Two-dimensional quasi periodic structures for large-scale light out-coupling with amplitude, phase and polarization control.

Chip-scale light-atom interactions are vital for the miniaturization of atomic sensing systems, including clocks, magnetometers, gyroscopes and more. Combining as many photonic elements as possible onto a photonic chip greatly reduces size and power consumption, where the critical elements are those interfacing between the 2D circuit and the 3D vapor cell. We introduce a new design method for large scale two-dimensional converter structures, enabling out-coupling of radiation from the photonic chip into the atomic medium. These structures allow light intensity and phase spatial distribution and polarization control, without external light-manipulating elements. Large, 100 × 100 µm2 structures were designed generating low divergence optical beams with high degree of circular polarization. Simulations obtain mean circular polarization contrast of better than 30 dB.

Lineshape study of optical force spectra on resonant structures.

Understanding the frequency spectrum of the optical force is important for controlling and manipulating micro- and nano-scale objects using light. Spectral resonances of these objects can significantly influence the optical force spectrum. In this paper, we develop a theoretical formalism based on the temporal coupled-mode theory that analytically describes the lineshapes of force spectra and their dependencies on resonant scatterers for arbitrary incident wavefronts. We obtain closed-form formulae and discuss the conditions for achieving symmetric as well as asymmetric lineshapes, pertaining, respectively, to a Lorentzian and Fano resonance. The relevance of formalism as a design tool is exemplified for a conceptual scheme of the size-sorting mechanism of small particles, which plays a role in biomedical diagnosis.

Functional Meta Lenses for Compound Plasmonic Vortex Field Generation and Control.

Surface plasmon polaritons carrying orbital angular momentum are of great fundamental and applied interest. However, common approaches for their generation are restricted to having a weak dependence on the properties of the plasmon-generating illumination, providing a limited degree of control over the amount of delivered orbital angular momentum. Here we experimentally show that by tailoring local and global geometries of vortex generators, a change in helicity of light imposes arbitrary large switching in the delivered plasmonic angular momentum. Using time-resolved photoemission electron microscopy we demonstrate pristine control over the generation and rotation direction of high-order plasmonic vortices. We generalize our approach to create complex topological fields and exemplify it by studying and controlling a "bright vortex", exhibiting the breakdown of a high-order vortex into a mosaic of unity-order vortices while maintaining the overall angular momentum density. Our results provide tools for plasmonic manipulation and could be utilized in lab-on-a-chip devices.

Universal Behavior of the Scattering Matrix Near Thresholds in Photonics.

Scattering thresholds and their associated spectral square root branch points are ubiquitous in photonics. In this Letter, we show that the scattering matrix has a simple universal behavior near scattering thresholds. We use unitarity, reciprocity, and time-reversal symmetry to construct a two-parameter model for a two-port scattering matrix near a threshold. We demonstrate this universal behavior in three different optical systems, namely, a photonic crystal slab, a planar dielectric interface, and a junction between metallic waveguides of different widths.

Theory for Twisted Bilayer Photonic Crystal Slabs.

We analyze scattering properties of twisted bilayer photonic crystal slabs through a high-dimensional plane wave expansion method. The method is applicable for arbitrary twist angles and does not suffer from the limitations of the commonly used supercell approximation. We show strongly tunable resonance properties of this system which can be accounted for semianalytically from a correspondence relation to a simpler structure. We also observe strongly tunable resonant chiral behavior in this system. Our work provides the theoretical foundation for predicting and understanding the rich optical physics of twisted multilayer photonic crystal systems.

Novel Ultra Localized and Dense Nitrogen Delta-Doping in Diamond for Advanced Quantum Sensing.

We introduce and demonstrate a new approach for nitrogen-vacancy (NV) patterning in diamond, achieving a deterministic, nanometer-thin, and dense delta-doped layer of negatively charged NV centers in diamond. We employed a pure nitridation stage using microwave plasma and a subsequent in situ diamond overgrowth. We present the highest reported nitrogen concentration in a delta-doped layer (1.8 × 1020 cm-3) while maintaining the pristine diamond crystal quality. This result combined with the large optically detected magnetic resonance contrast can pave the way toward highly sensitive NV-based magnetometers. We further employed this delta-doping technique on high-quality fabricated diamond nanostructures for realizing a topographic NV patterning in order to enhance the sensing and hyperpolarization capabilities of NV-based devices.

Maximal nighttime electrical power generation via optimal radiative cooling.

We present a systematic optimization of nighttime thermoelectric power generation system utilizing radiative cooling. We show that an electrical power density >2 W/m2, two orders of magnitude higher than the previously reported experimental result, is achievable using existing technologies. This system combines radiative cooling and thermoelectric power generation and operates at night when solar energy harvesting is unavailable. The thermoelectric power generator (TEG) itself covers less than 1 percent of the system footprint area when achieving this optimal power generation, showing economic feasibility. We study the influence of emissivity spectra, thermal convection, thermoelectric figure of merit and the area ratio between the TEG and the radiative cooler on the power generation performance. We optimize the thermal radiation emitter attached to the cold side and propose practical material implementation. The importance of the optimal emitter is elucidated by the gain of 153% in power density compared to regular blackbody emitters.

