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1.
Entropy (Basel) ; 24(8)2022 Aug 17.
Artigo em Inglês | MEDLINE | ID: mdl-36010807

RESUMO

We present a comprehensive simulation study of the Newtonian and quantum model of a Stern-Gerlach experiment with cold neutrons. By solving Newton's equation of motion and the time-dependent Pauli equation for a wide range of uniform magnetic field strengths, we scrutinize the role of the latter for drawing the conclusion that the magnetic moment of the neutron is quantized. We then demonstrate that a marginal modification of the Newtonian model suffices to construct, without invoking any concept of quantum theory, an event-based subquantum model that eliminates the shortcomings of the classical model and yields results that are in qualitative agreement with experiment and quantum theory. In this event-by-event model, the intrinsic angular momentum can take any value on the sphere, yet, for a sufficiently strong uniform magnetic field, the particle beam splits in two, exactly as in experiment and in concert with quantum theory.

2.
Phys Rev E ; 101(6-1): 062133, 2020 Jun.
Artigo em Inglês | MEDLINE | ID: mdl-32688487

RESUMO

Given a quantum many-body system and the expectation-value dynamics of some operator, we study how this reference dynamics is altered due to a perturbation of the system's Hamiltonian. Based on projection operator techniques, we unveil that if the perturbation exhibits a random-matrix structure in the eigenbasis of the unperturbed Hamiltonian, then this perturbation effectively leads to an exponential damping of the original dynamics. Employing a combination of dynamical quantum typicality and numerical linked cluster expansions, we demonstrate that our theoretical findings for random matrices can, in some cases, be relevant for the dynamics of realistic quantum many-body models as well. Specifically, we study the decay of current autocorrelation functions in spin-1/2 ladder systems, where the rungs of the ladder are treated as a perturbation to the otherwise uncoupled legs. We find a convincing agreement between the exact dynamics and the lowest-order prediction over a wide range of interchain couplings.

3.
Sci Rep ; 9(1): 6521, 2019 Apr 19.
Artigo em Inglês | MEDLINE | ID: mdl-31000781

RESUMO

A correction to this article has been published and is linked from the HTML and PDF versions of this paper. The error has not been fixed in the paper.

4.
Sci Rep ; 9(1): 1939, 2019 02 13.
Artigo em Inglês | MEDLINE | ID: mdl-30760789

RESUMO

When transmitting polarised light through histological brain sections, different types of diattenuation (polarisation-dependent attenuation of light) can be observed: In some brain regions, the light is minimally attenuated when it is polarised parallel to the nerve fibres (referred to as D+), in others, it is maximally attenuated (referred to as D-). The underlying mechanisms of these effects and their relationship to tissue properties were so far unknown. Here, we demonstrate in experimental studies that diattenuation of both types D+ and D- can be observed in brain tissue samples from different species (rodent, monkey, and human) and that the strength and type of diattenuation depend on the nerve fibre orientations. By combining finite-difference time-domain simulations and analytical modelling, we explain the observed diattenuation effects and show that they are caused both by anisotropic absorption (dichroism) and by anisotropic light scattering. Our studies demonstrate that the diattenuation signal depends not only on the nerve fibre orientations but also on other brain tissue properties like tissue homogeneity, fibre size, and myelin sheath thickness. This allows to use the diattenuation signal to distinguish between brain regions with different tissue properties and establishes Diattenuation Imaging as a valuable imaging technique.


Assuntos
Encéfalo/diagnóstico por imagem , Microscopia de Polarização/métodos , Fibras Nervosas/fisiologia , Animais , Anisotropia , Axônios/fisiologia , Chlorocebus aethiops , Simulação por Computador , Humanos , Camundongos , Bainha de Mielina/fisiologia , Fibras Nervosas Mielinizadas/fisiologia , Ratos
5.
Phys Chem Chem Phys ; 19(37): 25391-25400, 2017 Sep 27.
Artigo em Inglês | MEDLINE | ID: mdl-28894860

