Demonstration of an intense lithium beam for forward-directed pulsed neutron generation.

As an alternative to research nuclear reactors, a compact accelerator-driven neutron generator that uses a lithium beam driver could be a promising candidate since it produces almost no undesired radiation. However, providing an intense lithium-ion beam has been difficult, and it has been thought that the practical application of such a device would be impossible. The most critical problem of insufficient ion fluxes has been solved by applying a direct plasma injection scheme. In this scheme, a pulsed high-density plasma from a metallic lithium foil generated by laser ablation is efficiently injected and accelerated by a radio-frequency quadrupole linear accelerator (RFQ linac). We have obtained a peak beam current of 35 mA accelerated to 1.43 MeV, which is two orders of magnitude higher than a conventional injector and accelerator system can deliver.

Plasma instability inside solenoid with laser ion source.

Using a solenoid with a laser ion source can suppress divergence of the expanding plasma; however, it has been found that the plasma becomes unstable in a certain magnetic field region. In the previous research, instability of the plasma after the solenoid was found. In this study, we investigated how the plasma instability changes inside the solenoid. A Faraday cup was placed in the solenoid, and the unstable magnetic field range was investigated. This experiment was conducted while changing the Faraday cup position from the inlet to the outlet of the solenoid. By increasing the magnetic field strength, the Faraday cup position indicating a condition triggering instability moved toward upstream in the solenoid. In addition, the instability is gradually mitigated by transporting the laser ablation plasma through the rest of the solenoid. The detailed good working range of the solenoid for the Au1+ beam was also shown.

Evaluation of magnetic field error in ExtendedEBIS.

The upgrade of the EBIS, called ExtendedEBIS, is now in progress in Brookhaven National Laboratory. Two 5T-superconducting solenoids have been placed in series with 200 mm distance from each other for higher trap capacity and production of polarized 3He ions. Since the two superconducting solenoids are used, the field error is expected to be larger. In this research, the field error is estimated based on simulation. It was found that the magnetic field line can be 17 mm off from the center axis at the entrance of the collector, and this offset can be adjusted by three types of correction coils. Additionally, mismatch of the spin direction of polarized 3He due to the misalignment was estimated to be small.

Laser power density dependence on charge state distribution of Ta ion laser plasma.

Laser power density per pulse, which is commonly expressed with the unit of "W/cm2," is an important parameter to characterize ablation plasma. To match a design charge state of heavy ion beam induced by a laser ion source, a laser power density must be carefully chosen. Above around 108 W/cm2 of laser power density, laser ablation plasma is emitted from the surface of solid material. Then, up to 109 W/cm2, the most abundant charge state is 1+. Because the ionization energy increases with higher charge states, increasing the laser intensity leads to the charge state distribution shifting higher. Increasing the density to increase charge states also results in lower time of flight due to higher velocities. The maximum laser power density is obtained by the smallest available laser spot size on the target material which is determined by the quality of the laser beam. For many accelerator applications, higher charge state beams are preferred. In particular cases, singly charge ion beams are demanded. Therefore, production of intermediate charge state beams has not been investigated well. In this study, we selected Ta4+ as an example demanded beam and tried to clarify how the transition of charge state distribution depends on laser power density. Conclusively, the possible specification of a laser ion source for Ta4+ delivery was elucidated.

Neutron generator based on intense lithium beam driver.

We are proposing a compact neutron generator based on a Li beam driver. The proposed neutron generator comprises a laser ion source, a radio-frequency quadrupole linear accelerator (RFQ linac), a drift tube linac, and a target containing protons. In the generator, the lithium ion is used as a projectile instead of protons to utilize the kinematic focusing technique. The technique enables us to enhance the neutron flux without increasing the beam energy, which is important to develop a clean compact neutron generator. Moreover, the combination of a laser ion source and a RFQ linac with the direct plasma injection scheme will provide several tens of mA of a fully ionized lithium beam, which is much higher than that of conventional heavy ion sources comparable with proton drivers. Neutrons are generated by the nuclear reaction of the lithium ions and protons in the beam target. In this paper, we reported the current status of the development. For RFQ, we designed the RFQ rods to accelerate 40 mA of 7Li3+. We fabricated and installed the rods into a cavity, and, as a first test, accelerated 10 mA of C6+ successfully.

Low charge state lithium beam production from chemical compounds with laser ion source.

In recent years, the primary ion source for the Brookhaven National Laboratory has been the laser ion source, which provides many types of ions within a short switching time of several seconds. The task is difficult for other ion sources. In the previous work, we tested metallic lithium as a target material of the laser irradiation. Although an intense lithium beam was demonstrated, some operational difficulties were observed due to its reactiveness to oxygen. For accelerator applications, a more robust and reliable target material has been demanded. For this purpose, we tested lithium niobate, LiNbO3. Our study investigated the optimization of power density to produce low charge state lithium ions. We struck LiNbO3 with the laser and found lithium ion quantities for five different power densities. Based on the data obtained, we can conclude that the most efficient production of Li1+ occurs when the laser power density is 5 × 108 W/cm2.

Application of cryotarget to laser ion source.

We examined laser-produced argon plasma as part of a future laser ion source. Rare gases, which are in gas state at room temperature, need to be cooled to solid targets for laser irradiation. We generated solid Ar targets in a similar way used for neon. By irradiating the solid Ar with a neodymium doped yttrium aluminum garnet laser, we could generate Ar ions with a charge stage up to 8+ with a good stability. The feature of generated Ar plasma using this method is similar to the Ne case. The ion current density reached about 1.6 mA/cm(2) at 2.3 m from the target. This method would be applicable for a laser ion source.

