Dicke-Cooperativity-Assisted Ultrastrong Coupling Enhancement in Terahertz Metasurfaces.

A system of N two-level atoms cooperatively interacting with a photonic field can be described as a single giant atom coupled to the field with interaction strength ∝N. This enhancement, known as Dicke cooperativity in quantum optics, has recently become an indispensable element in quantum information technology. Here, we extend the coupling beyond the standard light-matter interaction paradigm, enhancing Dicke cooperativity in a terahertz metasurface with N meta-atoms. The cooperative enhancement is manifested through the hybridization of the localized surface plasmon resonance in individual meta-atoms and surface lattice resonance due to the periodic array. Furthermore, through engineering of the capacitive split-gap in the meta-atoms, we were able to enhance the coupling rate into the ultrastrong coupling regime by a factor of N. Our strategy can serve as a new platform for demonstrating effective control of fermionic systems by weak pumping, superradiant emission, and ultrasensitive sensing of molecules.

Superradiant Phase Transition in a Superconducting Circuit in Thermal Equilibrium.

We propose a superconducting circuit that shows a superradiant phase transition (SRPT) in thermal equilibrium. The existence of the SRPT is confirmed analytically in the limit of an infinite number of artificial atoms. We also perform a numerical diagonalization of the Hamiltonian with a finite number of atoms and observe an asymptotic behavior approaching the infinite limit as the number of atoms increases. The SRPT can also be interpreted intuitively in a classical analysis.

Perfect intrinsic squeezing at the superradiant phase transition critical point.

Some of the most exotic properties of the quantum vacuum are predicted in ultrastrongly coupled photon-atom systems; one such property is quantum squeezing leading to suppressed quantum fluctuations of photons and atoms. This squeezing is unique because (1) it is realized in the ground state of the system and does not require external driving, and (2) the squeezing can be perfect in the sense that quantum fluctuations of certain observables are completely suppressed. Specifically, we investigate the ground state of the Dicke model, which describes atoms collectively coupled to a single photonic mode, and we found that the photon-atom fluctuation vanishes at the onset of the superradiant phase transition in the thermodynamic limit of an infinite number of atoms. Moreover, when a finite number of atoms is considered, the variance of the fluctuation around the critical point asymptotically converges to zero, as the number of atoms is increased. In contrast to the squeezed states of flying photons obtained using standard generation protocols with external driving, the squeezing obtained in the ground state of the ultrastrongly coupled photon-atom systems is resilient against unpredictable noise.

Ultrastrong magnon-magnon coupling dominated by antiresonant interactions.

Exotic quantum vacuum phenomena are predicted in cavity quantum electrodynamics systems with ultrastrong light-matter interactions. Their ground states are predicted to be vacuum squeezed states with suppressed quantum fluctuations owing to antiresonant terms in the Hamiltonian. However, such predictions have not been realized because antiresonant interactions are typically negligible compared to resonant interactions in light-matter systems. Here we report an unusual, ultrastrongly coupled matter-matter system of magnons that is analytically described by a unique Hamiltonian in which the relative importance of resonant and antiresonant interactions can be easily tuned and the latter can be made vastly dominant. We found a regime where vacuum Bloch-Siegert shifts, the hallmark of antiresonant interactions, greatly exceed analogous frequency shifts from resonant interactions. Further, we theoretically explored the system's ground state and calculated up to 5.9 dB of quantum fluctuation suppression. These observations demonstrate that magnonic systems provide an ideal platform for exploring exotic quantum vacuum phenomena predicted in ultrastrongly coupled light-matter systems.

Entangled-photon generation in nano-to-bulk crossover regime.

We have theoretically investigated the generation of entangled photons from biexcitons in a semiconductor film with a thickness in the nano-to-bulk crossover regime. In contrast with the cases of quantum dots and bulk materials, we can highly control the generated state of entangled photons through the design of a peculiar energy structure of exciton-photon coupled modes in the thickness range between nanometers and micrometers. Owing to the enhancement of the radiative decay rate of excitons (exciton superradiance), the statistical accuracy of generated photons can be increased beyond the trade-off problem with signal intensity. By implementing an optical cavity structure in the strong-coupling regime, the generation efficiency can be enhanced while maintaining the high statistical accuracy.

Quantum squeezing generation versus photon localization in a disordered planar microcavity.

We investigate theoretically the nonlinear dynamics induced by an intense pump field in a disordered planar microcavity. Through a self-consistent theory, we show how the generation of quantum optical noise squeezing is affected by the breaking of the in-plane translational invariance and the occurrence of photon localization. We find that the generation of single-mode Kerr squeezing for the ideal planar case can be prevented by disorder as a result of multimode nonlinear coupling, even when the other modes are in the vacuum state. However, the excess noise is a nonmonotonic function of the disorder amplitude. In the strong localization limit, we show that the system becomes protected with respect to this fundamental coupling mechanism and that the ideal quadrature squeezing generation can be obtained.

Observation of Dicke cooperativity in magnetic interactions.

The interaction of N two-level atoms with a single-mode light field is an extensively studied many-body problem in quantum optics, first analyzed by Dicke in the context of superradiance. A characteristic of such systems is the cooperative enhancement of the coupling strength by a factor of N. In this study, we extended this cooperatively enhanced coupling to a solid-state system, demonstrating that it also occurs in a magnetic solid in the form of matter-matter interaction. Specifically, the exchange interaction of N paramagnetic erbium(III) (Er3+) spins with an iron(III) (Fe3+) magnon field in erbium orthoferrite (ErFeO3) exhibits a vacuum Rabi splitting whose magnitude is proportional to N. Our results provide a route for understanding, controlling, and predicting novel phases of condensed matter using concepts and tools available in quantum optics.