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1.
Phys Rev Lett ; 133(13): 136601, 2024 Sep 27.
Artigo em Inglês | MEDLINE | ID: mdl-39392969

RESUMO

Nonreciprocity in acoustics is of paramount importance in many practical applications and has been experimentally realized using nonlinear media, moving fluids, or time modulation, which regrettably suffer from large volumes and high-power consumption, difficulty in integration, and inevitable vibrations or phase noise. In modern Hamiltonian theory, the violation of system's reciprocity can be achieved via asymmetric Peierls phases, which typically involves with non-Hermiticity or time-reversal symmetry breaking. Here, we propose a framework for designing nonreciprocal acoustic devices based on the asymmetric Peierls phases that can be fully controlled via active acoustic components. The fully controlled Peierls phases enable various high-performance acoustic devices, including non-Hermitian extensions of isolators, gyrators, and circulators, which are otherwise impossible in previous approaches that are bound by Hermiticity or passivity. We reveal that the transmission phases in isolators are equivalent to the Peierls phase plus a constant. The nonreciprocal phase delay in gyrators and the unirotational transmission behavior in circulators result from the gauge-invariant Aharonov-Bohm phases determined by Peierls phases. Our work not only uncovers multiple intriguing physics related to Peierls phases but also provides a general approach to compact, integratable, nonreciprocal acoustic devices.

2.
Pharmaceuticals (Basel) ; 17(10)2024 Oct 16.
Artigo em Inglês | MEDLINE | ID: mdl-39459013

RESUMO

BACKGROUND: QT prolongation is a potential serious adverse drug reaction, and assessing the risk of QT-prolonging drugs is routinely included in psychotropic medication reviews. However, the actual clinical benefits of such assessments are unknown. We investigate whether QT prolongation (QTc value > 480 ms) manifests in psychiatric inpatients at risk of QT prolongation as identified by assessing drug regimens. Secondly, we test the predictive value of well-known risk factors for QT prolongation. RESULTS: The median patient age was 49 years (IQR 34-64) for patients treated with a median of nine drugs (IQR 6-12) and a median QT-prolonging drug sum of three daily defined dosages (IQR 1.88-4.76). We extracted 290 ECGs for patients where pharmacist-led-medication reviews (PMRs) identified an increased risk of QT prolongation and 190 ECGs for patients with no such risk, identifying 33 cases of verified QT prolongation equally distributed between groups. Unadjusted regression analysis revealed that advanced age (OR 3.27 CI 95% 1.60-6.84) and cardiovascular comorbidity (OR 3.53 CI 95% 1.71-7.29) were associated with manifest QT prolongation, while the QT-prolonging drug load was not. METHODS: We reviewed electronic health records (EHRs) of 799 psychiatric inpatients exposed to PMRs made from 1 September 2016 to 31 December 2018 in Region Zealand Denmark. CONCLUSIONS: Patients at risk of QT prolongation as identified by drug reviews rarely manifests with actual QT prolongation. Non-pharmacological risk factors seem to be better predictors for identifying patients with QT prolongation.

3.
Sci Bull (Beijing) ; 69(14): 2149-2150, 2024 Jul 30.
Artigo em Inglês | MEDLINE | ID: mdl-38880685
4.
Chem Mater ; 36(6): 2756-2766, 2024 Mar 26.
Artigo em Inglês | MEDLINE | ID: mdl-38558915

RESUMO

Water is one of the most reactive and abundant molecules on Earth, and it is thus crucial to understand its reactivity with various material families. One of the big unknown questions is how water in liquid and vapor forms impact the fast-emerging class of metal-organic frameworks (MOFs). Here, we discover that high-pressure water vapor drastically modifies the structure and hence the dynamic, thermodynamic, and mechanical properties of MOF glasses. In detail, we find that an archetypical MOF (ZIF-62) is extremely sensitive to heat treatments performed at 460 °C and water vapor pressures up to ∼110 bar. Both the melting and glass transition temperatures decrease remarkably (by >100 °C), and simultaneously, hardness and Young's modulus increase by up to 100% under very mild treatment conditions (<20 bar of hydrothermal pressure). Structural analyses suggest water to partially coordinate to Zn in the form of a hydroxide ion by replacing a bridging imidazolate-based linker. The work provides insight into the role of hot-compressed water in influencing the structure and properties of MOF glasses and opens a new route for systematically changing the thermodynamics and kinetics of MOF liquids and thus altering the thermal and mechanical properties of the resulting MOF glasses.

