Broadband frequency comb generation through cascaded quadratic nonlinearity in thin-film lithium niobate microresonators.

Broadband frequency comb generation through cascaded quadratic nonlinearity remains experimentally untapped in free-space cavities with bulk χ(2) materials mainly due to the high threshold power and restricted ability of dispersion engineering. Thin-film lithium niobate (LN) is a good platform for nonlinear optics due to the tight mode confinement in a nano-dimensional waveguide, the ease of dispersion engineering, large quadratic nonlinearities, and flexible phase matching via periodic poling. Here we demonstrate broadband frequency comb generation through dispersion engineering in a thin-film LN microresonator. Bandwidths of 150 nm (80 nm) and 25 nm (12 nm) for center wavelengths at 1560 and 780 nm are achieved, respectively, in a cavity-enhanced second-harmonic generation (doubly resonant optical parametric oscillator). Our demonstration paves the way for pure quadratic soliton generation, which is a great complement to dissipative Kerr soliton frequency combs for extended interesting nonlinear applications.

Non-invasive single photon imaging through strongly scattering media.

Non-invasive optical imaging through opaque and multi-scattering media remains highly desirable across many application domains. The random scattering and diffusion of light in such media inflict exponential decay and aberration, prohibiting diffraction-limited imaging. By non-interferometric few picoseconds optical gating of backscattered photons, we demonstrate single photon sensitive non-invasive 3D imaging of targets occluded by strongly scattering media with optical thicknesses reaching 9.5ls (19ls round trip). It achieves diffraction-limited imaging of a target placed 130 cm away through the opaque media, with millimeter lateral and depth resolution while requiring only one photon detection out of 50,000 probe pulses. Our single photon sensitive imaging technique does not require wavefront shaping nor computationally-intensive image reconstruction algorithms, promising practical solutions for diffraction-limited imaging through highly opaque and diffusive media with low illumination power.

Single-photon vibrometry.

We propose and demonstrate a single-photon sensitive technique for optical vibrometry. It uses high speed photon counting to sample the modulated backscattering from a vibrating target. Designed for remote vibration sensing with ultralow photon flux, we show that this technique can detect small displacements down to 110 nm and resolve vibration frequencies from DC up to several kilohertz, with ≤0.01 detected photons per pulse. This single-photon sensitive optical vibrometry may find important applications in acousto-optic sensing and imaging, especially in photon-starved environments.

Single-point material recognition by quantum parametric mode sorting and photon counting.

We explore an active illumination approach to remote material recognition, based on quantum parametric mode sorting and single-photon detection. By measuring a photon's time of flight at picosecond resolution, 97.8% recognition is demonstrated by illuminating only a single point on the materials. Thanks to the exceptional detection sensitivity and noise rejection, a high recognition accuracy of 96.1% is achieved even when the materials are occluded by a lossy and multiscattering obscurant.

Ultrabright Quantum Photon Sources on Chip.

Quantum photon sources of high rate, brightness, and purity are increasingly desirable as quantum information systems are quickly scaled up and applied to many fields. Using a periodically poled lithium niobate microresonator on chip, we demonstrate photon-pair generation at high rates of 8.5 and 36.3 MHz using only 3.4 and 13.4 µW pump power, respectively, marking orders of magnitude improvement over the state of the art, across all material platforms. These results constitute the first direct measurement of the device's giant single photon nonlinearity. The measured coincidence to accidental ratio is well above 100 at those high rates and reaches 14682±4427 at a lower pump power. The same chip enables heralded single-photon generation at tens of megahertz rates, each with low autocorrelation g_{H}^{(2)}(0)=0.008 and 0.097 for the microwatt pumps, which marks a new milestone. Such distinct performance, facilitated by the chip device's noiseless and giant optical nonlinearity, will contribute to the forthcoming pervasive adoption of quantum optical information technologies.

High-extinction electro-optic modulation on lithium niobate thin film.

Integrated nanophotonics using lithium-niobate-on-insulator promises much-awaited solutions for scalable photonics techniques. One of its core functions is electro-optic modulation, which currently suffers limited extinction (<30 dB) due to inevitable fabrication errors. We exploit a cascaded Mach-Zehnder interferometry design to offset those errors, demonstrating up to 53 dB modulation extinction for a wide range of wavelengths between 1500 nm and 1600 nm. Together, its favorable features of chip integration, high extinction, good stability, and being broadband may prove valuable in a plethora of flourishing photonics applications.

Mode selective up-conversion detection for LIDAR applications.

