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1.
Phys Rev Lett ; 123(21): 216404, 2019 Nov 22.
Artigo em Inglês | MEDLINE | ID: mdl-31809140

RESUMO

Quasiparticle interference (QPI) provides a wealth of information relating to the electronic structure of a material. However, it is often assumed that this information is constrained to two-dimensional electronic states. We show that this is not necessarily the case. For FeSe, a system dominated by surface defects, we show that it is actually all electronic states with negligible group velocity in the z axis that are contained within the experimental data. By using a three-dimensional tight-binding model of FeSe, fit to photoemission measurements, we directly reproduce the experimental QPI scattering dispersion, within a T-matrix formalism, by including both k_{z}=0 and k_{z}=π electronic states. This result unifies both tunnelling based and photoemission based experiments on FeSe and highlights the importance of k_{z} within surface sensitive measurements of QPI.

2.
Nat Mater ; 17(6): 499-503, 2018 06.
Artigo em Inglês | MEDLINE | ID: mdl-29662156

RESUMO

Unlike conventional spin-singlet Cooper pairs, spin-triplet pairs can carry spin1,2. Triplet supercurrents were discovered in Josephson junctions with metallic ferromagnet spacers, where spin transport can occur only within the ferromagnet and in conjunction with a charge current. Ferromagnetic resonance injects a pure spin current from a precessing ferromagnet into adjacent non-magnetic materials3,4. For spin-singlet pairing, the ferromagnetic resonance spin pumping efficiency decreases below the critical temperature (Tc) of a coupled superconductor5,6. Here we present ferromagnetic resonance experiments in which spin sink layers with strong spin-orbit coupling are added to the superconductor. Our results show that the induced spin currents, rather than being suppressed, are substantially larger in the superconducting state compared with the normal state; although further work is required to establish the details of the spin transport process, we show that this cannot be mediated by quasiparticles and is most likely a triplet pure spin supercurrent.

3.
Sci Rep ; 7(1): 1932, 2017 05 16.
Artigo em Inglês | MEDLINE | ID: mdl-28512309

RESUMO

Interfacing superconductors with strongly spin-polarized magnetic materials opens the possibility to discover new spintronic devices in which spin-triplet Cooper pairs play a key role. Motivated by the recent derivation of spin-polarized quasiclassical boundary conditions capable of describing such a scenario in the diffusive limit, we consider the emergent physics in hybrid structures comprised of a conventional s-wave superconductor (e.g. Nb, Al) and either strongly spin-polarized ferromagnetic insulators (e.g. EuO, GdN) or halfmetallic ferromagnets (e.g. CrO2, LCMO). In contrast to most previous works, we focus on how the superconductor itself is influenced by the proximity effect, and how the generated triplet Cooper pairs manifest themselves in the self-consistently computed density of states (DOS) and the superconducting critical temperature T c . We provide a comprehensive treatment of how the superconductor and its properties are affected by the triplet pairs, demonstrating that our theory can reproduce the recent observation of an unusually large zero-energy peak in a superconductor interfaced with a half-metal, which even exceeds the normal-state DOS. We also discuss the recent observation of a large superconducting spin-valve effect with a T c change ~1 K in superconductor/half-metal structures, in which case our results indicate that the experiment cannot be explained fully by a long-ranged triplet proximity effect.