5.
Adv Mater ; 36(25): e2311599, 2024 Jun.
Artigo em Inglês | MEDLINE | ID: mdl-38374796

RESUMO

Vertically stacked multiple atomically thin layers have recently widened the landscape of rich optical structures thanks to these quantum metamaterials or van der Waals (vdW) materials, featuring hyperbolic polaritons with unprecedented avenues for light. Despite their far-reaching implications, most of their properties rest entirely on a trivial band topological origin. Here, a 2D approach is adopted toward a micromechanical vdW analogue that, as a result of engineered chiral and mirror symmetries, provides topologically resilient hyperbolic radiation of mechanical vibrations in the ultrasonic regime. By applying laser vibrometry of the micrometer-sized metasurface, we are able to exhibit the exotic fingerprints of robust hyperbolic radiation spanning several frequencies, which beyond their physical relevance, may enable ultrasonic technologies.

6.
Nat Commun ; 14(1): 7633, 2023 Nov 22.
Artigo em Inglês | MEDLINE | ID: mdl-37993444

RESUMO

Self-imaging phenomena for nonperiodic waves along a parabolic trajectory encompass both the Talbot effect and the accelerating Airy beams. Beyond the ability to guide waves along a bent trajectory, the self-imaging component offers invaluable advantages to lensless imaging comprising periodic repetition of planar field distributions. In order to circumvent thermoviscous and diffraction effects, we structure subwavelength resonators in an acoustically impenetrable surface supporting spoof surface acoustic waves (SSAWs) to provide highly confined Airy-Talbot effect, extending Talbot distances along the propagation path and compressing subwavelength lobes in the perpendicular direction. From a linear array of loudspeakers, we judiciously control the amplitude and phase of the SSAWs above the structured surface and quantitatively evaluate the self-healing performance of the Airy-Talbot effect by demonstrating how the distinctive scattering patterns remain largely unaffected against superwavelength obstacles. Furthermore, we introduce a new mechanism utilizing subwavelength Airy beam as a coding/decoding degree of freedom for acoustic communication with high information density comprising robust transport of encoded signals.

7.
Phys Rev Lett ; 131(6): 066601, 2023 Aug 11.
Artigo em Inglês | MEDLINE | ID: mdl-37625050

RESUMO

The Su-Schrieffer-Heeger (SSH) model is an important cornerstone in modern condensed-matter topology, yet it is the simplest one-dimensional (1D) tight binding approach to dwell into the characteristics of spinless electrons in chains of staggered bonds. Moreover, the chiral symmetry assures that its surface-confining states pin to zero energy, i.e., they reside midgap in the energy dispersion. Symmetry is also an attribute related to artificial media that are subject to parity P and time-reversal T operations. This non-Hermitian family has been thoroughly nourished in a wave-based context, where anti-PT (APT) symmetric systems are the youngest belonging members, permitting refractionless optics, inverse PT-symmetry breaking transition, and asymmetric mode switching. Here, we report the first extension of APT symmetry in an acoustic setting by endowing a SSH lattice with gain and loss components. We show that the in-gap topological defect state hinges on the non-Hermitian phase, in that the broken symmetry suppresses it, yet when PT or APT symmetry is intact, it is observed with either damped or evanescent decay, respectively. Our experiments showcase how the non-Hermitian SSH lattice serves as a utile platform to investigate topological properties across various PT symmetric phases using sound.