Feasibility study of a laser ion source for primary ion injection into the Relativistic Heavy Ion Collider electron beam ion source.

Charge state 1+ions are required as a primary ion source for Relativistic Heavy Ion Collider-electron beam ion source (RHIC-EBIS) at BNL and laser ion source (LIS) is a candidate as one of the external ion source since low energy and low charge state ions can be generated by lower power density laser irradiation onto solid target surface. Plasma properties of (27)Al, (56)Fe, and (181)Ta using the second harmonics of Nd:yttrium aluminum garnet laser (0.73 J5.5 ns and 532 nm wavelength) for low charge state ion generation was measured. Charge state distribution of Ta was optimized for 1+with estimated laser power density of 9.1 x 10(8) Wcm(2) on the target. It has been shown that the LIS can produce sufficient ion charge with the appropriate pulse structure to satisfy injection requirements of the RHIC EBIS.

Ag ion generation irradiated by Nd:YAG laser onto solid target for use of direct plasma injection scheme.

Direct plasma injection scheme (DPIS) is an acceleration scheme which consists of laser ion source and a radio frequency quadrupole linac (RFQ) linac for high current heavy ion acceleration. With this scheme, over 60 mA of carbon and aluminum beam was achieved at the RFQ exit. We are planning to accelerate Ag ions as a heavier material than used previously. Ag plasma properties using Nd:YAG laser (2.3 J/6 ns) were measured toward the acceleration with DPIS. The results showed that the highest ion yield was obtained at Ag(15+). Based on these results, multicharged Ag ion transportation inside RFQ was simulated and the expected current at the exit of RFQ was over 14 mA for Ag(15+) using the RFQ dedicated for Ag acceleration.

Iron plasma generation using a Nd:YAG laser pulse of several hundred picoseconds.

We investigated the high intensity plasma generated by using a Nd:YAG laser to apply a laser-produced plasma to the direct plasma injection scheme. The capability of the source to generate high charge state ions strongly depends on the power density of the laser irradiation. Therefore, we focused on using a higher power laser with several hundred picoseconds of pulse width. The iron target was irradiated with the pulsed laser, and the ion current of the laser-produced iron plasma was measured using a Faraday cup and the charge state distribution was investigated using an electrostatic ion analyzer. We found that higher charge state iron ions (up to Fe(21+)) were obtained using a laser pulse of several hundred picoseconds in comparison to those obtained using a laser pulse of several nanoseconds (up to Fe(19+)). We also found that when the laser irradiation area was relatively large, the laser power was absorbed mainly by the contamination on the target surface.

Contribution of material's surface layer on charge state distribution in laser ablation plasma.

To generate laser ablation plasma, a pulse laser is focused onto a solid target making a crater on the surface. However, not all the evaporated material is efficiently converted to hot plasma. Some portion of the evaporated material could be turned to low temperature plasma or just vapor. To investigate the mechanism, we prepared an aluminum target coated by thin carbon layers. Then, we measured the ablation plasma properties with different carbon thicknesses on the aluminum plate. The results showed that C(6+) ions were generated only from the surface layer. The deep layers (over 250 nm from the surface) did not provide high charge state ions. On the other hand, low charge state ions were mainly produced by the deeper layers of the target. Atoms deeper than 1000 nm did not contribute to the ablation plasma formation.

Creation of mixed beam from alloy target and couple of pure targets with laser.

To create mixed species ion beam with laser pulses, we investigated charge state distributions of plasma formed from both Al-Fe alloy targets and pure Al and Fe targets placed close together. With two targets, we observed that the two kinds of atoms were mixed when the interval of two laser pulses was large enough (40 µs). On the other hand, when the interval was 0.0 µs, we observed fewer Fe ions and they did not mix well with the Al ions. The two species were mixed well in the plasma from the alloy target. Furthermore, we observed that specific charge states of Fe ions increased. From the results, it was determined that we can use two pure targets to mix two species whose difference of the drift velocity is large. On the other hand, we must use an alloy target when the drift velocities of the species are close.

Investigation of effect of solenoid magnet on emittances of ion beam from laser ablation plasma.

A magnetic field can increase an ion current of a laser ablation plasma and is expected to control the change of the plasma ion current. However, the magnetic field can also make some fluctuations of the plasma and the effect on the beam emittance and the emission surface is not clear. To investigate the effect of a magnetic field, we extracted the ion beams under three conditions where without magnetic field, with magnetic field, and without magnetic field with higher laser energy to measure the beam distribution in phase space. Then we compared the relations between the plasma ion current density into the extraction gap and the Twiss parameters with each condition. We observed the effect of the magnetic field on the emission surface.

Analyses of the plasma generated by laser irradiation on sputtered target for determination of the thickness used for plasma generation.

In Brookhaven National Laboratory, laser ion source has been developed to provide heavy ion beams by using plasma generation with 1064 nm Nd:YAG laser irradiation onto solid targets. The laser energy is transferred to the target material and creates a crater on the surface. However, only the partial material can be turned into plasma state and the other portion is considered to be just vaporized. Since heat propagation in the target material requires more than typical laser irradiation period, which is typically several ns, only the certain depth of the layers may contribute to form the plasma. As a result, the depth is more than 500 nm because the base material Al ions were detected. On the other hand, the result of comparing each carbon thickness case suggests that the surface carbon layer is not contributed to generate plasma.