RESUMO

A quartz-crystal-microbalance with dissipation (QCM-D) can measure molecular mass adsorption as well as register adhesion of colloidal particles. However, analysis of the QCM-D output to quantitatively analyze adhesion of (bio)colloids to obtain viscoelastic bond properties is still a subject of debate. Here, we analyze the QCM-D output to analyze the bond between two hydrophilic streptococcal strains 91 nm long and without fibrillar surface appendages and micron-sized hydrophobic polystyrene particles on QCM-D crystal surfaces with different hydrophobicities, using the Kelvin-Voigt model and the Maxwell model. A Poisson distribution was implemented in order to determine the possible virtues of including polydispersity when fitting model parameters to the data. The quality of the fits did not indicate whether the Kelvin-Voigt or the Maxwell model is preferable and only polydispersity in spring-constants improved the fit for polystyrene particles. The Kelvin-Voigt and Maxwell models both yielded higher spring-constants for the bald streptococcus than for the fibrillated one. In both models, the drag coefficients increased for the bald streptococcus with the ratio of electron-donating over electron-accepting parameters of the crystal surface, while for the fibrillated strain the drag coefficient was similar on all crystal surfaces. Combined with the propensity of fibrillated streptococci to bind to the sensor crystal as a coupled-resonator above the crystal surface, this suggests that the drag experienced by resonator-coupled, hydrophilic particles is more influenced by the viscosity of the bulk water than by interfacial water adjacent to the crystal surface. Hydrophilic particles that lack a surface tether are mass-coupled just above the crystal surface and accordingly probe the drag due to the thin layer of interfacial water that is differently structured on hydrophobic and hydrophilic surfaces. Hydrophobic particles without a surface tether are also mass-coupled, but their drag coefficient decreases when the ratio of electron-donating over electron-accepting parameters increases, suggesting that hydrophobic particles experience less drag due to the structured water adjacent to the surface.

6.
Colloids Surf B Biointerfaces ; 148: 255-262, 2016 Dec 01.
Artigo em Inglês | MEDLINE | ID: mdl-27616066

RESUMO

The quartz-crystal-microbalance-with-dissipation (QCM-D) has become a powerful tool for studying the bond viscoelasticity of biotic and abiotic colloidal particles adhering to substratum surfaces. A window-equipped QCM-D allows high-throughput analysis of the average bond viscoelasticity, measuring over 106 particles simultaneously in one single experiment. Other techniques require laborious analyses of individual particles. In this protocol, the quantitative derivation of the spring-constant and drag-coefficient of the bond between adhering colloidal particles and substratum surfaces using QCM-D is explained for bacteria and silica particles, using the particle-mass derived for validation. Bond viscoelasticity is calculated using a coupled resonator model, paying special attention to the protocol for mathematical fitting needed to obtain reliable quantitative output. Knowledge of the viscoelasticity of the bond between colloidal particles and substratum surfaces facilitates development of new strategies to detach adhering particles from or retain them on a surface.


Assuntos
Aderência Bacteriana , Elasticidade , Técnicas de Microbalança de Cristal de Quartzo , Viscosidade
7.
Proc Natl Acad Sci U S A ; 111(12): 4363-8, 2014 Mar 25.
Artigo em Inglês | MEDLINE | ID: mdl-24591592

RESUMO

Birds-of-paradise are nature's prime examples of the evolution of color by sexual selection. Their brilliant, structurally colored feathers play a principal role in mating displays. The structural coloration of both the occipital and breast feathers of the bird-of-paradise Lawes' parotia is produced by melanin rodlets arranged in layers, together acting as interference reflectors. Light reflection by the silvery colored occipital feathers is unidirectional as in a classical multilayer, but the reflection by the richly colored breast feathers is three-directional and extraordinarily complex. Here we show that the reflection properties of both feather types can be quantitatively explained by finite-difference time-domain modeling using realistic feather anatomies and experimentally determined refractive index dispersion values of keratin and melanin. The results elucidate the interplay between avian coloration and vision and indicate tuning of the mating displays to the spectral properties of the avian visual system.


Assuntos
Aves/anatomia & histologia , Cor , Plumas , Modelos Teóricos , Animais , Aves/fisiologia , Comportamento Sexual Animal , Visão Ocular
8.
Artigo em Inglês | MEDLINE | ID: mdl-24580196

RESUMO

A key feature of nonequilibrium thermodynamics is the Markovian, deterministic relaxation of coarse observables such as, for example, the temperature difference between two macroscopic objects which evolves independently of almost all details of the initial state. We demonstrate that the unitary dynamics for moderately sized spin-1/2 systems may yield the same type of relaxation dynamics for a given magnetization difference. This observation might contribute to the understanding of the emergence of thermodynamics within closed quantum systems.


