Dissipative Kerr soliton generation at 2µm in a silicon nitride microresonator.

Chip-scale optical frequency combs enable the generation of highly-coherent pulsed light at gigahertz-level repetition rates, with potential technological impact ranging from telecommunications to sensing and spectroscopy. In combination with techniques such as dual-comb spectroscopy, their utilization would be particularly beneficial for sensing of molecular species in the mid-infrared spectrum, in an integrated fashion. However, few demonstrations of direct microcomb generation within this spectral region have been showcased so far. In this work, we report the generation of Kerr soliton microcombs in silicon nitride integrated photonics. Leveraging a high-Q silicon nitride microresonator, our device achieves soliton generation under milliwatt-level pumping at 1.97 µm, with a generated spectrum encompassing a 422 nm bandwidth and extending up to 2.25 µm. The use of a dual pumping scheme allows reliable access to several comb states, including primary combs, modulation instability combs, as well as multi- and single-soliton states, the latter exhibiting high stability and low phase noise. Our work extends the domain of silicon nitride based Kerr microcombs towards the mid-infrared using accessible factory-grade technology and lays the foundations for the realization of fully integrated mid-infrared comb sources.

Observation of modulation instability in a coherently driven active fiber ring resonator at 2 µm wavelength.

We report the first, to our knowledge, observation of the nonlinear phenomenon known as modulation instability (MI) in a coherently driven fiber resonator pumped at 1972 nm. To compensate for the very high losses in this spectral region, we have integrated a thulium-doped fiber amplifier inside the cavity. Lower losses allow a lower MI threshold, leading to the observation of this phenomenon at a moderate input power. The results align closely with the numerical simulations of the system. Our study shows that active compensation of loss can be implemented in the 2 µm wavelength range to construct fiber ring cavities with high finesse. It paves the way to the observation of more complex nonlinear effects optical frequency comb through cavity soliton generation.

Cost-effective equalization of electro-optic frequency combs in a Sagnac interferometer.

We present a cost-effective electro-optic frequency comb generation and equalization method using a single phase modulator inserted in a Sagnac interferometer layout. The equalization relies on the interference of comb lines generated in both clockwise and counter-clockwise directions. Such a system is capable of providing flat-top combs with flatness values comparable with other approaches proposed in literature, yet offering a simplified synthesis and reduced complexity. The frequency range of operation at hundreds of MHz renders this scheme particularly interesting for some sensing and spectroscopy applications.

Towards efficient broadband parametric conversion in ultra-long Si3N4 waveguides.

Broadband continuous-wave parametric gain and efficient wavelength conversion is an important functionality to bring on-chip. Recently, meter-long silicon nitride waveguides have been utilized to obtain continuous-traveling-wave parametric gain, establishing the great potential of photonic-integrated-circuit-based parametric amplifiers. However, the effect of spiral structure on the performance and achievable bandwidth of such devices have not yet been studied. In this work, we investigate the efficiency-bandwidth performance in up to 2 meter-long waveguides engineered for broadband operation. Moreover, we analyze the conversion efficiency fluctuations that have been observed in meter-long Si3N4 waveguides and study the use of temperature control to limit the fluctuations.

Tunable photo-induced second-harmonic generation in a mode-engineered silicon nitride microresonator.

All-optical poling enables reconfigurable and efficient quasi-phase-matching for second-order parametric frequency conversion in silicon nitride integrated photonics. Here, we report broadly tunable milliwatt-level second-harmonic generation in a small free spectral range silicon nitride microresonator, where the pump and its second-harmonic are both always on the fundamental mode. By carefully engineering the light coupling region between the bus and microresonator, we simultaneously achieve critical coupling of the pump as well as efficient extraction of second-harmonic light from the cavity. Thermal tuning of second-harmonic generation is demonstrated with an integrated heater in a frequency grid of 47 GHz over a 10 nm band.

Integrated Backward Second-Harmonic Generation through Optically Induced Quasi-Phase-Matching.

