beams through a multimode fiber (MMF) is demonstrated. The regenerated quasi-Bessel beam shows the features of sub-diffraction focusing and a longer depth of field with respect to a Gaussian beam. Moreover, the reconstruction of vortex beams shows the fidelity of DOPC both in amplitude and phase, which is demonstrated for the first time, to the best of our knowledge. We also prove that the reconstruction results of DOPC through the MMF are indeed phase conjugate to the original targets. We expect that these results could be useful in super-resolution imaging and optical micromanipulation through complex media, and further pave the way for achieving three-dimensional imaging based on DOPC.

Sub-10 nm particle trapping enabled by a plasmonic dark mode.

We demonstrate that a highly localized plasmonic dark mode with radial symmetry, termed quadrupole-bonded radial breathing mode, can be used for optically trapping the dielectric nanoparticles. In particular, the annular potential well produced by this dark mode shows a sufficiently large depth to stably trap the 5 nm particles under a relatively low optical power. Our results address the quest for precisely trapping sub-10 nm particles with high yield and pave the way for placing sub-10 nm particles conforming to a specific geometric pattern.

Non-diffracting optical Bloch oscillations in hexagonal photonic lattices.

Light beams undergoing optical Bloch oscillations (OBOs) in two-dimensional (2D) photonic lattices suffer from severe diffraction along the perpendicular direction to the oscillation plane. In this paper, we propose and demonstrate that such diffraction could be suppressed in hexagonal photonic lattices via sophisticated managements of the discrete diffraction. By positioning the Fourier spectrum of the beam to a special region in the Brillouin zone, the light driven by the OBO experiences normal and anomalous diffractions alternatively, leading to a non-diffracting propagation for a long distance. We show that non-diffracting OBOs can be implemented not only for Gaussian beam but also for other complex 2D beams including self-accelerating Airy beams and vortex beams. Our results provide novel insights into the diffraction or dispersion engineering of waves in periodic structures.

Multiband coherent perfect absorption in a water-based metasurface.

We design an ultrathin water-based metasurface capable of coherent perfect absorption (CPA) at radio frequencies. It is demonstrated that such a metasurface can almost completely absorb two symmetrically incident waves within four frequency bands, each having its own modulation depth of metasurface absorptivity. Specifically, the absorptivity at 557.2 MHz can be changed between 0.59% and 99.99% via the adjustment of the phase difference between the waves. The high angular tolerance of our metasurface is shown to enable strong CPA at oblique incidence, with the CPA frequency almost independent of the incident angle for TE waves and varying from 557.2 up to 584.2 MHz for TM waves. One can also reduce this frequency from 712.0 to 493.3 MHz while retaining strong coherent absorption by varying the water layer thickness. It is also show that the coherent absorption performance can be flexibly controlled by adjusting the temperature of water. The proposed metasurface is low-cost, biocompatible, and useful for electromagnetic modulation and switching.

Wideband visible-light absorption in an ultrathin silicon nanostructure.

We design a new kind of metamaterial absorber in the form of an ultrathin silicon nanostructure capable of having wideband absorption of visible light. We show that our metamaterial can exhibit almost perfect absorption of incident light even though its thickness is several tens of times smaller than the optical wavelength. The combination of two resonant modes in a single nanostructure allows us to achieve absorptivities exceeding 80% in a wide band spanning from 437.9 to 578.3 nm. The physical origins of the two modes, elucidated via the analysis of current distribution inside the nanostructure, explain different metamaterial absorptivities for oblique incidence of TE- and TM-polarized waves. Our study opens a new prospect in designing ultrathin, yet wideband visible-light absorbers based on silicon.

Control the Raman response of individual carbon nanotubes by orbital angular momentum of light.

We propose and demonstrate an approach for tailoring the Raman response of an individual single-walled carbon nanotube (SWNT) by employing the optical vortex as the excitation. Specifically, we observe the blueshifts of radial breathing mode and G mode when the topological charge of the vortex beam is increased from 0 to 5. Further theoretical analysis yields that the optical absorption and the corresponding laser heating effect of SWNT are inversely proportional to the topological charge of the optical vortex. Such a decrease in the laser heating effect weakens the softening of C-C bonds, leading to the blueshifts of Raman modes.

Optical Bloch oscillations and Zener tunneling of Airy beams in ionic-type photonic lattices.

We report on the existence of optical Bloch oscillations (OBOs) and Zener tunneling (ZT) of Airy beams in ionic-type photonic lattices with a refractive index ramp. Different from their counterparts in uniform lattices, Airy beams undergoing OBOs show an alternatively switched concave and convex trajectory as well as a periodical revival of input beam profiles. Moreover, the ionic-type photonic lattice established in photorefractive crystal exhibits a reconfigurable lattice structure, which provides a flexible way to tune the amplitude and period of the OBOs. Remarkably, it is demonstrated that the band gap of the lattice can be readily controlled by rotating the lattice inducing beam, which forces the ZT rate to follow two significant different decay curves amidst decreasing index gradient. Our results open up new possibilities for all-optical switching, routing and manipulation of Airy beams.

Electrical control of second harmonic generation in a graphene-based plasmonic Fano structure.

We propose a strategy for active control of second harmonic generation (SHG) in a plasmonic Fano structure by electrically doping its underlying monolayer graphene. A detailed theoretical model for the proposed scheme is developed and numerical simulations are carried out to demonstrate the operation. Specifically, we show that a merely 30 meV change in graphene Fermi level can result in 45 times increase in SHG peak intensity, accompanied by a resonance wavelength shift spanning 220 nm. Further analysis uncovers that such tunability in SHG arises from the Fermi-level-modulated graphene permittivity, the real and imaginary parts of which dominate the resonance wavelength and the intensity of SHG, respectively.

Controlling Fano resonance of ring/crescent-ring plasmonic nanostructure with Bessel beam.

We propose a method to dynamically control the Fano resonance of a ring/crescent-ring gold nanostructure by spatially changing the phase distribution of a probe Bessel beam. We demonstrate that a highly tunable Fano interference between the quadrupole and bright dipole modes can be realized in the near-infrared range. Even though a complex interference between a broad resonance and a narrower resonance lead to these observations, we show that a simple coupled oscillator model can accurately describe the behavior, providing valuable insights into the dynamics of the system. A further analysis of this structure uncovers a series of interesting phenomena such as anticrossing, sign changing of coupling and the spectral inversion of quadrupole and bright dipole modes. We further show that near field enhancement at Fano resonance can be actively controlled by modulating the phase distribution of the exciting incident Bessel beam.