9.
Nature ; 618(7966): 687-697, 2023 Jun.
Artigo em Inglês | MEDLINE | ID: mdl-37344649

RESUMO

Light and sound are the most ubiquitous forms of waves, associated with a variety of phenomena and physical effects such as rainbows and echoes. Light and sound, both categorized as classical waves, have lately been brought into unexpected connections with exotic topological phases of matter. We are currently witnessing the onset of a second wave of active research into this topic. The past decade has been marked by fundamental advances comprising two-dimensional quantum Hall insulators and quantum spin and valley Hall insulators, whose topological properties are characterized using linear band topology. Here, going beyond these conventional topological systems, we focus on the latest frontiers, including non-Hermitian, nonlinear and non-Abelian topology as well as topological defects, for which the characterization of the topological features goes beyond the standard band-topology language. In addition to an overview of the current state of the art, we also survey future research directions for valuable applications.

10.
Nat Commun ; 13(1): 5096, 2022 Aug 30.
Artigo em Inglês | MEDLINE | ID: mdl-36042207

RESUMO

A single-wall carbon nanotube can be viewed as a one-dimensional material created by rolling up a sheet of graphene. Its electronic band structure depends on the chirality, i.e., how the sheet has been rolled up, yet synthesizing the symmetry at will is rather challenging. We structure an artificial honeycomb lattice in both a zigzag and an armchair tube and explore their topological features for sound. Our findings reveal how armchair tubes remain gapless, whereas the zigzag counterparts host nontrivial edge states of non-zero quantized Zak phase, which are dictated by the circumferential number of units. Unlike man-made planar lattices whose underling symmetry must be broken to harvest quantum Hall and pseudospin phases, interestingly, the structured tubular lattice symmetry remains intact, while its nontrivial phase alone is governed by the chirality and the tube diameter. We foresee that our results, not only for sound, but also in photonics, mechanics and electronics will broaden future avenues for fundamental and applied sciences.

11.
Adv Mater ; 34(29): e2202026, 2022 Jul.
Artigo em Inglês | MEDLINE | ID: mdl-35661432

RESUMO

Multiplexing technology with increased information capacity plays a crucial role in the realm of acoustic communication. Different quantities of sound waves, including time, frequency, amplitude, phase, and orbital angular momentum (OAM), have been independently introduced as the physical multiplexing approach to allow for enhanced communication densities. An acoustic metasurface is decorated with carbon nanotube patches, which when electrically pumped and set to rotate, functions as a hybrid mode-frequency-division multiplexer with synthetic dimensions. Based on this spatiotemporal modulation, a superposition of vortex beams with orthogonal OAMs and symmetric harmonics are both numerically and experimentally demonstrated. Also, flexible combinations of OAM modes with diverse frequency shifts are obtained by transforming the azimuthal phase distributions, which inspires a mode-frequency-division multiplexing approach that significantly promotes the communication capacity.

12.
Adv Mater ; 34(28): e2201575, 2022 Jul.
Artigo em Inglês | MEDLINE | ID: mdl-35526115

RESUMO

An ultrasonic motor built with a contactless meta engine block (MEB) is designed and experimentally demonstrated for twisting the linear momentum of sound emanating from a Helmholtz resonator-based metasurface into orbital angular momentum (OAM). The MEB is capable of hosting highly efficient excitations of eigenmodes carrying desired OAM whose Bessel acoustic intensity patterns are enhanced by over ten times compared to the incident wave. Thanks to this efficiency, bidirectional ultrasonic OAM is capable of driving loads at speeds up to 1000 rpm at 4 W and remarkable sound radiation torque levels. Moreover, the possibility of using arbitrarily shaped MEBs is also demonstrated by engineering its physical boundary condition based on an analytically derived criterion to guarantee the high twisting efficiency of man-made OAM. The results show how noninvasive driving of an ultrasonic motor can be made possible through appropriately designed momentum twisting, which opens the door to a new class of integrated mechanical devices solely powered by sound.