Quasi-phase-matching for efficient backward second-harmonic generation requires sub-µm poling periods, a nontrivial fabrication feat. For the first time, we report integrated first-order quasiphase-matched backward second-harmonic generation enabled by seeded all-optical poling. The self-organized grating inscription circumvents all fabrication challenges. We compare backward and forward processes and explain how grating period influences the conversion efficiency. These results showcase unique properties of the coherent photogalvanic effect and how it can bring new nonlinear functionalities to integrated photonics.

Polarization selective ultra-broadband wavelength conversion in silicon nitride waveguides.

We experimentally demonstrate broadband degenerate continuous-wave four-wave mixing in long silicon nitride (Si3N4) waveguides for operation both in the telecommunication L-band and the thulium band near 2 µm by leveraging polarization dependence of the waveguide dispersion. Broadband conversion is typically demonstrated in short milimeter long waveguides as the bandwidth is linked to the interaction length. This makes it challenging to simultaneously push bandwidth and efficiency, imposing stringent constraints on dispersion engineering. In this work, we show conversion bandwidths larger than 150 nm in the L-band when pumping in the transverse magnetic (TM) mode and larger than 120 nm at 2 µm when using transverse electric excitation, despite the use of 0.5 m long waveguides. In addition, we also show how extreme polarization selectivity can be leveraged in a single waveguide to enable switchable distant phase-matching based on higher-order dispersion. Relying on this approach, we demonstrate the selective conversion of light from the telecom band to the O-band for TM polarization or to the mid-infrared light up to 2.5 µm in TE. Our experiments are in excellent agreement with simulations, showing the high potential of the platform for broadband and distant conversion beyond the telecom band.

Near perfect two-photon interference out of a down-converter on a silicon photonic chip.

Integrated entangled photon-pair sources are key elements for enabling large-scale quantum photonic solutions and address the challenges of both scaling-up and stability. Here we report the first demonstration of an energy-time entangled photon-pair source based on spontaneous parametric down-conversion in silicon-based platform-stoichiometric silicon nitride (Si3N4)-through an optically induced second-order (χ(2)) nonlinearity, ensuring type-0 quasi-phase-matching of fundamental harmonic and its second-harmonic inside the waveguide. The developed source shows a coincidence-to-accidental ratio of 1635 for 8 µW pump power. We report two-photon interference with remarkable near-perfect visibility of 99.36±1.94%, showing high-quality photonic entanglement without excess background noise. This opens a new horizon for quantum technologies requiring the integration of a large variety of building functionalities on a single chip.

Temporal Talbot effect of optical dark pulse trains.

The temporal Talbot effect describes the periodic self-imaging of an optical pulse train along dispersive propagation. This is well studied in the context of bright pulse trains, where identical or multiplied pulse trains with uniform bright waveforms can be created. However, the temporal self-imaging has remained unexplored in the dark pulse regime. Here, we disclose such a phenomenon for optical dark pulse trains, and discuss the comparison with their bright pulse counterparts. It is found that the dark pulse train also revives itself at the Talbot length. For higher-order fractional self-imaging, a mixed pattern of bright and dark pulses is observed, as a result of the interference between the Talbot pulses and the background. Such unconventional behaviors are theoretically predicted and experimentally demonstrated by using programmable spectral shaping as well as by optical fiber propagation.

Single-photon nonlinearities and blockade from a strongly driven photonic molecule.

Achieving the regime of single-photon nonlinearities in photonic devices by just exploiting the intrinsic high-order susceptibilities of conventional materials would open the door to practical semiconductor-based quantum photonic technologies. Here we show that this regime can be achieved in a triply resonant integrated photonic device made of two coupled ring resonators, in a material platform displaying an intrinsic third-order nonlinearity. By strongly driving one of the three resonances of the system, a weak coherent probe at one of the others results in a strongly suppressed two-photon probability at the output, evidenced by an antibunched second-order correlation function at zero-time delay under continuous wave driving.

Wavelength-stabilized tunable mode-locked thulium-doped fiber laser beyond 2 µm.

