Low-loss VIS/IR-XUV beam splitter for high-power applications.

We present a low-loss VIS/IR-XUV beam splitter, suitable for high-power operation. The spatial separation of the VIS/IR and XUV components of a beam is achieved by the wedged top layer of a dielectric multilayer structure, onto which the beam is impinging under Brewster's angle (for VIS/IR). With a fused silica wedge with an angle of 0.5° we achieve a separation angle of 2.2° and an IR reflectivity of 0.9995. Typical XUV reflectivities amount to 0.1-0.2. The novel element is mechanically robust, exhibiting two major advantages over free-standing Brewster plates: (i) a significant improvement of heat conduction and (ii) easier handling, in particular for high-optical-quality fabrication. The beam splitter could be used as an output coupler for intracavity-generated XUV radiation, promising a boost of the power regime of current MHz-HHG experiments. It is also suited for single-pass experiments and as a beam combiner for pump-probe experiments.

Kinetics of ultrashort relativistic electron pulses emitted from solid targets.

Interaction of ultrashort high-intensity laser pulses with solid targets generates relativistic electrons which escape from the target. The kinetics of these ultrashort electron pulses is governed by self-fields generated by the charge of the electron cloud. In this paper an analytical theory is developed which allows calculation of electron trajectories, electron fluxes, and electron spectra at any distance from the target. The theory is exact for two limiting cases: (a) a monoenergetic electron pulse with an arbitrary temporal shape; (b) an infinitely short electron pulse with an arbitrary energy spectrum. These results have applications in high-intensity irradiation experiments, e.g., in experiments irradiating samples with ultrashort electron or x-ray pulses, in developing optics for fourth-generation light sources, and in work relating to x-ray lasers.

Preplasma conditions for operation of 10-Hz subjoule femtosecond-laser-pumped nickel-likex-ray lasers.

We present measurements of electron densities of plasmas with femtosecond (fs) temporal resolution. The plasmas are generated by laser pulses with different intensities at different time delays. Such plasmas are of great interest as preplasmas for transient, collisionally excited x-ray lasers. The laser pulses producing the plasmas are generated by stretching part of a 130-fs laser pulse of the ATLAS titanium-sapphire laser of our institute and focusing this radiation to a line on molybdenum and silver slab targets. The electron density is measured as a function of distance from the target by interferometry using a Wollaston prism. Using an ultrashort probe pulse allows one to obtain data extremely close, about 10 microm, to the target surface. Experimental data are compared with simulations using the MULTI hydrocode. The results allow comparison of the ablation from a hard (Mo) and a soft (Ag) material, optimization of prepulse-main pulse delay times, and selection of the best pump geometry allowing for propagation of the pump and x-ray beams. These points are key elements for the development of a high-repetition-rate soft-x-ray laser.

Time-resolved electron diffraction from selectively aligned molecules.

We experimentally demonstrate ultrafast electron diffraction from transiently aligned molecules in the absence of external (aligning) fields. A sample of aligned molecules is generated through photodissociation with femtosecond laser pulses, and the diffraction pattern is captured by probing the sample with picosecond electron pulses shortly after dissociation-before molecular rotation causes the alignment to vanish. In our experiments the alignment decays with a time constant of 2.6+/-1.2 ps.