Optical detection of attosecond ionization induced by a few-cycle laser field in a transparent dielectric material.

We observe an optical signature induced by the modulation of electron density inside a bulk transparent solid that is quasiperiodically ionized on an attosecond time scale by electric field peaks of a focused few-cycle laser pulse. The emitted optical signal resulting from the attosecond ionization dynamics is spatially, temporally and spectrally isolated from concomitant optical responses through the use of a noncollinear pump-probe technique. The method holds promise for developing an attosecond metrology for bulk solids, in which, unlike in the established attosecond metrology of gases and surfaces, direct detection of charged particles is unfeasible.

Optical detection of tunneling ionization.

We have experimentally detected optical harmonics that are generated due to a tunneling-ionization-induced modulation of the electron density. The optical signature of electron tunneling can be isolated from concomitant optical responses by using a noncollinear pump-probe setup. Whereas previously demonstrated tools for attosecond metrology of gases, plasmas, and surfaces rely on direct detection of charged particles, detection of the background-free time-resolved optical signal, which uniquely originates from electron tunneling, offers an interesting alternative that is especially suited for systems in which free electrons cannot be directly measured.

A hollow beam from a holey fiber.

A high-quality spectrally isolated hollow beam is produced through a nonlinear-optical transformation of Ti: sapphire laser pulses in a higher order mode of a photonic-crystal fiber (PCF). Instead of a doughnut shape, typical of hollow beams produced by other methods, the far-field image of the hollow-beam PCF output features perfect sixth-order rotation symmetry, dictated by the symmetry of the PCF structure. The frequency of the PCF-generated hollow beam can be tuned by varying the input beam parameters, making a few-mode PCF a convenient and flexible tool for the guiding and trapping of atoms and creation of all-fiber optical tweezers.

Broadband dynamic phase matching of high-order harmonic generation by a high-peak-power soliton pump field in a gas-filled hollow photonic-crystal fiber.

Hollow-core photonic-crystal fibers are shown to enable dynamically phase-matched high-order harmonic generation by a gigawatt soliton pump field. With a careful design of the waveguide structure and an appropriate choice of input-pulse and gas parameters, a remarkably broadband phase matching can be achieved for a soliton pump field and a large group of optical harmonics in the soft-x-ray-extreme-ultraviolet spectral range.

Time-resolved coherent anti-Stokes Raman scattering with a femtosecond soliton output of a photonic-crystal fiber.

We demonstrate time-resolved coherent anti-Stokes Raman scattering (CARS) by using a frequency-tunable femtosecond soliton output of a silica photonic-crystal fiber (PCF) as a Stokes field. This approach allows quantum beats originating from two close Raman modes to be resolved in the time-domain CARS response. The nonresonant CARS background is efficiently suppressed by introducing a delay time between the probe pulse and the pump-Stokes pulse dyad, suggesting a convenient fiber-optic format for the Stokes source in time-resolved CARS and allowing sensitivity improvement in PCF-based CARS spectroscopes and microscopes.