Pressure tuning of the spin-orbit coupled ground state in Sr2IrO4.
Phys Rev Lett
; 109(2): 027204, 2012 Jul 13.
Article
em En
| MEDLINE
| ID: mdl-23030204
ABSTRACT
X-ray absorption spectroscopy studies of the magnetic-insulating ground state of Sr2IrO4 at ambient pressure show a clear deviation from a strong spin-orbit (SO) limit J(eff)=1/2 state, a result of local exchange interactions and a nonzero tetragonal crystal field mixing SO split J(eff)=1/2, 3/2 states. X-ray magnetic circular dichroism measurements in a diamond anvil cell show a magnetic transition at a pressure of â¼17 GPa, where the "weak" ferromagnetic moment is quenched despite transport measurements showing insulating behavior to at least 40 GPa. The magnetic transition has implications for the origin of the insulating gap and the nature of exchange interactions in this SO coupled system. The expectation value of the angular part of the SO interaction,
Buscar no Google
Base de dados:
MEDLINE
Idioma:
En
Revista:
Phys Rev Lett
Ano de publicação:
2012
Tipo de documento:
Article
País de afiliação:
Estados Unidos