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1.
J Am Chem Soc ; 146(31): 21546-21554, 2024 Aug 07.
Artigo em Inglês | MEDLINE | ID: mdl-39048922

RESUMO

Two-dimensional (2D) magnets have attracted significant attention in recent years due to their importance in the research on both fundamental physics and spintronic applications. Here, we report the discovery of a new ternary compound FePd2Te2. It features a layered quasi-2D crystal structure with 1D Fe zigzag chains extending along the b-axis in the cleavage plane. Single crystals of FePd2Te2 with centimeter size could be grown. Density functional theory calculations, mechanical exfoliation, and atomic force microscopy on these crystals reveal that they are 2D materials that can be thinned down to ∼5 nm. Magnetic characterization shows that FePd2Te2 is an easy-plane ferromagnet with TC ∼ 183 K and strong in-plane uniaxial magnetic anisotropy. Magnetoresistance and the anomalous Hall effect demonstrate that ferromagnetism could be maintained in FePd2Te2 flakes with large coercivity. A crystal twinning effect is observed by scanning tunneling microscopy which makes the Fe chains right angle bent in the cleavage plane and creates an intriguing spin texture. Besides, a large electronic specific heat coefficient of up to γ ∼ 32.4 mJ mol-1 K-2 suggests FePd2Te2 is a strongly correlated metal. Our results show that FePd2Te2 is a correlated anisotropic 2D magnet that may attract multidisciplinary research interests.

2.
Opt Express ; 30(12): 22135-22142, 2022 Jun 06.
Artigo em Inglês | MEDLINE | ID: mdl-36224919

RESUMO

Lithium niobate on insulator (LNOI) is a new photonic integrated platform that provides high optical confinement and retains the inherent excellent properties of lithium niobate (LN). Tunable filters are one of the indispensable devices for integrated optics. Here we design and fabricate a thermo-optic (TO) tunable optical filter using two cascaded racetrack microring resonators (MRRs) based on LNOI. The filter shows a narrow and flat top passband with intra band ripple less than 0.3 dB, 3 dB bandwidth of 4.8 GHz and out-of-band rejection of about 35 dB. The insertion loss of the filter is about -14 dB, including grating coupling loss about -6.5 dB and on-chip loss less than -1 dB. The heating power for center wavelength shift of the filter is about 89.4 mW per free spectral range (FSR). Relevant applications of such filters include optical information processing and microwave photonics.

3.
Opt Express ; 30(16): 29611-29620, 2022 Aug 01.
Artigo em Inglês | MEDLINE | ID: mdl-36299132

RESUMO

High-speed analog-to-digital conversion (ADC) is experimentally demonstrated by employing a time and wavelength interleaved ultra-short optical pulse train to achieve photonic sampling and using wavelength division demultiplexing to realize speed matching between the fast optical front-end and the slow electronic back-end. The sampling optical pulse train is generated from a cavity-less ultra-short optical pulse source involving a packaged device that monolithically integrates an intensity modulator and a phase modulator into a chip based on lithium niobate on insulator (LNOI). In the experiment, the fiber-to-fiber insertion loss of the packaged modulation device is measured to be 6.9 dB. In addition, the half-wave voltages of the Mach-Zehnder modulator and the phase modulator in the LNOI-based modulation device are measured to be 3.6 V and 3.4 V at 5 GHz, respectively. These parameters and the device size are superior to those based on cascaded commercial devices. Through using the packaged modulation device, two ultra-short optical pulse trains centered at 1541.40 nm and 1555.64 nm are generated with time jitters of 19.2 fs and 18.9 fs in the integral offset frequency range of 1 kHz to 10 MHz, respectively, and are perfectly time interleaved into a single pulse train with a repetition rate of 10 GHz and a time jitter of 19.8 fs. Based on the time and wavelength interleaved ultra-short optical pulse train, direct digitization of microwave signals within the frequency range of 1 GHz to 40 GHz is demonstrated by using a two-channel wavelength demultiplexing photonic ADC architecture, where the effective number of bits are 5.85 bits and 3.75 bits for the input signal at 1.1 GHz and 36.3 GHz, respectively.

4.
Sci Adv ; 6(28): eaba8595, 2020 Jul.
Artigo em Inglês | MEDLINE | ID: mdl-32695878

RESUMO

The hologram is an ideal method for displaying three-dimensional images visible to the naked eye. Metasurfaces consisting of subwavelength structures show great potential in light field manipulation, which is useful for overcoming the drawbacks of common computer-generated holography. However, there are long-existing challenges to achieving dynamic meta-holography in the visible range, such as low frame rate and low frame number. In this work, we demonstrate a design of meta-holography that can achieve 228 different holographic frames and an extremely high frame rate (9523 frames per second) in the visible range. The design is based on a space channel metasurface and a high-speed dynamic structured laser beam modulation module. The space channel consists of silicon nitride nanopillars with a high modulation efficiency. This method can satisfy the needs of a holographic display and be useful in other applications, such as laser fabrication, optical storage, optics communications, and information processing.

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