PT-Symmetric Topological Edge-Gain Effect.

We demonstrate a non-Hermitian topological effect that is characterized by having complex eigenvalues only in the edge states of a topological material, despite the fact that the material is completely uniform. Such an effect can be constructed in any topological structure formed by two gapped subsystems, e.g., a quantum spin-Hall system, with a suitable non-Hermitian coupling between the spins. The resulting complex-eigenvalued edge state is robust against defects due to the topological protection. In photonics, such an effect can be used for the implementation of topological lasers, in which a uniform pumping provides gain only in the edge lasing state. Furthermore, such a topological lasing model is reciprocal and is thus compatible with standard photonic platforms.

Doubly Resonant Nanoantennas on Diamond for Spatial Addressing of Spin States.

The negatively charged nitrogen-vacancy (NV) color center in diamond is an important atom-like system for emergent quantum technologies and sensing at room temperature. The light emission rates and collection efficiency are key issues toward realizing NV-based quantum devices. In that aspect, we propose and experimentally demonstrate a selective and spatially localized method for enhancing the light-matter interaction of shallow NV centers in bulk diamonds. This was achieved by polarized doubly resonant plasmonic antennas, tuned to the NV phonon sideband transition peak in the red and the narrowband near infrared (NIR) singlet transition. We obtained a photoluminescence (PL) enhancement factor of about 10 from NV centers within the hot spot of the antenna area (excluding the extraction efficiency enhancement) and similar emission lifetime reduction. The functionality of the double resonance antenna is controlled by the impinging light polarization.

Epitaxial Nanoflag Photonics: Semiconductor Nanoemitters Grown with Their Nanoantennas.

Semiconductor nanostructures are desirable for electronics, photonics, quantum circuitry, and energy conversion applications as well as for fundamental science. In photonics, optical nanoantennas mediate the large size difference between photons and semiconductor nanoemitters or detectors and hence are instrumental for exhibiting high efficiency. In this work we present epitaxially grown InP nanoflags as optically active nanostructures encapsulating the desired characteristics of a photonic emitter and an efficient epitaxial nanoantenna. We experimentally characterize the polarized and directional emission of the nanoflag-antenna and show the control of these properties by means of structure, dimensions, and constituents. We analyze field enhancement and light extraction by the semiconductor nanoflag antenna, which yield comparable values to enhancement factors of metallic plasmonic antennas. We incorporated quantum emitters within the nanoflag structure and characterized their emission properties. Merging of active nanoemitters with nanoantennas at a single growth process enables a new class of devices to be used in nanophotonics applications.

InP Nanoflag Growth from a Nanowire Template by in Situ Catalyst Manipulation.

Quasi-two-dimensional semiconductor materials are desirable for electronic, photonic, and energy conversion applications as well as fundamental science. We report on the synthesis of indium phosphide flag-like nanostructures by epitaxial growth on a nanowire template at 95% yield. The technique is based on in situ catalyst unpinning from the top of the nanowire and its induced migration along the nanowire sidewall. Investigation of the mechanism responsible for catalyst movement shows that its final position is determined by the structural defect density along the nanowire. The crystal structure of the "flagpole" nanowire is epitaxially transferred to the nanoflag. Pure wurtzite InP nanomembranes with just a single stacking fault originating from the defect in the flagpole that pinned the catalyst were obtained. Optical characterization shows efficient highly polarized photoluminescence at room temperature from a single nanoflag with up to 90% degree of linear polarization. Electric field intensity enhancement of the incident light was calculated to be 57, concentrated at the nanoflag tip. The presented growth method is general and thus can be employed for achieving similar nanostructures in other III-V semiconductor material systems with potential applications in active nanophotonics.

Linearly dichroic plasmonic lens and hetero-chiral structures.

We present an experimental study of Hetero-Chiral (HC) plasmonic lenses, comprised of constituents with opposite chirality, demonstrating linearly dichroic focusing. The lenses focus only light with a specific linear polarization and result in a dark focal spot for the orthogonal polarization state. We introduce the design concepts and quantitatively compare several members of the HC family, deriving necessary conditions for linear dichroism and several comparative engineering parameters. The HC lenses were experimentally investigated using aperture-less near field scanning microscope collecting the amplitude of the plasmonic near-field. Our results exhibit an excellent match to the simulation predictions. The demonstrated ability for linearly dichroic functional focusing could lead to novel sensing applications.

Metafocusing by a Metaspiral Plasmonic Lens.

We designed and realized a metasurface (manipulating the local geometry) spiral (manipulating the global geometry) plasmonic lens, which fundamentally overcomes the multiple efficiency and functionality challenges of conventional in-plane plasmonic lenses. The combination of spirality and metasurface achieves much more efficient and uniform linear-polarization-independent plasmonic focusing. As for functionality, under matched circularly polarized illumination the lens directs all of the power coupled to surface plasmon polaritons (SPPs) into the focal spot, while the orthogonal polarization excites only diverging SPPs that do not penetrate the interior of the lens, achieving 2 orders of magnitude intensity contrast throughout the entire area of the lens. This optimal functional focusing is clearly demonstrated by near-field optical microscopy measurements that are in excellent agreement with simulations and are supported by a detailed theoretical interpretation of the underlying mechanisms. Our results advance the field of plasmonics toward functional detection and the employment of SPPs in smart pixels, near-field microscopy, lithography, and particle manipulation.