We report the development of a widely tunable mode-locked thulium-doped fiber laser based on a robust chirped fiber Bragg grating (CFBG). By applying mechanical tension and compression to the CFBG, an overall tunability of 20.1 nm, spanning from 2022.1 nm to 2042.2 nm, was achieved. The observed mode-locked pulse train from this fiber laser has a repetition rate of 9.4 MHz with an average power of 12.6 dBm and a pulse duration between 9.0 ps and 12.8 ps, depending on the central wavelength. To the best of our knowledge, this is the first demonstration of a tunable mode-locked thulium-doped fiber laser operating beyond 2 µm using a CFBG as a wavelength-selective element.

Extreme polarization-dependent supercontinuum generation in an uncladded silicon nitride waveguide.

We experimentally demonstrate the generation of a short-wave infrared supercontinuum in an uncladded silicon nitride (Si3N4) waveguide with extreme polarization sensitivity at the pumping wavelength of 2.1 µm. The air-clad waveguide is specifically designed to yield anomalous dispersion regime for transverse electric (TE) mode excitation and all-normal-dispersion (ANDi) at near-infrared wavelengths for the transverse magnetic (TM) mode. Dispersion engineering of the polarization modes allows for switching via simple adjustment of the input polarization state from an octave-spanning soliton fission-driven supercontinuum with fine spectral structure to a flat and smooth ANDi supercontinuum dominated by a self-phase modulation mechanism (SPM). Such a polarization sensitive supercontinuum source offers versatile applications such as broadband on-chip sensing to pulse compression and few-cycle pulse generation. Our experimental results are in very good agreement with numerical simulations.

Highly tunable second-harmonic generation in all-optically poled silicon nitride waveguides.

The availability of nonlinear parametric processes, such as frequency conversion in photonic integrated circuits is essential. In this contribution, we demonstrate a highly tunable second-harmonic generation in a fully complementary metal-oxide-semiconductor (CMOS)-fabrication-compatible silicon nitride integrated photonic platform. We induce the second-order nonlinearity using an all-optical poling technique with the second-harmonic light generated in the fundamental mode, and a narrow quasi-phase matching (QPM) spectrum by avoiding higher-order mode mixing. We are then able to broadly tune the phase-matched pump wavelength over the entire C-band (1540 nm to 1560 nm) by varying the poling conditions. Fine-tuning of QPM is enabled by thermo-optic effect with the tuning slope Δλ/ΔT in our device being 113.8 pm/°C. In addition, we exploit the measurable variation of the 3 dB QPM bandwidth to confirm how the length of the all-optically inscribed grating varies with exposure time.

Parallel gas spectroscopy using mid-infrared supercontinuum from a single Si3N4 waveguide.

Efficient third-order nonlinear optical processes have been successfully integrated on silicon nitride (Si3N4) waveguides. In particular, owing to Si3N4 wide transparency window spanning from the visible to the middle-infrared (mid-IR), efficient mid-IR dispersive-wave (DW) generation from a fiber laser has been recently demonstrated, and its potential as a source for absorption spectroscopy of a single gas has been established. Here we show that the system can be further engineered to broaden the coverage of a single DW without losing efficiency, as to enable simultaneous and discrete detection of several gas-phase molecules within the 2900 and 3380cm-1 functional group region. We demonstrate quantitative detection of acetylene, methane, and ethane using a simple direct-absorption spectroscopy scheme, achieving a several hundreds of parts-per-million noise-equivalent detection limit with a 5 cm long gas cell.

Investigation of temporal Talbot operation in a conventional optical tapped delay line structure.

We propose a novel scheme of temporal Talbot effect achieving optical pulse train repetition-rate multiplication in a conventional tapped delay line structure. While it is generally used for spectral amplitude filtering, we show that such architecture could also be configured for spectral phase-only filtering, as well as for a combination of amplitude and phase filtering regimes. We theoretically derive and numerically simulate the working principle of the concept, followed by a proof-of-principle experimental demonstration using an off-the-shelf Mach-Zehnder delay line interferometer, which corresponds to the simplest version of the proposed structure. We address the efficiency, and potential performance degradation in the presence of power imbalance and delay line length inaccuracy of the architecture, together with applied phase error.

Second- and third-order nonlinear wavelength conversion in an all-optically poled Si3N4 waveguide.

