Convective Steady State in Shallow Cloud Fields.

Shallow cloud fields exhibit different patterns, such as closed or open hexagonal cells and cloud streets. These patterns play a key role in determining the cloud fields' radiative effects, thereby affecting the climate. Here, we show that a large subset of shallow cloud fields forms organized, mesoscale-sized, regular patterns that persist for extended times. It emanates from the steady state of the underlying rigid configuration of convection cells. From a climate perspective, in a sea of cloud complexity, the convective steady-state provides an "island of simplicity." The convective steady state can be parametrized in climate models to better capture the feedback of such cloud fields in a warming climate.

Uncovering the Large-Scale Meteorology That Drives Continental, Shallow, Green Cumulus Through Supervised Classification.

One of the major sources of uncertainty in climate prediction results from the limitations in representing shallow cumulus (Cu) in models. Recently, a class of continental shallow convective Cu was shown to share distinct morphological properties and to emerge globally mostly over forests and vegetated areas, thus named greenCu. Using machine-learning supervised classification, we identify greenCu fields over three regions, from the tropics to mid- and higher-latitudes, and establish a novel satellite-based data set called greenCuDb, consisting of 1° × 1° sized, high-resolution MODIS images. Using greenCuDb in conjunction with ERA5 reanalysis data, we create greenCu composites for different regions and reveal that greenCu are driven by similar large-scale meteorological conditions, regardless of their geographical locations throughout the world's continents. These conditions include distinct profiles of temperature, humidity and large-scale vertical velocity. The boundary layer is anomalously warm and moderately humid, and is accompanied by a strong large-scale subsidence in the free troposphere.

Diel cycle of sea spray aerosol concentration.

Sea spray aerosol (SSA) formation have a major role in the climate system, but measurements at a global-scale of this micro-scale process are highly challenging. We measured high-resolution temporal patterns of SSA number concentration over the Atlantic Ocean, Caribbean Sea, and the Pacific Ocean covering over 42,000 km. We discovered a ubiquitous 24-hour rhythm to the SSA number concentration, with concentrations increasing after sunrise, remaining higher during the day, and returning to predawn values after sunset. The presence of dominating continental aerosol transport can mask the SSA cycle. We did not find significant links between the diel cycle of SSA number concentration and diel variations of surface winds, atmospheric physical properties, radiation, pollution, nor oceanic physical properties. However, the daily mean sea surface temperature positively correlated with the magnitude of the day-to-nighttime increase in SSA concentration. Parallel diel patterns in particle sizes were also detected in near-surface waters attributed to variations in the size of particles smaller than ~1 µm. These variations may point to microbial day-to-night modulation of bubble-bursting dynamics as a possible cause of the SSA cycle.

Non-Monotonic Aerosol Effect on Precipitation in Convective Clouds over Tropical Oceans.

Aerosol effects on convective clouds and associated precipitation constitute an important open-ended question in climate research. Previous studies have linked an increase in aerosol concentration to a delay in the onset of rain, invigorated clouds and stronger rain rates. Here, using observational data, we show that the aerosol effect on convective clouds shifts from invigoration to suppression with increasing aerosol optical depth. We explain this shift in trend (using a cloud model) as the result of a competition between two types of microphysical processes: cloud-core-based invigorating processes vs. peripheral suppressive processes. We show that the aerosol optical depth value that marks the shift between invigoration and suppression depends on the environmental thermodynamic conditions. These findings can aid in better parameterizing aerosol effects in climate models for the prediction of climate trends.

Shallow Convective Cloud Field Lifetime as a Key Factor for Evaluating Aerosol Effects.

Clouds control much of the Earth's energy and water budgets. Aerosols, suspended in the atmosphere, interact with clouds and affect their properties. Recent studies have suggested that the aerosol effect on warm convective cloud systems evolve in time and eventually approach a steady state for which the overall effects of aerosols can be considered negligible. Using numerical simulations, it was estimated that the time needed for such cloud fields to approach this state is >24 hr. These results suggest that the typical cloud field lifetime is an important parameter in determining the total aerosol effect. Here, analyzing satellite observations and reanalysis data (with the aid of numerical simulations), we show that the characteristic timescale of warm convective cloud fields is less than 12 hr. Such a timescale implies that these clouds should be regarded as transient-state phenomena and therefore can be highly susceptible to changes in aerosol properties.

Aerosol effect on the evolution of the thermodynamic properties of warm convective cloud fields.

Convective cloud formation and evolution strongly depend on environmental temperature and humidity profiles. The forming clouds change the profiles that created them by redistributing heat and moisture. Here we show that the evolution of the field's thermodynamic properties depends heavily on the concentration of aerosol, liquid or solid particles suspended in the atmosphere. Under polluted conditions, rain formation is suppressed and the non-precipitating clouds act to warm the lower part of the cloudy layer (where there is net condensation) and cool and moisten the upper part of the cloudy layer (where there is net evaporation), thereby destabilizing the layer. Under clean conditions, precipitation causes net warming of the cloudy layer and net cooling of the sub-cloud layer (driven by rain evaporation), which together act to stabilize the atmosphere with time. Previous studies have examined different aspects of the effects of clouds on their environment. Here, we offer a complete analysis of the cloudy atmosphere, spanning the aerosol effect from instability-consumption to enhancement, below, inside and above warm clouds, showing the temporal evolution of the effects. We propose a direct measure for the magnitude and sign of the aerosol effect on thermodynamic instability.

From aerosol-limited to invigoration of warm convective clouds.

Among all cloud-aerosol interactions, the invigoration effect is the most elusive. Most of the studies that do suggest this effect link it to deep convective clouds with a warm base and cold top. Here, we provide evidence from observations and numerical modeling of a dramatic aerosol effect on warm clouds. We propose that convective-cloud invigoration by aerosols can be viewed as an extension of the concept of aerosol-limited clouds, where cloud development is limited by the availability of cloud-condensation nuclei. A transition from pristine to slightly polluted atmosphere yields estimated negative forcing of ~15 watts per square meter (cooling), suggesting that a substantial part of this anthropogenic forcing over the oceans occurred at the beginning of the industrial era, when the marine atmosphere experienced such transformation.