4.
Rep Prog Phys ; 78(10): 104501, 2015 Oct.
Artigo em Inglês | MEDLINE | ID: mdl-26397456

RESUMO

During the past 15 years a new field has emerged, which combines superconductivity and spintronics, with the goal to pave a way for new types of devices for applications combining the virtues of both by offering the possibility of long-range spin-polarized supercurrents. Such supercurrents constitute a fruitful basis for the study of fundamental physics as they combine macroscopic quantum coherence with microscopic exchange interactions, spin selectivity, and spin transport. This report follows recent developments in the controlled creation of long-range equal-spin triplet supercurrents in ferromagnets and its contribution to spintronics. The mutual proximity-induced modification of order in superconductor-ferromagnet hybrid structures introduces in a natural way such evasive phenomena as triplet superconductivity, odd-frequency pairing, Fulde-Ferrell-Larkin-Ovchinnikov pairing, long-range equal-spin supercurrents, [Formula: see text]-Josephson junctions, as well as long-range magnetic proximity effects. All these effects were rather exotic before 2000, when improvements in nanofabrication and materials control allowed for a new quality of hybrid structures. Guided by pioneering theoretical studies, experimental progress evolved rapidly, and since 2010 triplet supercurrents are routinely produced and observed. We have entered a new stage of studying new phases of matter previously out of our reach, and of merging the hitherto disparate fields of superconductivity and spintronics to a new research direction: super-spintronics.

5.
Phys Rev Lett ; 106(4): 047003, 2011 Jan 28.
Artigo em Inglês | MEDLINE | ID: mdl-21405349

RESUMO

Recently, experimental studies of the spin excitation spectrum revealed a strong temperature dependence in the normal state and a resonance feature in the superconducting state of several Fe-based superconductors. Based on these findings, we develop a model of electrons interacting with a temperature dependent magnetic excitation spectrum and apply it to angle resolved photoemission in Ba(1-x)K(x)Fe(2)As(2). We reproduce in quantitative agreement with experiment a renormalization of the quasiparticle dispersion both in the normal and the superconducting state, and the dependence of the quasiparticle linewidth on binding energy. We estimate the strength of the coupling between electronic and spin excitations. Our findings support a dominantly magnetic pairing mechanism.

6.
Phys Rev Lett ; 105(20): 207001, 2010 Nov 12.
Artigo em Inglês | MEDLINE | ID: mdl-21231255

RESUMO

We report an extensive theoretical analysis of point-contact Andreev reflection data available in the literature on ferromagnetic CrO2. We find that the spectra can be well understood within a model of fully spin-polarized bands in CrO2 together with spin-active scattering at the contact. This is in contrast to analysis of the data within extended Blonder-Tinkham-Klapwijk models, which lead to a spin polarization varying between 50% and 100% depending on the transparency of the interface. We propose to utilize both the temperature dependence of the spectra and the excess current at voltages above the gap to resolve the spin polarization in CrO2 in a new generation of experiments.

7.
Phys Rev Lett ; 102(10): 107008, 2009 Mar 13.
Artigo em Inglês | MEDLINE | ID: mdl-19392152

RESUMO

We study the proximity-induced superconducting correlations in a normal metal connected to a superconductor when the interface between them is spin active and the normal metal is ballistic or diffusive. Remarkably, for any interface spin polarization there is a critical interface resistance, above which the conventional even-frequency proximity component vanishes completely at the chemical potential, while the odd-frequency component remains finite. We propose a way to unambiguously observe the odd-frequency component.

8.
Phys Rev Lett ; 100(7): 077003, 2008 Feb 22.
Artigo em Inglês | MEDLINE | ID: mdl-18352588

RESUMO

We study the pi phase in a superconductor-ferromagnet-superconductor Josephson junction, with a ferromagnet showing a cycloidal spiral spin modulation with in-plane propagation vector. Our results reveal a high sensitivity of the junction to the spiral order and indicate the presence of 0-pi quantum phase transitions as function of the spiral wave vector. We find that the chiral magnetic order introduces chiral superconducting triplet pairs that strongly influence the physics in such Josephson junctions, with potential applications in nanoelectronics and spintronics.

9.
Phys Rev Lett ; 95(18): 187003, 2005 Oct 28.
Artigo em Inglês | MEDLINE | ID: mdl-16383937

RESUMO

We present theoretical results on the interplay of magnetic and superconducting orders in diffusive ferromagnet-superconductor-ferromagnet trilayers. The induced triplet superconducting correlations throughout the trilayer lead to an induced spin magnetization. We include self-consistency of the order parameter in the superconducting layer at arbitrary temperatures, arbitrary interface transparency, and any relative orientation of the exchange fields in the two ferromagnets. We propose to use the torque on the trilayer in an external magnetic field as a probe of the presence of triplet correlations in the superconducting phase.

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