Depletion-limited Kerr solitons in singly resonant optical parametric oscillators.

We analyze the impact of pump depletion in the generation of parametrically driven Kerr cavity solitons in a degenerate optical parametric oscillator. Using variational methods, we derive an analytical expression that describes the soliton existence region. We use this expression to study the energy conversion efficiency and compare it to a linearly driven Kerr resonator modeled by the Lugiato-Lefever equation. Parametric driving is more efficient at high walk-off between the continuous wave driving and the soliton.

Modulated super-Gaussian laser pulse to populate a dark rovibrational state of acetylene.

A pulse-shaping technique in the mid-infrared spectral range based on pulses with a super-Gaussian temporal profile is considered for laser control. We show a realistic and efficient path to the population of a dark rovibrational state in acetylene (C2H2). The laser-induced dynamics in C2H2 are simulated using fully experimental structural parameters. Indeed, the rotation-vibration energy structure, including anharmonicities, is defined by the global spectroscopic Hamiltonian for the ground electronic state of C2H2 built from the extensive high-resolution spectroscopy studies on the molecule, transition dipole moments from intensities, and the effects of the (inelastic) collisions that are parameterized from line broadenings using the relaxation matrix [A. Aerts, J. Vander Auwera, and N. Vaeck, J. Chem. Phys. 154, 144308 (2021)]. The approach, based on an effective Hamiltonian, outperforms today's ab initio computations both in terms of accuracy and computational cost for this class of molecules. With such accuracy, the Hamiltonian permits studying the inner mechanism of theoretical pulse shaping [A. Aerts et al., J. Chem. Phys. 156, 084302 (2022)] for laser quantum control. Here, the generated control pulse presents a number of interferences that take advantage of the control mechanism to populate the dark state. An experimental setup is proposed for in-laboratory investigation.

Mode-locking induced by coherent driving in fiber lasers.

Mode-locking is a broad concept that encompasses different processes enabling short optical pulse formation in lasers. It typically requires an intracavity mechanism that discriminates between single and collective mode lasing, which can be complex and sometimes adds noise. Moreover, known mode-locking schemes do not guarantee phase stability of the carrier wave. Here, we theoretically propose that injecting a detuned signal seamlessly leads to mode-locking in fiber lasers. We show that phase-locked pulses, akin to cavity solitons, exist in a wide range of parameters. In that regime the laser behaves as a passive resonator due to the non-instantaneous gain saturation.

Laser control of a dark vibrational state of acetylene in the gas phase-Fourier transform pulse shaping constraints and effects of decoherence.

We propose a methodology to tackle the laser control of a non-stationary dark ro-vibrational state of acetylene (C2H2), given realistic experimental limitations in the 7.7 µm (1300 cm-1) region. Simulations are performed using the Lindblad master equation, where the so-called Lindblad parameters are used to describe the effect of the environment in the dilute gas phase. A phenomenological representation of the parameters is used, and they are extracted from high-resolution spectroscopy line broadening data. An effective Hamiltonian is used for the description of the system down to the rotational level close to experimental accuracy. The quality of both the Hamiltonian and Lindblad parameters is assessed by a comparison of a calculated infrared spectrum with the available experimental data. A single shaped laser pulse is used to perform the control, where elements of optics and pulse shaping using masks are introduced with emphasis on experimental limitations. The optimization procedure, based on gradients, explicitly takes into account the experimental constraints. Control performances are reported for shaping masks of increasing complexity. Although modest performances are obtained, mainly due to the strong pulse shaping constraints, we gain insights into the control mechanism. This work is the first step toward the conception of a realistic experiment that will allow for population characterization and manipulation of a non-stationary vibrational "dark" state. Effects of the collisions on the laser control in the dilute gas phase, leading to decoherence in the molecular system, are clearly shown.

Self-pulsing and chaos in the asymmetrically driven dissipative photonic Bose-Hubbard dimer: A bifurcation analysis.

We perform a systematic study of the temporal dynamics emerging in the asymmetrically driven dissipative Bose-Hubbard dimer model. This model successfully describes the nonlinear dynamics of photonic diatomic molecules in linearly coupled Kerr resonators coherently excited by a single laser beam. Such temporal dynamics may include self-pulsing oscillations, period doubled oscillatory states, chaotic dynamics, and spikes. We have thoroughly characterized such dynamical states, their origin, and their regions of stability by applying bifurcation analysis and dynamical system theory. This approach has allowed us to identify and classify the instabilities, which are responsible for the appearance of different types of temporal dynamics.

