Broadband, high-power optical frequency combs covering visible to near-infrared spectral range.

Optical frequency combs (OFCs) have become essential tools in a wide range of metrological and scientific research fields. However, in the reported literature, OFCs that cover the visible spectral range have a limited bandwidth and pulse energy. These drawbacks limit their potential applications, such as high-signal-to-noise ratio spectroscopic measurements. In this work, we demonstrate a broadband, high-power optical frequency comb covering the visible to near-infrared range (550 nm to 900 nm) with a high average power of approximately 300 mW. This is accomplished by the power scaling of optical pulses from a fully stabilized Er:fiber comb, coherent spectral broadening and finally the utilization of a PPLN's χ(2) nonlinearity. The broadband, high-power, fully stabilized visible OFCs showcased in this work offer reliable laser sources for high-precision spectroscopic measurements, imaging, and comparisons of optical clocks.

All-fiber frequency comb at 2 µm providing 1.4-cycle pulses.

We report an all-fiber approach to generating sub-2-cycle pulses at 2 µm and a corresponding octave-spanning optical frequency comb. Our configuration leverages mature erbium:fiber laser technology at 1.5 µm to provide a seed pulse for a thulium-doped fiber amplifier that outputs 330 mW average power at a 100 MHz repetition rate. Following amplification, nonlinear self-compression in fiber decreases the pulse duration to 9.5 fs, or 1.4 optical cycles. The spectrum of the ultrashort pulse spans from 1 to beyond 2.4 µm and enables direct measurement of the carrier-envelope offset frequency. Our approach employs only commercially available fiber components, resulting in a design that is easy to reproduce in the larger community. As such, this system should be useful as a robust frequency comb source in the near-infrared or as a pump source to generate mid-infrared frequency combs.

Linearly chirped mid-infrared supercontinuum in all-normal-dispersion chalcogenide photonic crystal fibers.

We demonstrate all-normal dispersion supercontinuum generation in chalcogenide photonic crystal fibers pumped at 2070-2080 nm with a femtosecond fiber laser. At 2.9 kW peak power, the generated supercontinuum has a 3 dB bandwidth of 27.6 THz and -20 dB bandwidth of 75.5 THz. We experimentally investigated the supercontinuum evolution inside our sample fiber at various peak powers and fiber lengths and study the impact of fiber water absorption on the generated supercontinuum spectrum. Multiple tests with fiber length- ranging from 0.34 to 10 cm-provide insight on pulse evolution along fiber length. Our simulations, which utilizes the generalized nonlinear Schrodinger equation model, match perfectly the experiments for all tested pump powers and fiber lengths, and confirm that the output pulse has a linear chirp, allowing linear pulse compression.

Fiber fuse in chalcogenide photonic crystal fibers.

We observe fiber fuse in tapered GeAsSe photonic crystal fibers (PCF) at around 7 MW/cm2 of intra-core intensity. Vertically cleaved facets from the un-tapered regions and the tapered regions were imaged. The images show shallow voids of different shapes confined to the fiber core. After longitudinally polishing a segment of the PCF, we imaged the PCF internal structure's top view, revealing the fuse voids' geometries and periodicity. In addition, fiber fuse was terminated in one PCF sample by a fast laser shutdown, hence saving a small segment from catastrophic damage. Four-wave-mixing was performed on this transmissive segment to estimate the dispersion. The results yielded an evident hole-pitch ratio change after fiber fuse. To our knowledge, this is the first report of fiber fuse on non-silica glass fibers and the first study of its aftermath on this un-destroyed segment of PCFs.

Characterization and modeling of microstructured chalcogenide fibers for efficient mid-infrared wavelength conversion.

We experimentally demonstrate wavelength conversion in the 2 µm region by four-wave mixing in an AsSe and a GeAsSe chalcogenide photonic crystal fibers. A maximum conversion efficiency of -25.4 dB is measured for 112 mW of coupled continuous wave pump in a 27 cm long fiber. We estimate the dispersion parameters and the nonlinear refractive indexes of the chalcogenide PCFs, establishing a good agreement with the values expected from simulations. The different fiber geometries and glass compositions are compared in terms of performance, showing that GeAsSe is a more suited candidate for nonlinear optics at 2 µm. Building from the fitted parameters we then propose a new tapered GeAsSe PCF geometry to tailor the waveguide dispersion and lower the zero dispersion wavelength (ZDW) closer to the 2 µm pump wavelength. Numerical simulations shows that the new design allows both an increased conversion efficiency and bandwidth, and the generation of idler waves further in the mid-IR regions, by tuning the pump wavelength in the vicinity of the fiber ZDW.

Broadband 1-GHz mid-infrared frequency comb.

Mid-infrared (MIR) spectrometers are invaluable tools for molecular fingerprinting and hyper-spectral imaging. Among the available spectroscopic approaches, GHz MIR dual-comb absorption spectrometers have the potential to simultaneously combine the high-speed, high spectral resolution, and broad optical bandwidth needed to accurately study complex, transient events in chemistry, combustion, and microscopy. However, such a spectrometer has not yet been demonstrated due to the lack of GHz MIR frequency combs with broad and full spectral coverage. Here, we introduce the first broadband MIR frequency comb laser platform at 1 GHz repetition rate that achieves spectral coverage from 3 to 13 µm. This frequency comb is based on a commercially available 1.56 µm mode-locked laser, robust all-fiber Er amplifiers and intra-pulse difference frequency generation (IP-DFG) of few-cycle pulses in χ(2) nonlinear crystals. When used in a dual comb spectroscopy (DCS) configuration, this source will simultaneously enable measurements with µs time resolution, 1 GHz (0.03 cm-1) spectral point spacing and a full bandwidth of >5 THz (>166 cm-1) anywhere within the MIR atmospheric windows. This represents a unique spectroscopic resource for characterizing fast and non-repetitive events that are currently inaccessible with other sources.