13.
Phys Rev Lett ; 127(15): 156401, 2021 Oct 08.
Artigo em Inglês | MEDLINE | ID: mdl-34678007

RESUMO

Dirac cones are essential features of the electronic band structure of materials like graphene and topological insulators (TIs). Lately, this avenue has found a growing interest in classical wave physics by using engineered artificial lattices. Here, we demonstrate an acoustic 3D honeycomb lattice that features a Dirac hierarchy comprising an eightfold bulk Dirac cone, a 2D fourfold surface state Dirac cone, and a 1D twofold hinge state Dirac cone. The lifting of the Dirac degeneracy in each hierarchy authorizes the 3D lattice to appear as a first-order TI with 2D topological surface states, a second-order TI exhibiting 1D hinge states, and a third-order TI of 0D midgap corner states. Analytically we discuss the topological origin of the surface, hinge, and corner states, which are all characterized by out-of-plane and in-plane winding numbers. Our study offers new routes to control sound and vibration for acoustic steering and guiding, on-chip ultrasonic energy concentration, and filtering to name a few.

14.
Phys Rev Lett ; 127(8): 084301, 2021 Aug 20.
Artigo em Inglês | MEDLINE | ID: mdl-34477409

RESUMO

In this Letter, we theoretically propose and experimentally demonstrate a three-dimensional soundproof acoustic cage structure, hereby denoted as an acoustic metacage. The metacage is composed of six acoustic metamaterial slabs with open holes and hidden bypass space coiling tunnels connected to the holes. Band structure analysis reveals a novel physical mechanism to open a low-frequency broad partial band gap via the band folding in other directions, which can also be interpreted by an effective medium with indefinite effective mass density and negative effective modulus. Transmission loss in simulations and in the acoustic impedance tube are administered. Strikingly, we prove that the soundproofing effect of the metacage is robust against the airflow perturbation induced by a fan. Our work paves a road for low-frequency airborne soundproof structures in the presence of ventilation.

15.
Nature ; 597(7878): 655-659, 2021 09.
Artigo em Inglês | MEDLINE | ID: mdl-34588672

RESUMO

In 1878, Lord Rayleigh observed the highly celebrated phenomenon of sound waves that creep around the curved gallery of St Paul's Cathedral in London1,2. These whispering-gallery waves scatter efficiently with little diffraction around an enclosure and have since found applications in ultrasonic fatigue and crack testing, and in the optical sensing of nanoparticles or molecules using silica microscale toroids. Recently, intense research efforts have focused on exploring non-Hermitian systems with cleverly matched gain and loss, facilitating unidirectional invisibility and exotic characteristics of exceptional points3,4. Likewise, the surge in physics using topological insulators comprising non-trivial symmetry-protected phases has laid the groundwork in reshaping highly unconventional avenues for robust and reflection-free guiding and steering of both sound and light5,6. Here we construct a topological gallery insulator using sonic crystals made of thermoplastic rods that are decorated with carbon nanotube films, which act as a sonic gain medium by virtue of electro-thermoacoustic coupling. By engineering specific non-Hermiticity textures to the activated rods, we are able to break the chiral symmetry of the whispering-gallery modes, which enables the out-coupling of topological 'audio lasing' modes with the desired handedness. We foresee that these findings will stimulate progress in non-destructive testing and acoustic sensing.

16.
Nat Commun ; 12(1): 3670, 2021 Jun 16.
Artigo em Inglês | MEDLINE | ID: mdl-34135332

RESUMO

Transceiving ultra-weak sound typically relies on signal pre-amplification at the transmitting end via active electro-acoustic devices, which inherently perturbs the environment in the form of noise that inevitably leads to information leakage. Here we demonstrate a passive remote-whispering metamaterial (RWM) enabling weak airborne sound at audible frequencies to reach unprecedented signal enhancement without altering the detected ambient soundscape, which is based on the extraordinary scattering properties of a metamaterial formed by a pair of self-resonating subwavelength Mie meta-cavities, constituting the acoustic analogy of Förster resonance energy transfer. We demonstrate efficient non-radiative sound transfer over distances hundreds times longer than the radius of the meta-cavities, which enables the RWM to recover weak sound signals completely overwhelmed by strong noise with enhanced signal-to-noise ratio from -3 dB below the detection limit of 0 dB in free space to 17.7 dB.

