Your browser doesn't support javascript.
loading
High order harmonic generation from SF6: Deconvolution of macroscopic effects.
Wilson, B P; Fulfer, K D; Mondal, S; Ren, X; Tross, J; Poliakoff, E D; Jose, J; Le, Anh-Thu; Lucchese, R R; Trallero-Herrero, C.
Afiliação
  • Wilson BP; Department of Chemistry, Louisiana State University, Baton Rouge, Louisiana 70803, USA.
  • Fulfer KD; Department of Chemistry, Louisiana State University, Baton Rouge, Louisiana 70803, USA.
  • Mondal S; J.R. Macdonald Laboratory, Kansas State University, Manhattan, Kansas 66506, USA.
  • Ren X; J.R. Macdonald Laboratory, Kansas State University, Manhattan, Kansas 66506, USA.
  • Tross J; J.R. Macdonald Laboratory, Kansas State University, Manhattan, Kansas 66506, USA.
  • Poliakoff ED; Department of Chemistry, Louisiana State University, Baton Rouge, Louisiana 70803, USA.
  • Jose J; Department of Chemistry, Texas A&M University, College Station, Texas 77843, USA.
  • Le AT; J.R. Macdonald Laboratory, Kansas State University, Manhattan, Kansas 66506, USA.
  • Lucchese RR; Department of Chemistry, Texas A&M University, College Station, Texas 77843, USA.
  • Trallero-Herrero C; J.R. Macdonald Laboratory, Kansas State University, Manhattan, Kansas 66506, USA.
J Chem Phys ; 145(22): 224305, 2016 Dec 14.
Article em En | MEDLINE | ID: mdl-27984891
ABSTRACT
We measure high order harmonics from the molecule SF6 over a large range of phase matching conditions and observe several features in the harmonics that are largely independent of such macroscopic conditions. The experimental data are then compared to the quantitative rescattering theory for the generation of harmonics from three orbitals. With this comparison, we are able to assign spectroscopic features in the harmonics to contributions from 1t1g (HOMO) and 5t1u (HOMO-1) orbitals.
Buscar no Google
Imprimir
XML
PubMed Links

Base de dados: MEDLINE Idioma: En Revista: J Chem Phys Ano de publicação: 2016 Tipo de documento: Article País de afiliação: Estados Unidos
Buscar no Google
Imprimir
XML
PubMed Links

Base de dados: MEDLINE Idioma: En Revista: J Chem Phys Ano de publicação: 2016 Tipo de documento: Article País de afiliação: Estados Unidos