Quantum Plasmonic Sensors.

The extraordinary sensitivity of plasmonic sensors is well-known in the optics and photonics community. These sensors exploit simultaneously the enhancement and the localization of electromagnetic fields close to the interface between a metal and a dielectric. This enables, for example, the design of integrated biochemical sensors at scales far below the diffraction limit. Despite their practical realization and successful commercialization, the sensitivity and associated precision of plasmonic sensors are starting to reach their fundamental classical limit given by quantum fluctuations of light-known as the shot-noise limit. To improve the sensing performance of these sensors beyond the classical limit, quantum resources are increasingly being employed. This area of research has become known as "quantum plasmonic sensing", and it has experienced substantial activity in recent years for applications in chemical and biological sensing. This review aims to cover both plasmonic and quantum techniques for sensing, and it shows how they have been merged to enhance the performance of plasmonic sensors beyond traditional methods. We discuss the general framework developed for quantum plasmonic sensing in recent years, covering the basic theory behind the advancements made, and describe the important works that made these advancements. We also describe several key works in detail, highlighting their motivation, the working principles behind them, and their future impact. The intention of the review is to set a foundation for a burgeoning field of research that is currently being explored out of intellectual curiosity and for a wide range of practical applications in biochemistry, medicine, and pharmaceutical research.

Quantum plasmonic sensing using single photons.

Reducing the noise below the shot-noise limit in sensing devices is one of the key promises of quantum technologies. Here, we study quantum plasmonic sensing based on an attenuated total reflection configuration with single photons as input. Our sensor is the Kretschmann configuration with a gold film, and a blood protein in an aqueous solution with different concentrations serves as an analyte. The estimation of the refractive index is performed using heralded single photons. We also determine the estimation error from a statistical analysis over a number of repetitions of identical and independent experiments. We show that the errors of our plasmonic sensor with single photons are below the shot-noise limit even in the presence of various experimental imperfections. Our results demonstrate a practical application of quantum plasmonic sensing is possible given certain improvements are made to the setup investigated, and pave the way for a future generation of quantum plasmonic applications based on similar techniques.

Experimental characterization of a non-local convertor for quantum photonic networks.

We experimentally characterize a quantum photonic gate that is capable of converting multiqubit entangled states while acting only on two qubits. It is an important tool in large quantum networks, where it can be used for re-wiring of multipartite entangled states or for generating various entangled states required for specific tasks. The gate can be also used to generate quantum information processing resources, such as entanglement and discord. In our experimental demonstration, we characterized the conversion of a linear four-qubit cluster state into different entangled states, including GHZ and Dicke states. The high quality of the experimental results show that the gate has the potential of being a flexible component in distributed quantum photonic networks.

Quantum entanglement distillation with metamaterials.

We propose a scheme for the distillation of partially entangled two-photon Bell and three-photon W states using metamaterials. The distillation of partially entangled Bell states is achieved by using two metamaterials with polarization dependence, one of which is rotated by π/2 around the direction of propagation of the photons. On the other hand, the distillation of three-photon W states is achieved by using one polarization dependent metamaterial and two polarization independent metamaterials. Upon transmission of the photons of the partially entangled states through the metamaterials the entanglement of the states increases and they become distilled. This work opens up new directions in quantum optical state engineering by showing how metamaterials can be used to carry out a quantum information processing task.

Quantum statistics of surface plasmon polaritons in metallic stripe waveguides.

Heralded single surface plasmon polaritons are excited using photons generated via spontaneous parametric down conversion. The mean excitation rates, intensity correlations, and Fock state populations are studied. The observed dependence of the second-order coherence in our experiment is consistent with a linear uncorrelated Markovian environment in the quantum regime. Our results provide important information about the effect of loss for assessing the potential of plasmonic waveguides for future nanophotonic circuitry in the quantum regime.

Implementation of single-qubit measurement-based t-designs using IBM processors.

Random unitary matrices sampled from the uniform Haar ensemble have a number of important applications both in cryptography and in the simulation of a variety of fundamental physical systems. Since the Haar ensemble is very expensive to sample, pseudorandom ensembles in the form of t-designs are frequently used as an efficient substitute, and are sufficient for most applications. We investigate t-designs generated using a measurement-based approach on superconducting quantum computers. In particular, we implemented an exact single-qubit 3-design on IBM quantum processors by performing measurements on a 6-qubit graph state. By analysing channel tomography results, we were able to show that the ensemble of unitaries realised was a 1-design, but not a 2-design or a 3-design under the test conditions set, which we show to be a result of depolarising noise during the measurement-based process. We obtained improved results for the 2-design test by implementing an approximate 2-design, in which measurements were performed on a smaller 5-qubit graph state, but the test still did not pass for all states. This suggests that the practical realisation of measurement-based t-designs on superconducting quantum computers will require further work on the reduction of depolarising noise in these devices.

Demonstration of Shor's factoring algorithm for N [Formula: see text] 21 on IBM quantum processors.

We report a proof-of-concept demonstration of a quantum order-finding algorithm for factoring the integer 21. Our demonstration involves the use of a compiled version of the quantum phase estimation routine, and builds upon a previous demonstration. We go beyond this work by using a configuration of approximate Toffoli gates with residual phase shifts, which preserves the functional correctness and allows us to achieve a complete factoring of [Formula: see text]. We implemented the algorithm on IBM quantum processors using only five qubits and successfully verified the presence of entanglement between the control and work register qubits, which is a necessary condition for the algorithm's speedup in general. The techniques we employ may be useful in carrying out Shor's algorithm for larger integers, or other algorithms in systems with a limited number of noisy qubits.

Distillation of photon entanglement using a plasmonic metamaterial.

Plasmonics is a rapidly emerging platform for quantum state engineering with the potential for building ultra-compact and hybrid optoelectronic devices. Recent experiments have shown that despite the presence of decoherence and loss, photon statistics and entanglement can be preserved in single plasmonic systems. This preserving ability should carry over to plasmonic metamaterials, whose properties are the result of many individual plasmonic systems acting collectively, and can be used to engineer optical states of light. Here, we report an experimental demonstration of quantum state filtering, also known as entanglement distillation, using a metamaterial. We show that the metamaterial can be used to distill highly entangled states from less entangled states. As the metamaterial can be integrated with other optical components this work opens up the intriguing possibility of incorporating plasmonic metamaterials in on-chip quantum state engineering tasks.