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1.
Environ Sci Technol ; 46(8): 4275-82, 2012 Apr 17.
Artigo em Inglês | MEDLINE | ID: mdl-22380547

RESUMO

In jurisdictions including the US and the EU ground transportation and marine fuels have recently been required to contain lower concentrations of sulfur, which has resulted in reduced atmospheric SO(x) emissions. In contrast, the maximum sulfur content of aviation fuel has remained unchanged at 3000 ppm (although sulfur levels average 600 ppm in practice). We assess the costs and benefits of a potential ultra-low sulfur (15 ppm) jet fuel standard ("ULSJ"). We estimate that global implementation of ULSJ will cost US$1-4bn per year and prevent 900-4000 air quality-related premature mortalities per year. Radiative forcing associated with reduction in atmospheric sulfate, nitrate, and ammonium loading is estimated at +3.4 mW/m(2) (equivalent to about 1/10th of the warming due to CO(2) emissions from aviation) and ULSJ increases life cycle CO(2) emissions by approximately 2%. The public health benefits are dominated by the reduction in cruise SO(x) emissions, so a key uncertainty is the atmospheric modeling of vertical transport of pollution from cruise altitudes to the ground. Comparisons of modeled and measured vertical profiles of CO, PAN, O(3), and (7)Be indicate that this uncertainty is low relative to uncertainties regarding the value of statistical life and the toxicity of fine particulate matter.


Assuntos
Poluentes Atmosféricos/normas , Poluição do Ar/prevenção & controle , Hidrocarbonetos/normas , Óxidos de Enxofre/normas , Enxofre/normas , Poluentes Atmosféricos/economia , Poluentes Atmosféricos/toxicidade , Poluição do Ar/economia , Poluição do Ar/legislação & jurisprudência , Mudança Climática , Análise Custo-Benefício , Humanos , Modelos Teóricos , Material Particulado/economia , Material Particulado/normas , Material Particulado/toxicidade , Enxofre/economia , Óxidos de Enxofre/economia , Incerteza
2.
J Air Waste Manag Assoc ; 59(1): 91-100, 2009 Jan.
Artigo em Inglês | MEDLINE | ID: mdl-19216192

RESUMO

Today, about one-fourth of U.S. commercial service airports, including 41 of the busiest 50, are either in nonattainment or maintenance areas per the National Ambient Air Quality Standards. U.S. aviation activity is forecasted to triple by 2025, while at the same time, the U.S. Environmental Protection Agency (EPA) is evaluating stricter particulate matter (PM) standards on the basis of documented human health and welfare impacts. Stricter federal standards are expected to impede capacity and limit aviation growth if regulatory mandated emission reductions occur as for other non-aviation sources (i.e., automobiles, power plants, etc.). In addition, strong interest exists as to the role aviation emissions play in air quality and climate change issues. These reasons underpin the need to quantify and understand PM emissions from certified commercial aircraft engines, which has led to the need for a methodology to predict these emissions. Standardized sampling techniques to measure volatile and nonvolatile PM emissions from aircraft engines do not exist. As such, a first-order approximation (FOA) was derived to fill this need based on available information. FOA1.0 only allowed prediction of nonvolatile PM. FOA2.0 was a change to include volatile PM emissions on the basis of the ratio of nonvolatile to volatile emissions. Recent collaborative efforts by industry (manufacturers and airlines), research establishments, and regulators have begun to provide further insight into the estimation of the PM emissions. The resultant PM measurement datasets are being analyzed to refine sampling techniques and progress towards standardized PM measurements. These preliminary measurement datasets also support the continued refinement of the FOA methodology. FOA3.0 disaggregated the prediction techniques to allow for independent prediction of nonvolatile and volatile emissions on a more theoretical basis. The Committee for Aviation Environmental Protection of the International Civil Aviation Organization endorsed the use of FOA3.0 in February 2007. Further commitment was made to improve the FOA as new data become available, until such time the methodology is rendered obsolete by a fully validated database of PM emission indices for today's certified commercial fleet. This paper discusses related assumptions and derived equations for the FOA3.0 methodology used worldwide to estimate PM emissions from certified commercial aircraft engines within the vicinity of airports.


Assuntos
Poluentes Atmosféricos/análise , Aeronaves , Monitoramento Ambiental/métodos , Material Particulado/análise , Emissões de Veículos/análise , Poluentes Atmosféricos/química , Gasolina/análise , Material Particulado/química , Fuligem/análise , Fuligem/química , Enxofre/análise , Enxofre/química , Estados Unidos , United States Environmental Protection Agency , Volatilização
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