We study mode selective up-conversion detection as a viable approach to improving signal-to-noise and ranging resolution in LIDAR applications. It involves pumping a nonlinear waveguide at the edge of phase matching with picosecond pulses, so that only the backscattered signal photons in a single or few desirable time-frequency modes are efficiently up-converted while the broadband background noise in all other modes is rejected. We demonstrate a 41-dB increase in the signal-to-noise ratio for single-photon counting compared to that of direct detection using a commercial InGaAs single-photon detector, while achieving sub-millimeter ranging resolution with few detected photons. The proposed technique implies new LIDAR capabilities for ranging and imaging.

Programmable quantum random number generator without postprocessing.

We demonstrate a viable source of unbiased quantum random numbers whose statistical properties can be arbitrarily programmed without the need for any postprocessing such as randomness distillation or distribution transformation. It is based on measuring the arrival time of single photons in shaped temporal modes that are tailored with an electro-optical modulator. We show that quantum random numbers can be created directly in customized probability distributions and pass all randomness tests of the NIST and Dieharder test suites without any randomness extraction. The min-entropies of such generated random numbers are measured close to the theoretical limits, indicating their near-ideal statistics and ultrahigh purity. Easy to implement and arbitrarily programmable, this technique can find versatile uses in a multitude of data analysis areas.

Ultra-wideband and high-gain parametric amplification in telecom wavelengths with an optimally mode-matched PPLN waveguide.

We report a wideband optical parametric amplification (OPA) over 14 THz covering telecom S, C, and L bands with observed maximum parametric gain of 38.3 dB. The OPA is realized through cascaded second-harmonic generation and difference-frequency generation (cSHG-DFG) in a 2 cm periodically poled LiNbO3 (PPLN) waveguide. With tailored cross section geometry, the waveguide is optimally mode matched for efficient cascaded nonlinear wave mixing. We also identify and study the effect of competing nonlinear processes in this cSHG-DFG configuration.

Highly sensitive multi-core flat fiber surface plasmon resonance refractive index sensor.

A simple multi-core flat fiber (MCFF) based surface plasmon resonance (SPR) sensor operating in telecommunication wavelengths is proposed for refractive index sensing. Chemically stable gold (Au) and titanium dioxide (TiO(2)) layers are used outside the fiber structure to realize a simple detection mechanism. The modeled sensor shows average wavelength interrogation sensitivity of 9,600 nm/RIU (Refractive Index Unit) and maximum sensitivity of 23,000 nm/RIU in the sensing range of 1.46-1.485 and 1.47-1.475, respectively. Moreover, the refractive index resolution of 4.35 × 10(-6) is demonstrated. Additionally, proposed sensor had shown the maximum amplitude interrogation sensitivity of 820 RIU(-1), with the sensor resolution of 1.22 × 10(-5) RIU. To the best of our knowledge, the proposed sensor achieved the highest wavelength interrogation sensitivity among the reported fiber based SPR sensors. Finally we anticipate that, this novel and highly sensitive MCFF SPR sensor will find the potential applications in real time remote sensing and monitoring, ultimately enabling inexpensive and accurate chemical and biochemical analytes detection.

Quantum correlation of fiber-based telecom-band photon pairs through standard loss and random media.

We study quantum correlation and interference of fiber-based telecom-band photon pairs with one photon of the pair experiencing multiple scattering in a random medium. We measure joint probability of two-photon detection for signal photon in a normal channel and idler photon in a channel, which is subjected to two independent conditions: standard loss (neutral density filter) and random media. We observe that both conditions degrade the correlation of signal and idler photons, and depolarization of the idler photon in random medium can enhance two-photon interference at certain relative polarization angles. Our theoretical calculation on two-photon polarization correlation and interference as a function of mean free path is in agreement with our experiment data. We conclude that quantum correlation of a polarization-entangled photon pair is better preserved than a polarization-correlated photon pair as one photon of the pair scatters through a random medium.

Generation of high-purity entangled photon pair in a short highly nonlinear fiber.

We generate photon pairs at telecom wavelength through a spontaneous four-wave mixing process in a short 10 m of highly nonlinear fiber. We use a counterpropagating scheme to generate a correlated and entangled photon pair. We observe coincidence to accidental-coincidence ratio of 29±3 at room temperature (300 K) and as high as 130±5 when the fiber is cooled to liquid-nitrogen temperature (77 K). Two-photon interference with visibility >98% (>92%) and the violation of Bell's inequality by >12 (≈5) standard deviation are observed at 77 K (300 K), respectively, without subtracting accidental-coincidence count. We obtain a photon-pair production rate about factor 3(2) higher than a 300 m dispersion-shifted fiber at 300 K (77 K).

Optical phase-space-time-frequency tomography.

