Inhibition and enhancement of the spontaneous emission in spherical cavities surrounded by zero-index-materials.

There exist resonance degeneracy and nesting in the spherical dielectric cavity embedded in an infinite zero-index-material (ZIM). However, its spontaneous emission (SE) has been scarcely studied. Here, we investigate the inhibition and enhancement of SE in spherical dielectric cavities surrounded by ZIMs at the nanoscale. In the cavities embedded in ε-near-zero materials, by adjusting the polarization of the emitter, the SE of the emitter can be controlled from inhibition to enhancement, ranging from 10-2 to dozens. For the cavities embedded in µ-near-zero or ε-µ-near-zero materials, the enhancement of SE is also achieved in a large range of cavities. These findings provide more application possibilities in single-photon sources, deformable optical devices with ZIMs, etc.

Absorption Reduction of Large Purcell Enhancement Enabled by Topological State-Led Mode Coupling.

We propose the mechanism of edge state-led mode coupling under topological protection; i.e., localized surface plasmons almost do not have any influence on the edge state, while the edge state greatly changes the local field distribution of surface plasmons. Based on this mechanism, in the well-designed topological photonic structure containing a resonant plasmon nanoantenna, an obvious absorption reduction in the spontaneous emission spectra appears due to the near-field deformation around the antenna induced by the edge state. Because a plasmon antenna with ultrasmall mode volume provides large Purcell enhancement and simultaneously the photonic crystal guides almost all scattering light into its edge state, the rate of nonscattering single photons reaches more than 10^{4}γ_{0}. This topological state-led mode coupling mechanism and induced absorption reduction, which are based on topological protection, will have a profound effect on the study of composite topological photonic structures and related micro- and nanoscale cavity quantum electrodynamics. Also, nonscattering large Purcell enhancement will provide practical use for on-chip quantum light sources, such as single-photon sources and nanolasers.

Large Purcell enhancement with nanoscale non-reciprocal photon transmission in chiral gap-plasmon-emitter systems.

Chiral photon-emitter coupling has been extensively explored in its non-reciprocal property, which results from spin-locked photon transmission. It manifests the potential in on-chip non-reciprocal devices, such as optical isolators and photon routing in quantum networks. However, the enhancement of chiral coupling, which has been seldom studied, remains wanting. Here, we numerically propose a gap-plasmon-emitter system demonstrating large Purcell enhancement with effective nanoscale non-reciprocal photon transmission. Owing to the strong field enhancement and high transverse spin momentum (TSM) in gap plasmons, the Purcell factor reaches 104. Simultaneously, the transmission in the nanowire is directional, in which 91% propagates in a single direction. The transmission confined around the nanowire also obtains a ∼700-fold enhancement compared with the vacuum decay rate of the emitter. Furthermore, the circularly polarized emitter couples preferentially to the opposite transmission direction in the two eigenmodes. This phenomenon is attributed to the special TSM profile of the two eigenmodes, that is, the transmission direction is locked to the opposite TSM in the two eigenmodes. Our proposed system offers an efficient way for photon routing in optical circuits and quantum networks and also extends methods for manipulating non-reciprocal devices.

Accumulation and directionality of large spontaneous emission enabled by epsilon-near-zero film.

We demonstrate the spectral accumulation of large spontaneous emission (SE) for nanocavities with different sizes in the coupled Ag nanorod and epsilon-near-zero (ENZ) film system. This effect originates from the slowing down of the spectral shift of resonant nanocavities at the wavelength where the permittivity of the substrate vanishes, i.e., the resonance "pinning" near the ENZ frequency. In addition, most far field radiation of the emitter is concentrated in the forward field with small solid angle due to the impedance mismatch between the ENZ film and the free space. This kind of size-relaxed nanocavity for directional SE has potential applications in the bright single photon sources, plasmon-based nanolasers, and on-chip nanodevices.