Assuntos
Algoritmos , Cadeias de Markov , Modelos Estatísticos , Teoria Quântica , Marcadores de Spin , Temperatura , Termodinâmica , Simulação por Computador
9.
PLoS One ; 7(11): e49743, 2012.
Artigo em Inglês | MEDLINE | ID: mdl-23185423

RESUMO

Mature male Calopteryx japonica damselflies have dark-blue wings, due to darkly coloured wing membranes and blue reflecting veins. The membranes contain a high melanin concentration and the veins have a multilayer of melanin and chitin. Female and immature C. japonica damselflies have brown wings. We have determined the refractive index of melanin by comparing the differently pigmented wing membranes and applying Jamin-Lebedeff interference microscopy. Together with the previously measured refractive index of chitin the blue, structural colour of the male wing veins could be quantitatively explained by an optical multilayer model. The obtained melanin refractive index data will be useful in optical studies on melanized tissues, especially where melanin is concentrated in layers, thus causing iridescence.


Assuntos
Quitina/metabolismo , Melaninas/metabolismo , Odonatos/genética , Asas de Animais/fisiologia , Animais , Cor , Feminino , Masculino , Microscopia Eletrônica de Transmissão/métodos , Pigmentação , Refratometria , Caracteres Sexuais , Espectrofotometria/métodos
10.
Proc Biol Sci ; 279(1738): 2524-30, 2012 Jul 07.
Artigo em Inglês | MEDLINE | ID: mdl-22378806

RESUMO

The neotropical diamond weevil, Entimus imperialis, is marked by rows of brilliant spots on the overall black elytra. The spots are concave pits with intricate patterns of structural-coloured scales, consisting of large domains of three-dimensional photonic crystals that have a diamond-type structure. Reflectance spectra measured from individual scale domains perfectly match model spectra, calculated with anatomical data and finite-difference time-domain methods. The reflections of single domains are extremely directional (observed with a point source less than 5°), but the special arrangement of the scales in the concave pits significantly broadens the angular distribution of the reflections. The resulting virtually angle-independent green coloration of the weevil closely approximates the colour of a foliaceous background. While the close-distance colourful shininess of E. imperialis may facilitate intersexual recognition, the diffuse green reflectance of the elytra when seen at long-distance provides cryptic camouflage.


Assuntos
Comportamento Animal , Besouros/ultraestrutura , Fótons , Pigmentação , Asas de Animais/ultraestrutura , Animais , Besouros/química , Besouros/fisiologia , Simulação por Computador , Cristalização , Microscopia Eletrônica de Transmissão , Refratometria , Asas de Animais/química
11.
Interface Focus ; 2(5): 681-7, 2012 Oct 06.
Artigo em Inglês | MEDLINE | ID: mdl-24098853

RESUMO

The cover scales on the wing of the Emerald-patched Cattleheart butterfly, Parides sesostris, contain gyroid-type biological photonic crystals that brightly reflect green light. A pigment, which absorbs maximally at approximately 395 nm, is immersed predominantly throughout the elaborate upper lamina. This pigment acts as a long-pass filter shaping the reflectance spectrum of the underlying photonic crystals. The additional effect of the filtering is that the spatial distribution of the scale reflectance is approximately angle-independent, leading to a stable wing pattern contrast. The spectral tuning of the original reflectance is verified by photonic band structure modelling.

12.
J R Soc Interface ; 9(72): 1609-14, 2012 Jul 07.
Artigo em Inglês | MEDLINE | ID: mdl-22188768

RESUMO

The brilliant structural body colours of many animals are created by three-dimensional biological photonic crystals that act as wavelength-specific reflectors. Here, we report a study on the vividly coloured scales of the diamond weevil, Entimus imperialis. Electron microscopy identified the chitin and air assemblies inside the scales as domains of a single-network diamond (Fd3m) photonic crystal. We visualized the topology of the first Brillouin zone (FBZ) by imaging scatterometry, and we reconstructed the complete photonic band structure diagram (PBSD) of the chitinous photonic crystal from reflectance spectra. Comparison with calculated PBSDs indeed showed a perfect overlap. The unique method of non-invasive hemispherical imaging of the FBZ provides key insights for the investigation of photonic crystals in the visible wavelength range. The characterized extremely large biophotonic nanostructures of E. imperialis are structurally optimized for high reflectance and may thus be well suited for use as a template for producing novel photonic devices, e.g. through biomimicry or direct infiltration from dielectric material.


Assuntos
Quitina/química , Besouros/química , Nanoestruturas/química , Pigmentação , Animais , Quitina/ultraestrutura , Besouros/ultraestrutura , Microscopia Eletrônica , Nanoestruturas/ultraestrutura
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