Suppression of parasitic lasing in high energy, high repetition rate Ti:sapphire laser amplifiers.

Transverse parasitic lasing is well known for limiting the signal gain and the pulse energy that can be extracted from Ti:sapphire petawatt amplifiers. We have developed a technique for suppressing these parasitic lasing modes based on perfect refractive index-matching liquid doped with a broad-bandwidth absorber to suppress the transverse lasing while ensuring proper heat removal from the Ti:sapphire crystal. The 800 nm laser output with a bandwidth of 41 nm (FWHM) and peak energy of 22.7 J at a repetition rate of 1 Hz is demonstrated.

Accuracy measurements and improvement for complete characterization of optical pulses from nonlinear processes via multiple spectral-shearing interferometry.

We demonstrate that multiple spectral-shearing interferometry increases the precision and accuracy of measurements of the spectral phase of a complex pulse (time-bandwidth product = 125) arising from self-phase modulation in a gas filled capillary. We verify that the measured interferometric phase is accurate to 0.1 rad across the full bandwidth by checking the consistency between the spectral phases of each individual shear measurement. The accuracy of extracting pulse parameters (group delay dispersion, pulse duration and peak intensity) for single shear measurements were verified to better than 10% by comparison with the multishear reconstruction. High order space-time coupling is quantified across a single transverse dimension, verifying the suitability of such pulses for use in strong field experiments.

Spatiotemporal amplitude and phase retrieval of space-time coupled ultrashort pulses using the Shackled-FROG technique.

We demonstrate the validity of the Shackled-frequency-resolved-optical-gating technique for the complete characterization, both in space and in time, of ultrashort optical pulses that present strong angular dispersion. Combining a simple imaging grating with a Hartmann-Shack sensor and standard frequency-resolved-optical-gating detection at a single spatial position, we are able to retrieve the full spatiotemporal structure of a tilted pulse.

Optical amplification in the near-infrared in gas-filled hollow-core fibers.

We demonstrate efficient optical parametric amplification and generation in a gas-filled hollow-core fiber of near-infrared pulses, peaked at 1.4 microm wavelength, with 5 microJ energy and 45 fs duration at the fiber output. Numerical simulations confirm that the OPA is phase matched through excitation of higher-order fiber modes.

Mid-IR short-pulse OPCPA with micro-Joule energy at 100kHz.

We present a novel mid-IR source based on optical parametric chirped pulse amplification (OPCPA) generating 96 fs pulses (9.0 cycles) at 3.2 mm with an energy of 1.2 microJ, at a repetition rate of 100 kHz. The amplified spectrum supports a minimum Fourier transform limited pulse duration of 45 fs, or 4.2 cycles. Our use of OPCPA allows the direct amplification of few-cycle pulses at this mid-IR wavelength, and is inherently scalable to higher energies. The seed source for the system is based on difference frequency generation (DFG) between two outputs of the same fibre laser: this source is expected to be intrinsically CEP stable.