We present a new approach for constructing optical phase-space-time-frequency tomography (OPSTFT) of an optical wave field. This tomography can be measured by using a novel four-window optical imaging system based on two local oscillator fields balanced heterodyne detection. The OPSTFT is a Wigner distribution function of two independent Fourier Transform pairs, i.e., phase-space and time-frequency. From its theoretical and experimental aspects, it can provide information of position, momentum, time and frequency of a spatial light field with precision beyond the uncertainty principle. Besides the distributions of x-p and t-ω, the OPSTFT can provide four other distributions such as x-t, p-t, x-ω and p-ω. We simulate the OPSTFT for a light field obscured by a wire and a single-line absorption filter. We believe that the four-window system can provide spatial and temporal properties of a wave field for quantum image processing and biophotonics.

Noise-tolerant single photon sensitive three-dimensional imager.

Active imagers capable of reconstructing 3-dimensional (3D) scenes in the presence of strong background noise are highly desirable for many sensing and imaging applications. A key to this capability is the time-resolving photon detection that distinguishes true signal photons from the noise. To this end, quantum parametric mode sorting (QPMS) can achieve signal to noise exceeding by far what is possible with typical linear optics filters, with outstanding performance in isolating temporally and spectrally overlapping noise. Here, we report a QPMS-based 3D imager with exceptional detection sensitivity and noise tolerance. With only 0.0006 detected signal photons per pulse, we reliably reconstruct the 3D profile of an obscured scene, despite 34-fold spectral-temporally overlapping noise photons, within the 6 ps detection window (amounting to 113,000 times noise per 20 ns detection period). Our results highlight a viable approach to suppress background noise and measurement errors of single photon imager operation in high-noise environments.

Quantum Parametric Mode Sorting: Beating the Time-Frequency Filtering.

Selective detection of signal over noise is essential to measurement and signal processing. Time-frequency filtering has been the standard approach for the optimal detection of non-stationary signals. However, there is a fundamental tradeoff between the signal detection efficiency and the amount of undesirable noise detected simultaneously, which restricts its uses under weak signal yet strong noise conditions. Here, we demonstrate quantum parametric mode sorting based on nonlinear optics at the edge of phase matching to improve the tradeoff. By tailoring the nonlinear process in a commercial lithium-niobate waveguide through optical arbitrary waveform generation, we demonstrate highly selective detection of picosecond signals overlapping temporally and spectrally but in orthogonal time-frequency modes as well as against broadband noise, with performance well exceeding the theoretical limit of the optimized time-frequency filtering. We also verify that our device does not introduce any significant quantum noise to the detected signal and demonstrate faithful detection of pico-second single photons. Together, these results point to unexplored opportunities in measurement and signal processing under challenging conditions, such as photon-starving quantum applications.

Observation of Quantum Zeno Blockade on Chip.

Overlapping in an optical medium with nonlinear susceptibilities, lightwaves can interact, changing each other's phase, wavelength, waveform shape, or other properties. Such nonlinear optical phenomena, discovered over a half-century ago, have led to a breadth of important applications. Applied to quantum-mechanical signals, however, these phenomena face fundamental challenges that arise from the multimodal nature of the interaction between the electromagnetic fields, such as phase noises and spontaneous Raman scattering. The quantum Zeno blockade allows strong interaction between lightwaves without physical overlap between them, thus offering a viable solution for the aforementioned challenges, as indicated in recent bulk-optics experiments. Here, we report on the observation of quantum Zeno blockade on chip, where a lightwave is modulated by another in a distinct "interaction-free" manner. For quantum applications, we also verify its operations on single-photon signals. Our results promise a scalable platform for overcoming several longstanding challenges in applied nonlinear and quantum optics, enabling manipulation and interaction of quantum signals without decoherence.

Direct Generation and Detection of Quantum Correlated Photons with 3.2 um Wavelength Spacing.

Quantum correlated, highly non-degenerate photons can be used to synthesize disparate quantum nodes and link quantum processing over incompatible wavelengths, thereby constructing heterogeneous quantum systems for otherwise unattainable superior performance. Existing techniques for correlated photons have been concentrated in the visible and near-IR domains, with the photon pairs residing within one micron. Here, we demonstrate direct generation and detection of high-purity photon pairs at room temperature with 3.2 um wavelength spacing, one at 780 nm to match the rubidium D2 line, and the other at 3950 nm that falls in a transparent, low-scattering optical window for free space applications. The pairs are created via spontaneous parametric downconversion in a lithium niobate waveguide with specially designed geometry and periodic poling. The 780 nm photons are measured with a silicon avalanche photodiode, and the 3950 nm photons are measured with an upconversion photon detector using a similar waveguide, which attains 34% internal conversion efficiency. Quantum correlation measurement yields a high coincidence-to-accidental ratio of 54, which indicates the strong correlation with the extremely non-degenerate photon pairs. Our system bridges existing quantum technology to the challenging mid-IR regime, where unprecedented applications are expected in quantum metrology and sensing, quantum communications, medical diagnostics, and so on.