Efficient type II second harmonic generation in an indium gallium phosphide on insulator wire waveguide aligned with a crystallographic axis.

We theoretically and experimentally investigate type II second harmonic generation in III-V-on-insulator wire waveguides. We show that the propagation direction plays a crucial role and that longitudinal field components can be leveraged for robust and efficient conversion. We predict that the maximum theoretical conversion is larger than that of type I second harmonic generation for similar waveguide dimensions and reach an experimental conversion efficiency of 12%/W, limited by the propagation loss.

Influence of longitudinal mode components on second harmonic generation in III-V-on-insulator nanowires.

The large index contrast and the subwalength tranverse dimensions of nanowires induce strong longitudinal electric field components. We show that these components play an important role for second harmonic generation in III-V wire waveguides. To illustrate this behavior, an efficiency map of nonlinear conversion is determined based on full-vectorial calculations. It reveals that many different waveguide dimensions and directions are suitable for efficient conversion of a fundamental quasi-TE pump mode around the 1550 nm telecommunication wavelength to a higher-order second harmonic mode.

Enhancement of nonlinear functionality of step-index silica fibers combining thermal poling and 2D materials deposition.

This work proposes a new route to overcome the limits of the thermal poling technique for the creation of second order nonlinearity in conventional silica optical fibers. We prove that it is possible to enhance the nonlinear behavior of periodically poled fibers merging the effects of poling with the nonlinear intrinsic properties of some materials, such as MoS2, which are deposited inside the cladding holes of a twin-hole silica fiber. The optical waves involved in a second harmonic generation process partially overlap inside the thin film of the nonlinear material and exploit its higher third order susceptibility to produce an enhanced SHG.

Single is better than double: theoretical and experimental comparison between two thermal poling configurations of optical fibers.

Thermal poling, a technique to create permanently effective second-order susceptibility in silica optical fibers, has a suite of applications including frequency conversion and mixing for high harmonic generation and phase sensitive amplification, optical switching and modulation, and polarization-entangled photon pair generation. In this work, we compare both theoretically and experimentally two different electrode configurations for poling optical fibers, namely double-anode and single-anode, for two different geometries of the cladding holes. This analysis reveals that the single-anode configuration is optimal, both for the absolute value of effective χ (2) created in the fiber core, and for the simplification of the fiber fabrication process.

Observation of an optical event horizon in a silicon-on-insulator photonic wire waveguide.

We report on the first experimental observation of an optical analogue of an event horizon in integrated nanophotonic waveguides, through the reflection of a continuous wave on an intense pulse. The experiment is performed in a dispersion-engineered silicon-on-insulator waveguide. In this medium, solitons do not suffer from Raman induced self-frequency shift as in silica fibers, a feature that is interesting for potential applications of optical event horizons. As shown by simulations, this also allows the observation of multiple reflections at the same time on fundamental solitons ejected by soliton fission.

Scattering of a cross-polarized linear wave by a soliton at an optical event horizon in a birefringent nanophotonic waveguide.

The scattering of a linear wave on an optical event horizon, induced by a cross-polarized soliton, is experimentally and numerically investigated in integrated structures. The experiments are performed in a dispersion-engineered birefringent silicon nanophotonic waveguide. In stark contrast with copolarized waves, the large difference between the group velocity of the two cross-polarized waves enables a frequency conversion almost independent of the soliton wavelength. It is shown that the generated idler is only shifted by 10 nm around 1550 nm over a pump tuning range of 350 nm. Simulations using two coupled full vectorial nonlinear Schrödinger equations fully support the experimental results.

Measuring the nonlinear refractive index of graphene using the optical Kerr effect method.

By means of the ultrafast optical Kerr effect method coupled to optical heterodyne detection (OHD-OKE), we characterize the third-order nonlinear response of graphene and compare it to experimental values obtained by the Z-scan method on the same samples. From these measurements, we estimate a negative nonlinear refractive index for monolayer graphene, n2=-1.1×10-13 m2/W. This is in contradiction to previously reported values, which leads us to compare our experimental measurements obtained by the OHD-OKE and the Z-scan method with theoretical and experimental values found in the literature and to discuss the discrepancies, taking into account parameters such as doping.

Nonlinear properties of dispersion engineered InGaP photonic wire waveguides in the telecommunication wavelength range.