Spin-patterned plasmonics: towards optical access to topological-insulator surface states.

Topological insulators (TI) are new phases of matter with topologically protected surface states (SS) possessing novel physical properties such as spin-momentum locking. Coupling optical angular momentum to the SS is of interest for both fundamental understanding and applications in future spintronic devices. However, due to the nanoscale thickness of the surface states, the light matter interaction is dominated by the bulk. Here we propose and experimentally demonstrate a plasmonic cavity enabling both nanoscale light confinement and control of surface plasmon-polariton (SPP) spin angular momentum (AM)--towards coupling to topological-insulator SS. The resulting SPP field components within the cavity are arranged in a chess-board-like pattern. Each chess-board square exhibits approximately a uniform circular polarization (spin AM) of the local in-plane field interleaved by out-of-plane field vortices (orbital AM). As the first step, we demonstrate the predicted pattern experimentally by near-field measurements on a gold-air interface, with excellent agreement to our theory. Our results pave the way towards efficient optical access to topological-insulator surface states using plasmonics.

Perfect Lensing by a Single Interface: Defying Loss and Bandwidth Limitations of Metamaterials.

Loss is known to be detrimental for achieving perfect focusing with the passive perfect lens designs suggested thus far, and it is believed to pose a fundamental barrier. We show that perfect lensing can be achieved with actual lossy left-handed metamaterials, without a need for gain or nonlinearity. The proposed loss-immune perfect lens is composed of a single interface between a conventional dielectric material on the source side and a lossy left-handed material on the image side. Its immunity to material loss was derived analytically using three complementary methodologies, confirming perfect lensing with point-to-point accuracy and shedding light on the underlying focusing mechanism. This result provides a new road map for practical realization of a near-field camera based on the single-interface lens design.

First demonstration of plasmonic GaN quantum cascade detectors with enhanced efficiency at normal incidence.

We have designed, fabricated and measured the first plasmon-assisted normal incidence GaN/AlN quantum cascade detector (QCD) making use of the surface plasmon resonance of a two-dimensional nanohole Au array integrated on top of the detector absorption region. The spectral response of the detector at room temperature is peaked at the plasmon resonance of 1.82 µm. We show that the presence of the nanohole array induces an absolute enhancement of the responsivity by a factor of ~30 over that of the bare device at normal incidence and by a factor of 3 with respect to illumination by the 45° polished side facet. We show that this significant improvement arises from two phenomena, namely, the polarization rotation of the impinging light from tangential to normal induced by the plasmonic structure and from the enhancement of the absorption cross-section per quantum well due to the near-field optical intensity of the plasmonic wave.

Measuring the refractive index around intersubband transition resonance in GaN/AlN multi quantum wells.

We present the direct measurement of the refractive index distribution (spectral dispersion) arising from an intersubband transition in GaN/AlN multi quantum wells structure. The measurement is carried out through a novel interferometric technique. The measured interferogram yields a change in the refractive index varying from -5 × 10(-3) to 6 × 10(-3) as a function of the wavelength, introduced by the intersubband resonance at 1.5 µm. These results compare well with those derived using Kramers-Kronig transform of the measured absorption spectrum.

Giant resonance absorption in ultra-thin metamaterial periodic structures.

We study the interaction of an incident plane wave with a metamaterial periodic structure consisting of alternating layers of positive and negative refractive index with average zero refractive index. We show that the existence of very narrow resonance peaks for which giant absorption - 50% at layer thickness of 1% of the incident wavelength - is exhibited. Maximum absorption is obtained at a specific layer thickness satisfying the critical coupling condition. This phenomenon is explained by the Rayleigh anomaly and by the excitation of Fabry Perot modes in the periodic layer. In addition, we investigate the modes supported by the structures for several limiting cases, and show that zero phase accumulation in the periodic metamaterial is obtained at resonance.

Thin wire shortening of plasmonic nanoparticle dimers: the reason for red shifts.

We studied experimentally and theoretically resonance characteristics of plasmonic nanoparticle dimers connected by a narrow metal wire. The "conductive" coupling between the particles results in complete redistribution of the surface charge yielding abrupt red shift of the plasmon resonance: detuning >900 nm and order of magnitude improvement in intensity enhancement. The resonance in the conductive coupling regime is determined completely by the characteristics of the unified particle and significantly different from that of capacitive coupling.

Resonances on-demand for plasmonic nano-particles.

A method for designing plasmonic particles with desired resonance spectra by exploiting the interaction of local geometry with surface charge distribution and applying evolutionary algorithm is presented. The method is based on repetitive perturbations of an initial particle's shape while calculating the eigenvalues of the various quasistatic resonances. Novel family of particles with collocated dipole-quadrupole resonances was designed, as an example for the unique power of the method.