17.
Nat Nanotechnol ; 16(5): 487-489, 2021 05.
Artigo em Inglês | MEDLINE | ID: mdl-33875871
18.
ACS Appl Mater Interfaces ; 13(15): 17753-17765, 2021 Apr 21.
Artigo em Inglês | MEDLINE | ID: mdl-33822572

RESUMO

Humans primarily interact with information technology through glass touch screens, and the world would indeed be unrecognizable without glass. However, the low toughness of oxide glasses continues to be their Achilles heel, limiting both future applications and the possibility to make thinner, more environmentally friendly glasses. Here, we show that with proper control of plasticity mechanisms, record-high values of fracture toughness for transparent bulk oxide glasses can be achieved. Through proper combination of gas-mediated permanent densification and rational composition design, we increase the glasses' propensity for plastic deformation. Specifically, we demonstrate a fracture toughness of an aluminoborate glass (1.4 MPa m0.5) that is twice as high as that of commercial glasses for mobile devices. Atomistic simulations reveal that the densification of the adaptive aluminoborate network increases coordination number changes and bond swapping, ultimately enhancing plasticity and toughness upon fracture. Our findings thus provide general insights into the intrinsic toughening mechanisms of oxide glasses.

19.
Phys Rev Lett ; 125(21): 214301, 2020 Nov 20.
Artigo em Inglês | MEDLINE | ID: mdl-33275023

RESUMO

Twisted bilayer graphene develops quasiflat bands at specific "magic" interlayer rotation angles through an unconventional mechanism connected to carrier chirality. Quasiflat bands are responsible for a wealth of exotic, correlated-electron phases in the system. In this Letter, we propose a mechanical analog of twisted bilayer graphene made of two vibrating plates patterned with a honeycomb mesh of masses and coupled across a continuum elastic medium. We show that flexural waves in the device exhibit vanishing group velocity and quasiflat bands at magic angles in close correspondence with electrons in graphene models. The strong similarities of spectral structure and spatial eigenmodes in the two systems demonstrate the chiral nature of the mechanical flat bands. We derive analytical expressions that quantitatively connect the mechanical and electronic models, which allow us to predict the parameters required for an experimental realization of our proposal.

20.
Phys Rev Lett ; 125(20): 206402, 2020 Nov 13.
Artigo em Inglês | MEDLINE | ID: mdl-33258615

RESUMO

The bulk-boundary or bulk-edge correspondence is a principle relating surface confined states to the topological classification of the bulk. By marrying non-Hermitian ingredients in terms of gain or loss with media that violate reciprocity, an unconventional non-Bloch bulk-boundary correspondence leads to unusual localization of bulk states at boundaries-a phenomenon coined non-Hermitian skin effect. Here, we numerically employ the acoustoelectric effect in electrically biased and layered piezophononic media as a solid framework for non-Hermitian and nonreciprocal topological mechanics in the MHz regime. Thanks to a non-Hermitian skin effect for mechanical vibrations, we find that the bulk bands of finite systems are highly sensitive to the type of crystal termination, which indicates a failure of using traditional Bloch bands to predict the wave characteristics. More surprisingly, when reversing the electrical bias, we unveil how topological edge and bulk vibrations can be harnessed either at the same or opposite interfaces. Yet, while bulk states are found to display this unconventional skin effect, we further discuss how in-gap edge states in the same instant, counterintuitively are able to delocalize along the entire layered medium. We foresee that our predictions will stimulate new avenues in echo-less ultrasonics based on exotic wave physics.

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