We propose high index contrast InGaP photonic wires as a platform for the integration of nonlinear optical functions in the telecom wavelength window. We characterize the linear and nonlinear properties of these waveguide structures. Waveguides with a linear loss of 12 dB/cm and which are coupled to a single mode fiber through gratings with a -7.5 dB coupling loss are realized. From four wave mixing experiments, we extract the real part of the nonlinear parameter γ to be 475 ± 50 W(-1)m(-1) and from nonlinear transmission measurements we infer the absence of two-photon absorption and measure a three-photon absorption coefficient of (2.5 ± 0.5) x 10(-2) cm(3)GW(-2).

3D super-resolved in vitro multiphoton microscopy by saturation of excitation.

We demonstrate a significant resolution enhancement beyond the conventional limit in multiphoton microscopy (MPM) using saturated excitation of fluorescence. Our technique achieves super-resolved imaging by temporally modulating the excitation laser-intensity and demodulating the higher harmonics from the saturated fluorescence signal. The improvement of the lateral and axial resolutions is measured on a sample of fluorescent microspheres. While the third harmonic already provides an enhanced resolution, we show that a further improvement can be obtained with an appropriate linear combination of the demodulated harmonics. Finally, we present in vitro imaging of fluorescent microspheres incorporated in HeLa cells to show that this technique performs well in biological samples.

Coherent supercontinuum generation in a silicon photonic wire in the telecommunication wavelength range.

We demonstrate a fully coherent supercontinuum spectrum spanning 500 nm from a silicon-on-insulator photonic wire waveguide pumped at 1575 nm wavelength. An excellent agreement with numerical simulations is reported. The simulations also show that a high level of two-photon absorption can essentially enforce the coherence of the spectral broadening process irrespective of the pump pulse duration.

Dispersive-wave-based octave-spanning supercontinuum generation in InGaP membrane waveguides on a silicon substrate.

We demonstrate the generation of an octave-spanning supercontinuum in InGaP membrane waveguides on a silicon substrate pumped by a 1550-nm femtosecond source. The broadband nature of the supercontinuum in these dispersion-engineered high-index-contrast waveguides is enabled by dispersive wave generation on both sides of the pump as well as by the low nonlinear losses inherent to the material. We also measure the coherence properties of the output spectra close to the pump wavelength and find that the supercontinuum is highly coherent at least in this wavelength range.

Supercontinuum generation in hydrogenated amorphous silicon waveguides at telecommunication wavelengths.

We report supercontinuum (SC) generation centered on the telecommunication C-band (1550 nm) in CMOS compatible hydrogenated amorphous silicon waveguides. A broadening of more than 550 nm is obtained in 1cm long waveguides of different widths using as pump picosecond pulses with on chip peak power as low as 4 W.

Dispersive wave emission and supercontinuum generation in a silicon wire waveguide pumped around the 1550 nm telecommunication wavelength.

We experimentally and numerically study dispersive wave emission, soliton fission, and supercontinuum generation in a silicon wire at telecommunication wavelengths. Through dispersion engineering, we experimentally confirm a previously reported numerical study and show that the emission of resonant radiation from the solitons can lead to the generation of a supercontinuum spanning over 500 nm. An excellent agreement with numerical simulations is observed.

Heat accumulation during infrared stimulation impacts the response of ex vivo rat sciatic nerve.

Infrared neural stimulation (INS) is a neuromodulation technique that involves short optical pulses delivered to the neural tissue, resulting in the initiation of action potentials. In this work, we studied the compound neural action potentials (CNAP) generated by INS in five ex vivo sciatic nerves. A 1470 nm laser emitting a sequence of 0.4 ms light pulses with a peak power of 10 W was used. A single 4 mJ stimulus is not capable of eliciting a nerve response. However, repetition of the optical stimuli resulted in the induction of CNAPs. Heat accumulation induced by repetition rates as high as 10 Hz may be involved in the increase in CNAP amplitude. This sensitization effect may help to reduce the pulse energy required to evoke CNAP. In addition, these results highlight the importance of investigating the role of the slow nerve temperature dynamics in INS.

Neck instability of bright solitons in normally dispersive Kerr media.

The neck instability of bright solitons of the hyperbolic nonlinear Shrödinger equation is investigated. It is shown that this instability originates from a four-wave mixing interaction that links on-axis to off-axis radiation at opposite frequency bands. Our experiment supports this interpretation.