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1.
Air Qual Atmos Health ; 15(7): 1205-1220, 2022.
Artigo em Inglês | MEDLINE | ID: mdl-34840623

RESUMO

Abstract: During the COVID-19 pandemic, restrictive measures are taken by several cities around the world, as well as Rio de Janeiro, reducing routine activities in large urban centers and primary pollutant emissions. This study aims to assess air quality during this partial lockdown through O3, CO, and PM10 concentrations and meteorological data collected in five air quality monitoring stations spread over the whole city, considering the substantial changes in city routine. The period evaluated starts in March 2020, when the partial lockdown was decreed, and ends in September 2020, when economic opening ended. Compared with 2019 data, CO concentration reduced significantly, as expected since the main source of these pollutants is vehicular traffic. O3 concentration increased, most probably as a consequence of the reduction in primary pollutants. On the other hand, PM10 concentration did not vary significantly. From June to September, pollutant concentrations increased responding to the economic opening. Thereby, the partial lockdown contributed to improving air quality in Rio de Janeiro City, which means that changes in work format may be an alternative to reduce atmospheric pollution in big cities, since home office contributes to mobility reductions, and consequently to vehicular emissions. Highlights: • Lockdown contributed to CO reduction and O3 increase.• Differences on rain profile explain low variation on PM10 concentrations.• Lockdown has been like a very long weekend concerning atmospheric pollution.• Home office and distance learning improve air quality. Supplementary Information: The online version contains supplementary material available at 10.1007/s11869-021-01127-2.

2.
J Geophys Res Atmos ; 126(8): e2020JD034213, 2021 Apr.
Artigo em Inglês | MEDLINE | ID: mdl-34230871

RESUMO

We use the global Community Earth System Model to investigate the response of secondary pollutants (ozone O3, secondary organic aerosols SOA) in different parts of the world in response to modified emissions of primary pollutants during the COVID-19 pandemic. We quantify the respective effects of the reductions in NOx and in volatile organic carbon (VOC) emissions, which, in most cases, affect oxidants in opposite ways. Using model simulations, we show that the level of NOx has been reduced by typically 40% in China during February 2020 and by similar amounts in many areas of Europe and North America in mid-March to mid-April 2020, in good agreement with space and surface observations. We show that, relative to a situation in which the emission reductions are ignored and despite the calculated increase in hydroxyl and peroxy radicals, the ozone concentration increased only in a few NOx-saturated regions (northern China, northern Europe, and the US) during the winter months of the pandemic when the titration of this molecule by NOx was reduced. In other regions, where ozone is NOx-controlled, the concentration of ozone decreased. SOA concentrations decrease in response to the concurrent reduction in the NOx and VOC emissions. The model also shows that atmospheric meteorological anomalies produced substantial variations in the concentrations of chemical species during the pandemic. In Europe, for example, a large fraction of the ozone increase in February 2020 was associated with meteorological anomalies, while in the North China Plain, enhanced ozone concentrations resulted primarily from reduced emissions of primary pollutants.

3.
Nat Commun ; 12(1): 5197, 2021 08 31.
Artigo em Inglês | MEDLINE | ID: mdl-34465790

RESUMO

The energy demand for heating and cooling buildings is changing with global warming. Using proxies of climate-driven energy demand based on the heating and cooling Degree-Days methodology applied to thirty global climate model simulations, we show that, over all continental areas, the climate-driven energy demand trends for heating and cooling were weak, changing by less than 10% from 1950 to 1990, but become stronger from 1990 to 2030, changing by more than 10%. With the multi-model mean, the increasing trends in cooling energy demand are more pronounced than the decreasing trends in heating. The changes in cooling, however, are highly variable depending on individual simulations, ranging from a few to several hundred percent in most of the densely populated mid-latitude areas. This work presents an example of the challenges that accompany future energy demand quantification as a result of the uncertainty in the projected climate.

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