RESUMO
Cerium 4f electronic spin dynamics in single crystals of the heavy-fermion system CeFePO is studied by means of ac susceptibility, specific heat, and muon-spin relaxation (µSR). Short-range static magnetism occurs below the freezing temperature T(g) ≈ 0.7 K, which prevents the system from accessing a putative ferromagnetic quantum critical point. In the µSR, the sample-averaged muon asymmetry function is dominated by strongly inhomogeneous spin fluctuations below 10 K and exhibits a characteristic time-field scaling relation expected from glassy spin dynamics, strongly evidencing cooperative and critical spin fluctuations. The overall behavior can be ascribed neither to canonical spin glasses nor other disorder-driven mechanisms.
Assuntos
Cério/química , Compostos Férricos/química , Imãs , Modelos Químicos , Teoria Quântica , Óxidos/química , Fósforo/químicaRESUMO
The high-field superconducting state in CeCoIn(5) has been studied by transverse field muon spin rotation measurements with an applied field parallel to the crystallographic c axis close to the upper critical field mu(0)H(c2) = 4.97 T. At magnetic fields mu(0)H > or = 4.8 T the muon Knight shift is enhanced and the superconducting transition changes from second order towards first order as predicted for Pauli-limited superconductors. The field and temperature dependence of the transverse muon spin relaxation rate sigma reveal paramagnetic spin fluctuations in the field regime from 2 T < or = mu(0)H < 4.8 T. In the normal state close to H(c2) correlated spin fluctuations as described by the self-consistent renormalization theory are observed. The results support the formation of a mode-coupled superconducting and antiferromagnetically ordered phase in CeCoIn(5) for H directed parallel to the c axis.