Silicon nitride (Si3N4) is commonly employed to integrate third-order nonlinear optical processes on a chip. Its amorphous state, however, inhibits significant second-order nonlinear response. Recently, second-harmonic generation enhancement has been observed in Si3N4 waveguides after an all-optical poling (AOP) method. Here we demonstrate that, after AOP of a Si3N4 waveguide, for up to 2 W of coupled pump power, the same telecom-band signal undergoes larger interband wavelength conversion efficiency, based on sum-frequency generation (SFG), than intraband wavelength conversion, based on four-wave mixing. We also confirm the appearance of a phase-matching condition after AOP by measuring the conversion bandwidth and efficiency of SFG at different pump wavelengths.

Linearly chirped mid-infrared supercontinuum in all-normal-dispersion chalcogenide photonic crystal fibers.

We demonstrate all-normal dispersion supercontinuum generation in chalcogenide photonic crystal fibers pumped at 2070-2080 nm with a femtosecond fiber laser. At 2.9 kW peak power, the generated supercontinuum has a 3 dB bandwidth of 27.6 THz and -20 dB bandwidth of 75.5 THz. We experimentally investigated the supercontinuum evolution inside our sample fiber at various peak powers and fiber lengths and study the impact of fiber water absorption on the generated supercontinuum spectrum. Multiple tests with fiber length- ranging from 0.34 to 10 cm-provide insight on pulse evolution along fiber length. Our simulations, which utilizes the generalized nonlinear Schrodinger equation model, match perfectly the experiments for all tested pump powers and fiber lengths, and confirm that the output pulse has a linear chirp, allowing linear pulse compression.

Talbot effect on orbital angular momentum beams: azimuthal intensity repetition-rate multiplication.

We propose and experimentally demonstrate the azimuthal Talbot effect on orbital angular momentum (OAM) beams. By applying predetermined phases to a number of OAM beams carrying different topological charges, the intensity petal is self-imaged in the azimuthal angle, with arbitrary azimuthal repetition-rate multiplication. The close analogy between temporal and azimuthal Talbot self-imaging is studied. In addition, the effect of amplitude apodization of the OAM spectrum on the resulting intensity pattern, and the azimuthal Talbot effect on Laguerre-Gaussian beams of the same radial indices, are experimentally investigated. All of our experimental images are in excellent agreement with simulation results.

Fiber fuse in chalcogenide photonic crystal fibers.

We observe fiber fuse in tapered GeAsSe photonic crystal fibers (PCF) at around 7 MW/cm2 of intra-core intensity. Vertically cleaved facets from the un-tapered regions and the tapered regions were imaged. The images show shallow voids of different shapes confined to the fiber core. After longitudinally polishing a segment of the PCF, we imaged the PCF internal structure's top view, revealing the fuse voids' geometries and periodicity. In addition, fiber fuse was terminated in one PCF sample by a fast laser shutdown, hence saving a small segment from catastrophic damage. Four-wave-mixing was performed on this transmissive segment to estimate the dispersion. The results yielded an evident hole-pitch ratio change after fiber fuse. To our knowledge, this is the first report of fiber fuse on non-silica glass fibers and the first study of its aftermath on this un-destroyed segment of PCFs.

Characterization and modeling of microstructured chalcogenide fibers for efficient mid-infrared wavelength conversion.

We experimentally demonstrate wavelength conversion in the 2 µm region by four-wave mixing in an AsSe and a GeAsSe chalcogenide photonic crystal fibers. A maximum conversion efficiency of -25.4 dB is measured for 112 mW of coupled continuous wave pump in a 27 cm long fiber. We estimate the dispersion parameters and the nonlinear refractive indexes of the chalcogenide PCFs, establishing a good agreement with the values expected from simulations. The different fiber geometries and glass compositions are compared in terms of performance, showing that GeAsSe is a more suited candidate for nonlinear optics at 2 µm. Building from the fitted parameters we then propose a new tapered GeAsSe PCF geometry to tailor the waveguide dispersion and lower the zero dispersion wavelength (ZDW) closer to the 2 µm pump wavelength. Numerical simulations shows that the new design allows both an increased conversion efficiency and bandwidth, and the generation of idler waves further in the mid-IR regions, by tuning the pump wavelength in the vicinity of the fiber ZDW.