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1.
Nat Commun ; 9(1): 517, 2018 02 06.
Artigo em Inglês | MEDLINE | ID: mdl-29410418

RESUMO

SmB6 is predicted to be the first member of the intersection of topological insulators and Kondo insulators, strongly correlated materials in which the Fermi level lies in the gap of a many-body resonance that forms by hybridization between localized and itinerant states. While robust, surface-only conductivity at low temperature and the observation of surface states at the expected high symmetry points appear to confirm this prediction, we find both surface states at the (100) surface to be topologically trivial. We find the [Formula: see text] state to appear Rashba split and explain the prominent [Formula: see text] state by a surface shift of the many-body resonance. We propose that the latter mechanism, which applies to several crystal terminations, can explain the unusual surface conductivity. While additional, as yet unobserved topological surface states cannot be excluded, our results show that a firm connection between the two material classes is still outstanding.

2.
Nat Commun ; 7: 10876, 2016 Mar 15.
Artigo em Inglês | MEDLINE | ID: mdl-26976632

RESUMO

Some heavy fermion materials show so-called hidden-order phases which are invisible to many characterization techniques and whose microscopic origin remained controversial for decades. Among such hidden-order compounds, CeB6 is of model character due to its simple electronic configuration and crystal structure. Apart from more conventional antiferromagnetism, it shows an elusive phase at low temperatures, which is commonly associated with multipolar order. Here we show that this phase roots in a Fermi surface instability. This conclusion is based on a full 3D tomographic sampling of the electronic structure by angle-resolved photoemission and comparison with inelastic neutron scattering data. The hidden order is mediated by itinerant electrons. Our measurements will serve as a paradigm for the investigation of hidden-order phases in f-electron systems, but also generally for situations where the itinerant electrons drive orbital or spin order.


Assuntos
Cério/química , Elétrons , Hidróxidos/química , Nêutrons , Cristalização , Magnetismo , Modelos Químicos , Temperatura , Tomografia Computadorizada por Raios X
3.
Nat Commun ; 3: 830, 2012 May 15.
Artigo em Inglês | MEDLINE | ID: mdl-22588292

RESUMO

Resonant magnetic excitations are recognised as hallmarks of unconventional superconductivity in copper oxides, iron pnictides and heavy-fermion compounds. Model calculations have related these modes to the microscopic properties of the pair wave function, but the mechanisms of their formation are still debated. Here we report the discovery of a similar resonant mode in the non-superconducting antiferromagnetic heavy-fermion metal CeB(6). Unlike conventional magnons, the mode is non-dispersive and is sharply peaked around a wave vector separate from those characterising the antiferromagnetic order. It is likely associated with a co-existing order parameter of the unusual antiferro-quadrupolar phase of CeB(6), which has long remained hidden to neutron-scattering probes. The mode energy increases continuously below the onset temperature for antiferromagnetism, in parallel to the opening of a nearly isotropic spin gap throughout the Brillouin zone. These attributes are similar to those of the resonant modes in unconventional superconductors. This unexpected commonality between the two disparate ground states indicates the dominance of itinerant spin dynamics in the ordered low-temperature phases of CeB(6) and throws new light on the interplay between antiferromagnetism, superconductivity and 'hidden' order parameters in correlated-electron materials.

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